Kusigerski, Vladan

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Authority KeyName Variants
orcid::0000-0003-0880-6722
  • Kusigerski, Vladan (71)
Projects
Magnetic and radionuclide labeled nanostructured materials for medical applications Synthesis, processing and characterization of nanostructured materials for application in the field of energy, mechanical engineering, environmental protection and biomedicine
Strukturne i magnetne osobine nanočestičnih i polikristalnih oksida retkih zemalja i 3d metala. Modifikacija, sinteza i analiza nanostrukturnih materijala jonskim snopovima, gama zračenjem i vakuumskim deponovanjem
Strengthening of the MagBioVin Research and Innovation Team for Development of Novel Approaches for Tumour Therapy based on Nanostructured Materials Molecular designing of nanoparticles with controlled morphological and physicochemical characteristics and functional materials based on them
Serbian Ministry of Science and Environmental Protection [141027] Bilateral Serbia-Slovenia projects (projects No. 451-03-38/2016-09/26 and 06-00-118/2018-09/32/02)
COST Action TD1402-RADIOMAG ERANETs 2021A, Action: ΕRANET RUS PLUS [project “Rational design of novel magnetic nanocarriers for targeted vascular therapies” MIS 5161147]
ERDF EU [VEGA02/0132/16, ITMS26220120047, SKSRB-2013-0050] HFRI and GSRT [GA. no. 14650]
Effects of laser radiation and plasma on novel materials in their synthesis, modification, and analysis Synthesis and characterization of novel functional polymers and polymeric nanocomposites
Advanced technologies for monitoring and environmental protection from chemical pollutants and radiation burden Nanostructured multifunctional materials and nanocomposites
MagBioVin Project Ministry of Education and Science of the Russian Federation [3.9002.2017/6.7]
Ministry of Education,Science, and Technological Development of the Republic of Serbia Ministry of Science [141027]
Ministry of Science and Environmental Protection of Serbia [141027] Ministry of Science, Technologies and Development of the Republic of Serbia ”Physical Properties of Bulk and Nanoparticled Rare Earths and Transition Metal Based Magnetic Materials” [Grant No.2022-OI]
RFBR [17-32-50202\17] Russian Academic Excellence Project at the Immanuel Kant Baltic Federal University
Serbian Ministry of Science [141027] Serbian Ministry of Science and Ecology
Serbian Ministry of Science and Ecology and Slovenian Ministry of Science have financially supported this work through joint project "Synthesis and physical properties of nanosize and polycrystalline magnetic materials" Serbian Ministry of Sciences [Project 01E15]
Serbian-Slovak bilateral project [SK-SRB-00207], Serbian-Slovak national projects [P-141027, VEGA 2/0057/10] Slovak Scientific Grant Agency [SK-SRB-0054-11, VEGA0057]

Author's Bibliography

Iron oxide nanoflowers encapsulated in thermosensitive fluorescent liposomes for hyperthermia treatment of lung adenocarcinoma

Theodosiou, Maria; Sakellis, Elias; Boukos, Nikos; Kusigerski, Vladan; Kalska-Szostko, Beata; Efthimiadou, Eleni

(2022)

