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Non-contact thermometry with Dy3+ doped Gd2Ti2O7 nano-powders

Authorized Users Only
2016
Authors
Ćulubrk, Sanja
Lojpur, Vesna
Ahrenkiel, Scott Phillip
Nedeljković, Jovan
Dramićanin, Miroslav
Article
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Abstract
The performance of Dy3+ doped Gd2Ti2O7 nano-powders for luminescence temperature sensing was tested over a temperature range from 293 to 443 K. The Dy3+ ions were incorporated into Gd2Ti2O7 nanocrystals using a hydrolytic sal-gel route. Microstructural characterization of the obtained material was performed using transmission electron microscopy and X-ray diffraction measurements. Luminescence spectra of Dy3+ doped Gd2Ti2O7 nano-powders consists of two distinct spectral regions: the highenergy region associated with the trap emission of the Gd2Ti2O7 host and the low-energy region with well-resolved emission peaks of the Dy3+ ions. The ratio between intensities of two Dy3+ emission lines, as well as the ratio between intensities of trap emission of host and Dy3+ emission show strong temperature dependence and are tested for temperature sensing. In both cases, ratiometric measurements provide comparable quality of temperature sensing, and when they are combined the relative sensor sensit...ivities were found to be higher than 0.9% K-1 over given temperature range. The fluorescence quenching of Dy3+ ions was discussed in terms of simple theoretical models. (C) 2015 Elsevier B.V. All rights reserved.

Keywords:
Luminescence thermometry / Nanomaterials / Luminescence / Rare earths / Pyrochlores
Source:
Journal of Luminescence, 2016, 170, SI, 395-400
Projects:
  • Materials of Reduced Dimensions for Efficient Light Harvesting and Energy conversion (RS-45020)

DOI: 10.1016/j.jlumin.2015.06.006

ISSN: 0022-2313; 1872-7883

WoS: 000367638500010

Scopus: 2-s2.0-84954382199
[ Google Scholar ]
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42
URI
http://vinar.vin.bg.ac.rs/handle/123456789/877
Collections
  • WoS Import
Institution
Vinča
TY  - JOUR
AU  - Ćulubrk, Sanja
AU  - Lojpur, Vesna
AU  - Ahrenkiel, Scott Phillip
AU  - Nedeljković, Jovan
AU  - Dramićanin, Miroslav
PY  - 2016
UR  - http://vinar.vin.bg.ac.rs/handle/123456789/877
AB  - The performance of Dy3+ doped Gd2Ti2O7 nano-powders for luminescence temperature sensing was tested over a temperature range from 293 to 443 K. The Dy3+ ions were incorporated into Gd2Ti2O7 nanocrystals using a hydrolytic sal-gel route. Microstructural characterization of the obtained material was performed using transmission electron microscopy and X-ray diffraction measurements. Luminescence spectra of Dy3+ doped Gd2Ti2O7 nano-powders consists of two distinct spectral regions: the highenergy region associated with the trap emission of the Gd2Ti2O7 host and the low-energy region with well-resolved emission peaks of the Dy3+ ions. The ratio between intensities of two Dy3+ emission lines, as well as the ratio between intensities of trap emission of host and Dy3+ emission show strong temperature dependence and are tested for temperature sensing. In both cases, ratiometric measurements provide comparable quality of temperature sensing, and when they are combined the relative sensor sensitivities were found to be higher than 0.9% K-1 over given temperature range. The fluorescence quenching of Dy3+ ions was discussed in terms of simple theoretical models. (C) 2015 Elsevier B.V. All rights reserved.
T2  - Journal of Luminescence
T1  - Non-contact thermometry with Dy3+ doped Gd2Ti2O7 nano-powders
VL  - 170
IS  - SI
SP  - 395
EP  - 400
DO  - 10.1016/j.jlumin.2015.06.006
ER  - 
@article{
author = "Ćulubrk, Sanja and Lojpur, Vesna and Ahrenkiel, Scott Phillip and Nedeljković, Jovan and Dramićanin, Miroslav",
year = "2016",
url = "http://vinar.vin.bg.ac.rs/handle/123456789/877",
abstract = "The performance of Dy3+ doped Gd2Ti2O7 nano-powders for luminescence temperature sensing was tested over a temperature range from 293 to 443 K. The Dy3+ ions were incorporated into Gd2Ti2O7 nanocrystals using a hydrolytic sal-gel route. Microstructural characterization of the obtained material was performed using transmission electron microscopy and X-ray diffraction measurements. Luminescence spectra of Dy3+ doped Gd2Ti2O7 nano-powders consists of two distinct spectral regions: the highenergy region associated with the trap emission of the Gd2Ti2O7 host and the low-energy region with well-resolved emission peaks of the Dy3+ ions. The ratio between intensities of two Dy3+ emission lines, as well as the ratio between intensities of trap emission of host and Dy3+ emission show strong temperature dependence and are tested for temperature sensing. In both cases, ratiometric measurements provide comparable quality of temperature sensing, and when they are combined the relative sensor sensitivities were found to be higher than 0.9% K-1 over given temperature range. The fluorescence quenching of Dy3+ ions was discussed in terms of simple theoretical models. (C) 2015 Elsevier B.V. All rights reserved.",
journal = "Journal of Luminescence",
title = "Non-contact thermometry with Dy3+ doped Gd2Ti2O7 nano-powders",
volume = "170",
number = "SI",
pages = "395-400",
doi = "10.1016/j.jlumin.2015.06.006"
}
Ćulubrk S, Lojpur V, Ahrenkiel SP, Nedeljković J, Dramićanin M. Non-contact thermometry with Dy3+ doped Gd2Ti2O7 nano-powders. Journal of Luminescence. 2016;170(SI):395-400
Ćulubrk, S., Lojpur, V., Ahrenkiel, S. P., Nedeljković, J.,& Dramićanin, M. (2016). Non-contact thermometry with Dy3+ doped Gd2Ti2O7 nano-powders.
Journal of Luminescence, 170(SI), 395-400.
https://doi.org/10.1016/j.jlumin.2015.06.006
Ćulubrk Sanja, Lojpur Vesna, Ahrenkiel Scott Phillip, Nedeljković Jovan, Dramićanin Miroslav, "Non-contact thermometry with Dy3+ doped Gd2Ti2O7 nano-powders" 170, no. SI (2016):395-400,
https://doi.org/10.1016/j.jlumin.2015.06.006 .

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