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Electrocatalytic Activity of Ionic-Liquid-Derived Porous Carbon Materials for the Oxygen Reduction Reaction

Authorized Users Only
2018
Authors
Zdolšek, Nikola
Dimitrijević, Aleksandra
Bendova, Magdalena
Krstić, Jugoslav B.
Rocha, Raquel P.
Figueiredo, Jose L.
Bajuk-Bogdanović, Danica V.
Trtić-Petrović, Tatjana M.
Šljukić, Biljana
Article (Published version)
,
© 2018 Wiley‐VCH Verlag GmbH & Co. KGaA, Weinheim
Metadata
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Abstract
Carbon materials, prepared by using different methods with ionicliquids, are compared as electrocatalysts for the oxygen reductionreaction (ORR). Materials were synthesized through the hydrothermalcarbonization of glucose and by using the same method in the presence of1-butyl-3-methylimidazolium methanesulfonate {[}bmim]{[}MeSO3] as anadditive. Another two carbon-based materials were prepared by usingionic-liquid-based methods: ionothermal carbonization of glucose using{[}bmim]{[}MeSO3] as a recyclable medium for the carbonization reactionand by direct carbonization of the ionic liquid in a one-step methodusing {[}bmim]{[}MeSO3] as the precursor for N- and S-doped porouscarbon (Carb-IL). Characterization results showed the possibility ofmorphology and porosity control by using {[}bmim]{[}MeSO3]. Allmaterials were subsequently tested for the ORR in alkaline media.Carb-IL showed enhanced and stable electrocatalytic ORR activity, evenin the presence of methanol, ethanol, and borohydride, ...opening thepossibility for its application in fuel cells.

Keywords:
ionic liquids / porous carbon materials / fuel cells / ionothermal carbonization / oxygen reduction reaction
Source:
ChemElectroChem, 2018, 5, 7, 1037-1046
Funding / projects:
  • Physics and Chemistry with Ion Beams (RS-45006)
  • Lithium-ion batteries and fuel cells - research and development (RS-45014)
  • Nanostructured Functional and Composite Materials in Catalytic and Sorption Processes (RS-45001)
  • ERDF through COMPETE - Programa Operacional Competitividade e Internacionalizacao (POCI) [POCI-01-0145-FEDER-006984]
  • FCT - Fundacao para a Ciencia e a Tecnologia [SFRH/BD/95411/2013]
  • Ministry of Education, Sports, and Youth of the Czech Republic [COST LD14090]
  • COST Action [CM1206]
Note:
  • Peer-reviewed article: https://vinar.vin.bg.ac.rs/handle/123456789/9881
Related info:
  • Referenced by
    https://vinar.vin.bg.ac.rs/handle/123456789/9881