TY  - JOUR
AU  - Theodosiou, Maria
AU  - Sakellis, Elias
AU  - Boukos, Nikos
AU  - Kusigerski, Vladan
AU  - Kalska-Szostko, Beata
AU  - Efthimiadou, Eleni
PY  - 2022
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/10346
AB  - Magnetic hyperthermia (MHT) is in the spotlight of nanomedical research for the treatment of cancer employing magnetic iron oxide nanoparticles and their intrinsic capability for heat dissipation under an alternating magnetic field (AMF). Herein we focus on the synthesis of iron oxide nanoflowers (Nfs) of different sizes (15 and 35 nm) and coatings (bare, citrate, and Rhodamine B) while comparing their physicochemical and magnetothermal properties. We encapsulated colloidally stable citrate coated Nfs, of both sizes, in thermosensitive liposomes via extrusion, and RhB was loaded in the lipid bilayer. All formulations proved hemocompatible and cytocompatible. We found that 35 nm Nfs, at lower concentrations than 15 nm Nfs, served better as nanoheaters for magnetic hyperthermia applications. In vitro, magnetic hyperthermia results showed promising therapeutic and imaging potential for RhB loaded magnetoliposomes containing 35 nm Nfs against LLC and CULA cell lines of lung adenocarcinoma.
T2  - Scientific Reports
T1  - Iron oxide nanoflowers encapsulated in thermosensitive fluorescent liposomes for hyperthermia treatment of lung adenocarcinoma
VL  - 12
IS  - 1
SP  - 8697
DO  - 10.1038/s41598-022-12687-3
ER  - 
@article{
author = "Theodosiou, Maria and Sakellis, Elias and Boukos, Nikos and Kusigerski, Vladan and Kalska-Szostko, Beata and Efthimiadou, Eleni",
year = "2022",
abstract = "Magnetic hyperthermia (MHT) is in the spotlight of nanomedical research for the treatment of cancer employing magnetic iron oxide nanoparticles and their intrinsic capability for heat dissipation under an alternating magnetic field (AMF). Herein we focus on the synthesis of iron oxide nanoflowers (Nfs) of different sizes (15 and 35 nm) and coatings (bare, citrate, and Rhodamine B) while comparing their physicochemical and magnetothermal properties. We encapsulated colloidally stable citrate coated Nfs, of both sizes, in thermosensitive liposomes via extrusion, and RhB was loaded in the lipid bilayer. All formulations proved hemocompatible and cytocompatible. We found that 35 nm Nfs, at lower concentrations than 15 nm Nfs, served better as nanoheaters for magnetic hyperthermia applications. In vitro, magnetic hyperthermia results showed promising therapeutic and imaging potential for RhB loaded magnetoliposomes containing 35 nm Nfs against LLC and CULA cell lines of lung adenocarcinoma.",
journal = "Scientific Reports",
title = "Iron oxide nanoflowers encapsulated in thermosensitive fluorescent liposomes for hyperthermia treatment of lung adenocarcinoma",
volume = "12",
number = "1",
pages = "8697",
doi = "10.1038/s41598-022-12687-3"
}
Theodosiou, M., Sakellis, E., Boukos, N., Kusigerski, V., Kalska-Szostko, B.,& Efthimiadou, E.. (2022). Iron oxide nanoflowers encapsulated in thermosensitive fluorescent liposomes for hyperthermia treatment of lung adenocarcinoma. in Scientific Reports, 12(1), 8697.
https://doi.org/10.1038/s41598-022-12687-3
Theodosiou M, Sakellis E, Boukos N, Kusigerski V, Kalska-Szostko B, Efthimiadou E. Iron oxide nanoflowers encapsulated in thermosensitive fluorescent liposomes for hyperthermia treatment of lung adenocarcinoma. in Scientific Reports. 2022;12(1):8697.
doi:10.1038/s41598-022-12687-3 .
Theodosiou, Maria, Sakellis, Elias, Boukos, Nikos, Kusigerski, Vladan, Kalska-Szostko, Beata, Efthimiadou, Eleni, "Iron oxide nanoflowers encapsulated in thermosensitive fluorescent liposomes for hyperthermia treatment of lung adenocarcinoma" in Scientific Reports, 12, no. 1 (2022):8697,
https://doi.org/10.1038/s41598-022-12687-3 . .
2
17
1
14

Unvailing the spin–phonon coupling in nanocrystalline BiFeO3 by resonant two-phonon Raman active modes

Stojadinović, Bojan; Đokić, Dejan M.; Paunović, Novica; Živković, Ivica; Ćirić, Luka; Kusigerski, Vladan; Dohčević-Mitrović, Zorana

(2021)

TY  - JOUR
AU  - Stojadinović, Bojan
AU  - Đokić, Dejan M.
AU  - Paunović, Novica
AU  - Živković, Ivica
AU  - Ćirić, Luka
AU  - Kusigerski, Vladan
AU  - Dohčević-Mitrović, Zorana
PY  - 2021
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/9956
AB  - We report on temperature dependence of two-phonon Raman spectra in BiFeO3 nanocrystals, above and below the Néel temperature TN using a resonant laser excitation line (λ=532 nm). Two-phonon modes exhibited anomalous frequency hardening and deviation from the anharmonic decay below TN. Such behavior strongly supported the existence of spin-two-phonon interaction, because these modes are known to be very sensitive to the antiferromagnetic ordering. Within the mean-field theory for the nearest-neighbor interaction, the linear relationship between spin–spin correlation function and observed two-phonon frequency shift below TN was obtained. This approach enabled to quantify the spin–phonon interaction by spin–phonon coupling strength for both two-phonon modes and justified the application of mean-field approach. Magnetic measurements revealed the coexistence of antiferromagnetic and weak ferromagnetic phases below TN, which were found non competitive, additionally supporting the mean-field approach from which we deduced that the two-phonon modes in BiFeO3 are correlated with antiferromagnetic ordering below TN.
T2  - Materials Science and Engineering: B
T1  - Unvailing the spin–phonon coupling in nanocrystalline BiFeO3 by resonant two-phonon Raman active modes
VL  - 274
SP  - 115444
DO  - 10.1016/j.mseb.2021.115444
ER  - 
@article{
author = "Stojadinović, Bojan and Đokić, Dejan M. and Paunović, Novica and Živković, Ivica and Ćirić, Luka and Kusigerski, Vladan and Dohčević-Mitrović, Zorana",
year = "2021",
abstract = "We report on temperature dependence of two-phonon Raman spectra in BiFeO3 nanocrystals, above and below the Néel temperature TN using a resonant laser excitation line (λ=532 nm). Two-phonon modes exhibited anomalous frequency hardening and deviation from the anharmonic decay below TN. Such behavior strongly supported the existence of spin-two-phonon interaction, because these modes are known to be very sensitive to the antiferromagnetic ordering. Within the mean-field theory for the nearest-neighbor interaction, the linear relationship between spin–spin correlation function and observed two-phonon frequency shift below TN was obtained. This approach enabled to quantify the spin–phonon interaction by spin–phonon coupling strength for both two-phonon modes and justified the application of mean-field approach. Magnetic measurements revealed the coexistence of antiferromagnetic and weak ferromagnetic phases below TN, which were found non competitive, additionally supporting the mean-field approach from which we deduced that the two-phonon modes in BiFeO3 are correlated with antiferromagnetic ordering below TN.",
journal = "Materials Science and Engineering: B",
title = "Unvailing the spin–phonon coupling in nanocrystalline BiFeO3 by resonant two-phonon Raman active modes",
volume = "274",
pages = "115444",
doi = "10.1016/j.mseb.2021.115444"
}
Stojadinović, B., Đokić, D. M., Paunović, N., Živković, I., Ćirić, L., Kusigerski, V.,& Dohčević-Mitrović, Z.. (2021). Unvailing the spin–phonon coupling in nanocrystalline BiFeO3 by resonant two-phonon Raman active modes. in Materials Science and Engineering: B, 274, 115444.
https://doi.org/10.1016/j.mseb.2021.115444
Stojadinović B, Đokić DM, Paunović N, Živković I, Ćirić L, Kusigerski V, Dohčević-Mitrović Z. Unvailing the spin–phonon coupling in nanocrystalline BiFeO3 by resonant two-phonon Raman active modes. in Materials Science and Engineering: B. 2021;274:115444.
doi:10.1016/j.mseb.2021.115444 .
Stojadinović, Bojan, Đokić, Dejan M., Paunović, Novica, Živković, Ivica, Ćirić, Luka, Kusigerski, Vladan, Dohčević-Mitrović, Zorana, "Unvailing the spin–phonon coupling in nanocrystalline BiFeO3 by resonant two-phonon Raman active modes" in Materials Science and Engineering: B, 274 (2021):115444,
https://doi.org/10.1016/j.mseb.2021.115444 . .
1
1

Search for high temperature memory effects in magnetic nanoparticles

Perović, Marija M.; Bošković, Marko; Kusigerski, Vladan; Jagličić, Zvonko; Blanuša, Jovan; Spasojević, Vojislav; Pizurova, Nadežda; Schneeweiss, Oldřich B.