DOI: 10.1002/celc.201701369

ISSN: 2196-0216

WoS: 000429413700007

Scopus: 2-s2.0-85041637185
[ Google Scholar ]
17
16
URI
https://vinar.vin.bg.ac.rs/handle/123456789/7672
Collections
  • Radovi istraživača
Institution/Community
Vinča
TY  - JOUR
AU  - Zdolšek, Nikola
AU  - Dimitrijević, Aleksandra
AU  - Bendova, Magdalena
AU  - Krstić, Jugoslav B.
AU  - Rocha, Raquel P.
AU  - Figueiredo, Jose L.
AU  - Bajuk-Bogdanović, Danica V.
AU  - Trtić-Petrović, Tatjana M.
AU  - Šljukić, Biljana
PY  - 2018
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/7672
AB  - Carbon materials, prepared by using different methods with ionicliquids, are compared as electrocatalysts for the oxygen reductionreaction (ORR). Materials were synthesized through the hydrothermalcarbonization of glucose and by using the same method in the presence of1-butyl-3-methylimidazolium methanesulfonate {[}bmim]{[}MeSO3] as anadditive. Another two carbon-based materials were prepared by usingionic-liquid-based methods: ionothermal carbonization of glucose using{[}bmim]{[}MeSO3] as a recyclable medium for the carbonization reactionand by direct carbonization of the ionic liquid in a one-step methodusing {[}bmim]{[}MeSO3] as the precursor for N- and S-doped porouscarbon (Carb-IL). Characterization results showed the possibility ofmorphology and porosity control by using {[}bmim]{[}MeSO3]. Allmaterials were subsequently tested for the ORR in alkaline media.Carb-IL showed enhanced and stable electrocatalytic ORR activity, evenin the presence of methanol, ethanol, and borohydride, opening thepossibility for its application in fuel cells.
T2  - ChemElectroChem
T1  - Electrocatalytic Activity of Ionic-Liquid-Derived Porous Carbon Materials for the Oxygen Reduction Reaction
VL  - 5
IS  - 7
SP  - 1037
EP  - 1046
DO  - 10.1002/celc.201701369
ER  - 
@article{
author = "Zdolšek, Nikola and Dimitrijević, Aleksandra and Bendova, Magdalena and Krstić, Jugoslav B. and Rocha, Raquel P. and Figueiredo, Jose L. and Bajuk-Bogdanović, Danica V. and Trtić-Petrović, Tatjana M. and Šljukić, Biljana",
year = "2018",
abstract = "Carbon materials, prepared by using different methods with ionicliquids, are compared as electrocatalysts for the oxygen reductionreaction (ORR). Materials were synthesized through the hydrothermalcarbonization of glucose and by using the same method in the presence of1-butyl-3-methylimidazolium methanesulfonate {[}bmim]{[}MeSO3] as anadditive. Another two carbon-based materials were prepared by usingionic-liquid-based methods: ionothermal carbonization of glucose using{[}bmim]{[}MeSO3] as a recyclable medium for the carbonization reactionand by direct carbonization of the ionic liquid in a one-step methodusing {[}bmim]{[}MeSO3] as the precursor for N- and S-doped porouscarbon (Carb-IL). Characterization results showed the possibility ofmorphology and porosity control by using {[}bmim]{[}MeSO3]. Allmaterials were subsequently tested for the ORR in alkaline media.Carb-IL showed enhanced and stable electrocatalytic ORR activity, evenin the presence of methanol, ethanol, and borohydride, opening thepossibility for its application in fuel cells.",
journal = "ChemElectroChem",
title = "Electrocatalytic Activity of Ionic-Liquid-Derived Porous Carbon Materials for the Oxygen Reduction Reaction",
volume = "5",
number = "7",
pages = "1037-1046",
doi = "10.1002/celc.201701369"
}
Zdolšek, N., Dimitrijević, A., Bendova, M., Krstić, J. B., Rocha, R. P., Figueiredo, J. L., Bajuk-Bogdanović, D. V., Trtić-Petrović, T. M.,& Šljukić, B.. (2018). Electrocatalytic Activity of Ionic-Liquid-Derived Porous Carbon Materials for the Oxygen Reduction Reaction. in ChemElectroChem, 5(7), 1037-1046.
https://doi.org/10.1002/celc.201701369
Zdolšek N, Dimitrijević A, Bendova M, Krstić JB, Rocha RP, Figueiredo JL, Bajuk-Bogdanović DV, Trtić-Petrović TM, Šljukić B. Electrocatalytic Activity of Ionic-Liquid-Derived Porous Carbon Materials for the Oxygen Reduction Reaction. in ChemElectroChem. 2018;5(7):1037-1046.
doi:10.1002/celc.201701369 .
Zdolšek, Nikola, Dimitrijević, Aleksandra, Bendova, Magdalena, Krstić, Jugoslav B., Rocha, Raquel P., Figueiredo, Jose L., Bajuk-Bogdanović, Danica V., Trtić-Petrović, Tatjana M., Šljukić, Biljana, "Electrocatalytic Activity of Ionic-Liquid-Derived Porous Carbon Materials for the Oxygen Reduction Reaction" in ChemElectroChem, 5, no. 7 (2018):1037-1046,
https://doi.org/10.1002/celc.201701369 . .

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