(2021)

TY  - JOUR
AU  - Perović, Marija M.
AU  - Bošković, Marko
AU  - Kusigerski, Vladan
AU  - Jagličić, Zvonko
AU  - Blanuša, Jovan
AU  - Spasojević, Vojislav
AU  - Pizurova, Nadežda
AU  - Schneeweiss, Oldřich B.
PY  - 2021
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/9674
AB  - Nanoparticle materials have become a promising candidate for a new kind of storage media based on thermally induced memory effects due to the possibility to tailor their magnetic properties and behaviour. In this study, we have investigated whether the magnetic memory effects could appear at high, industry accessible temperatures including the possibility of thermal data inscription. Investigated iron oxide nanoparticles were synthesized by poliol method, which has been modified in order to allow control of particle agglomeration and consequently magnetic properties. Structure, morphology and the degree of nanoparticle agglomeration were studied by X-Ray diffraction, Transmission Electron Microscopy and Dynamic Light Scattering techniques, while magnetic properties as well as memory effects were measured on a commercial SQUID-based magnetometer. Results of the study confirmed that in super spin glass magnetite nanoparticles, magnetic memory effects can be observed up to 200 K which represents much higher temperatures in comparison to those achieved in spin glasses and other glassy materials. Procedures of writing and reading (inscribing and retrieving) of digital information in such a material were demonstrated and discussed in details.
T2  - Journal of Alloys and Compounds
T1  - Search for high temperature memory effects in magnetic nanoparticles
VL  - 855
SP  - 157523
DO  - 10.1016/j.jallcom.2020.157523
ER  - 
@article{
author = "Perović, Marija M. and Bošković, Marko and Kusigerski, Vladan and Jagličić, Zvonko and Blanuša, Jovan and Spasojević, Vojislav and Pizurova, Nadežda and Schneeweiss, Oldřich B.",
year = "2021",
abstract = "Nanoparticle materials have become a promising candidate for a new kind of storage media based on thermally induced memory effects due to the possibility to tailor their magnetic properties and behaviour. In this study, we have investigated whether the magnetic memory effects could appear at high, industry accessible temperatures including the possibility of thermal data inscription. Investigated iron oxide nanoparticles were synthesized by poliol method, which has been modified in order to allow control of particle agglomeration and consequently magnetic properties. Structure, morphology and the degree of nanoparticle agglomeration were studied by X-Ray diffraction, Transmission Electron Microscopy and Dynamic Light Scattering techniques, while magnetic properties as well as memory effects were measured on a commercial SQUID-based magnetometer. Results of the study confirmed that in super spin glass magnetite nanoparticles, magnetic memory effects can be observed up to 200 K which represents much higher temperatures in comparison to those achieved in spin glasses and other glassy materials. Procedures of writing and reading (inscribing and retrieving) of digital information in such a material were demonstrated and discussed in details.",
journal = "Journal of Alloys and Compounds",
title = "Search for high temperature memory effects in magnetic nanoparticles",
volume = "855",
pages = "157523",
doi = "10.1016/j.jallcom.2020.157523"
}
Perović, M. M., Bošković, M., Kusigerski, V., Jagličić, Z., Blanuša, J., Spasojević, V., Pizurova, N.,& Schneeweiss, O. B.. (2021). Search for high temperature memory effects in magnetic nanoparticles. in Journal of Alloys and Compounds, 855, 157523.
https://doi.org/10.1016/j.jallcom.2020.157523
Perović MM, Bošković M, Kusigerski V, Jagličić Z, Blanuša J, Spasojević V, Pizurova N, Schneeweiss OB. Search for high temperature memory effects in magnetic nanoparticles. in Journal of Alloys and Compounds. 2021;855:157523.
doi:10.1016/j.jallcom.2020.157523 .
Perović, Marija M., Bošković, Marko, Kusigerski, Vladan, Jagličić, Zvonko, Blanuša, Jovan, Spasojević, Vojislav, Pizurova, Nadežda, Schneeweiss, Oldřich B., "Search for high temperature memory effects in magnetic nanoparticles" in Journal of Alloys and Compounds, 855 (2021):157523,
https://doi.org/10.1016/j.jallcom.2020.157523 . .
2
2

Influence of Ni2+/Co2+ ratio in electrolyte on morphology, structure and magnetic properties of electrolytically produced Ni−Co alloy powders

Maksimović, Vesna; Kusigerski, Vladan; Stoiljković, Milovan; Maletaškić, Jelena; Nikolić, Nebojša D.

(2020)

TY  - JOUR
AU  - Maksimović, Vesna
AU  - Kusigerski, Vladan
AU  - Stoiljković, Milovan
AU  - Maletaškić, Jelena
AU  - Nikolić, Nebojša D.
PY  - 2020
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/8950
AB  - Nickel−cobalt (Ni−Co) alloy powders were produced galvanostatically by using sulphate electrolytes withvarious ratios of Ni2+/Co2+ (mole ratios). The morphology, phase structure, chemical composition and magneticproperties were examined by scanning electron microscope (SEM), X-ray diffractometer (XRD), atomic emissionspectrometer (AES), and SQUID-based magnetometer, respectively. Morphology of the particles changed fromcauliflower-like and dendritic to coral-like and spongy-like ones with increasing Ni2+/Co2+ ratio from 0.25 to 4.0. XRDanalysis of the Ni−Co powders revealed that the decrease of Ni2+/Co2+ ratios (the increase of Co content) caused achange of structure from face centered cubic (FCC) obtained for the ratios of 4.0, 1.5 and 0.67 to a mixture of FCC andhexagonal closed-packed (HCP) phases for the ratio of 0.25. The increasing content of nickel led to change ofmechanism of electrolysis from irregular (up to ~40 wt.% Ni in the electrolytes) to close to equilibrium (between~40 and 60 wt.% Ni in the electrolytes) and anomalous co-deposition (over 60 wt.% Ni in the electrolytes) type. All ofthe obtained Ni−Co alloy samples behaved as soft magnetic materials while their magnetic parameters showedimmediate composition dependence since both coercivity and saturation magnetization almost linearly increased withincrease of the Co content.
T2  - Transactions of Nonferrous Metals Society of China
T1  - Influence of Ni2+/Co2+ ratio in electrolyte on morphology, structure and magnetic properties of electrolytically produced Ni−Co alloy powders
VL  - 30
IS  - 4
SP  - 1046
EP  - 1057
DO  - 10.1016/S1003-6326(20)65276-1
ER  - 
@article{
author = "Maksimović, Vesna and Kusigerski, Vladan and Stoiljković, Milovan and Maletaškić, Jelena and Nikolić, Nebojša D.",
year = "2020",
abstract = "Nickel−cobalt (Ni−Co) alloy powders were produced galvanostatically by using sulphate electrolytes withvarious ratios of Ni2+/Co2+ (mole ratios). The morphology, phase structure, chemical composition and magneticproperties were examined by scanning electron microscope (SEM), X-ray diffractometer (XRD), atomic emissionspectrometer (AES), and SQUID-based magnetometer, respectively. Morphology of the particles changed fromcauliflower-like and dendritic to coral-like and spongy-like ones with increasing Ni2+/Co2+ ratio from 0.25 to 4.0. XRDanalysis of the Ni−Co powders revealed that the decrease of Ni2+/Co2+ ratios (the increase of Co content) caused achange of structure from face centered cubic (FCC) obtained for the ratios of 4.0, 1.5 and 0.67 to a mixture of FCC andhexagonal closed-packed (HCP) phases for the ratio of 0.25. The increasing content of nickel led to change ofmechanism of electrolysis from irregular (up to ~40 wt.% Ni in the electrolytes) to close to equilibrium (between~40 and 60 wt.% Ni in the electrolytes) and anomalous co-deposition (over 60 wt.% Ni in the electrolytes) type. All ofthe obtained Ni−Co alloy samples behaved as soft magnetic materials while their magnetic parameters showedimmediate composition dependence since both coercivity and saturation magnetization almost linearly increased withincrease of the Co content.",
journal = "Transactions of Nonferrous Metals Society of China",
title = "Influence of Ni2+/Co2+ ratio in electrolyte on morphology, structure and magnetic properties of electrolytically produced Ni−Co alloy powders",
volume = "30",
number = "4",
pages = "1046-1057",
doi = "10.1016/S1003-6326(20)65276-1"
}
Maksimović, V., Kusigerski, V., Stoiljković, M., Maletaškić, J.,& Nikolić, N. D.. (2020). Influence of Ni2+/Co2+ ratio in electrolyte on morphology, structure and magnetic properties of electrolytically produced Ni−Co alloy powders. in Transactions of Nonferrous Metals Society of China, 30(4), 1046-1057.
https://doi.org/10.1016/S1003-6326(20)65276-1
Maksimović V, Kusigerski V, Stoiljković M, Maletaškić J, Nikolić ND. Influence of Ni2+/Co2+ ratio in electrolyte on morphology, structure and magnetic properties of electrolytically produced Ni−Co alloy powders. in Transactions of Nonferrous Metals Society of China. 2020;30(4):1046-1057.
doi:10.1016/S1003-6326(20)65276-1 .
Maksimović, Vesna, Kusigerski, Vladan, Stoiljković, Milovan, Maletaškić, Jelena, Nikolić, Nebojša D., "Influence of Ni2+/Co2+ ratio in electrolyte on morphology, structure and magnetic properties of electrolytically produced Ni−Co alloy powders" in Transactions of Nonferrous Metals Society of China, 30, no. 4 (2020):1046-1057,
https://doi.org/10.1016/S1003-6326(20)65276-1 . .
3
3

A study of defect structures in Fe-alloyed ZnO: Morphology, magnetism, and hyperfine interactions

Ivanovski, Valentin N.; Belošević-Čavor, Jelena; Rajić, Vladimir; Umićević, Ana; Marković, Smilja; Kusigerski, Vladan; Mitrić, Miodrag; Koteski, Vasil J.

(2019)

TY  - JOUR
AU  - Ivanovski, Valentin N.
AU  - Belošević-Čavor, Jelena
AU  - Rajić, Vladimir
AU  - Umićević, Ana
AU  - Marković, Smilja
AU  - Kusigerski, Vladan
AU  - Mitrić, Miodrag
AU  - Koteski, Vasil J.
PY  - 2019
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/8515
AB  - In order to study the effect of Fe cation substitution on the local structure, defect formation, and hyperfine interactions in ZnO, Mössbauer spectroscopy measurements of the microwave processed Zn 1 - x Fe x O (x = 0.05, 0.10, 0.15, and 0.20) nanoparticles, together with ab initio calculations, were performed. Complementary information on the distribution of particle size and morphology, as well as magnetic properties, were obtained by X-ray diffraction, transmission electron microscopy, and squid-magnetometry. The selected model for analyzing the Mössbauer spectra of our samples is a distribution of quadrupole splittings. The fitting model with two Lorentz doublets was rejected due to its failure to include larger doublets. The Fe 3 + ions do not yield magnetic ordering in the samples at room temperature. The results from first-principles calculations confirm that the major component of the Mössbauer spectra corresponds to the Fe-alloyed ZnO with Zn vacancy in the next nearest neighbor environment. The magnetic measurements are consistent with the description of the distribution of iron ions over the randomly formed clusters in the ZnO host lattice. While at room temperature all the samples are paramagnetic, magnetic interactions cause a transition into a cluster spin-glass state at low temperatures. © 2019 Author(s).
T2  - Journal of Applied Physics
T1  - A study of defect structures in Fe-alloyed ZnO: Morphology, magnetism, and hyperfine interactions
VL  - 126
IS  - 12
SP  - 125703
DO  - 10.1063/1.5095837
ER  - 
@article{
author = "Ivanovski, Valentin N. and Belošević-Čavor, Jelena and Rajić, Vladimir and Umićević, Ana and Marković, Smilja and Kusigerski, Vladan and Mitrić, Miodrag and Koteski, Vasil J.",
year = "2019",
abstract = "In order to study the effect of Fe cation substitution on the local structure, defect formation, and hyperfine interactions in ZnO, Mössbauer spectroscopy measurements of the microwave processed Zn 1 - x Fe x O (x = 0.05, 0.10, 0.15, and 0.20) nanoparticles, together with ab initio calculations, were performed. Complementary information on the distribution of particle size and morphology, as well as magnetic properties, were obtained by X-ray diffraction, transmission electron microscopy, and squid-magnetometry. The selected model for analyzing the Mössbauer spectra of our samples is a distribution of quadrupole splittings. The fitting model with two Lorentz doublets was rejected due to its failure to include larger doublets. The Fe 3 + ions do not yield magnetic ordering in the samples at room temperature. The results from first-principles calculations confirm that the major component of the Mössbauer spectra corresponds to the Fe-alloyed ZnO with Zn vacancy in the next nearest neighbor environment. The magnetic measurements are consistent with the description of the distribution of iron ions over the randomly formed clusters in the ZnO host lattice. While at room temperature all the samples are paramagnetic, magnetic interactions cause a transition into a cluster spin-glass state at low temperatures. © 2019 Author(s).",
journal = "Journal of Applied Physics",
title = "A study of defect structures in Fe-alloyed ZnO: Morphology, magnetism, and hyperfine interactions",
volume = "126",
number = "12",
pages = "125703",
doi = "10.1063/1.5095837"
}
Ivanovski, V. N., Belošević-Čavor, J., Rajić, V., Umićević, A., Marković, S., Kusigerski, V., Mitrić, M.,& Koteski, V. J.. (2019). A study of defect structures in Fe-alloyed ZnO: Morphology, magnetism, and hyperfine interactions. in Journal of Applied Physics, 126(12), 125703.
https://doi.org/10.1063/1.5095837
Ivanovski VN, Belošević-Čavor J, Rajić V, Umićević A, Marković S, Kusigerski V, Mitrić M, Koteski VJ. A study of defect structures in Fe-alloyed ZnO: Morphology, magnetism, and hyperfine interactions. in Journal of Applied Physics. 2019;126(12):125703.
doi:10.1063/1.5095837 .
Ivanovski, Valentin N., Belošević-Čavor, Jelena, Rajić, Vladimir, Umićević, Ana, Marković, Smilja, Kusigerski, Vladan, Mitrić, Miodrag, Koteski, Vasil J., "A study of defect structures in Fe-alloyed ZnO: Morphology, magnetism, and hyperfine interactions" in Journal of Applied Physics, 126, no. 12 (2019):125703,
https://doi.org/10.1063/1.5095837 . .
5
5
6

Effects of fluorination on the structure, magnetic and electrochemical properties of the P2-type NaxCoO2 powder

Jugović, Dragana; Milović, Miloš; Popović, Maja; Kusigerski, Vladan; Škapin, Srečo Davor; Rakočević, Zlatko Lj.; Mitrić, Miodrag

(2019)

TY  - JOUR
AU  - Jugović, Dragana
AU  - Milović, Miloš
AU  - Popović, Maja
AU  - Kusigerski, Vladan
AU  - Škapin, Srečo Davor
AU  - Rakočević, Zlatko Lj.
AU  - Mitrić, Miodrag
PY  - 2019
UR  - https://linkinghub.elsevier.com/retrieve/pii/S0925838818336375
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/7897
AB  - The main goal of this research has been to investigate for the first time the effects of fluorination on the crystal structure, magnetic, and electrochemical properties of the P2-type NaxCoO2 powder. Sodium cobalt oxide with a P2-type structure is synthesized by a modified solid-state reaction consisting of alternating processes of rapid heating up to 750 °C and rapid cooling to the room temperature. The obtained powder is fluorinated using a gas-solid reaction with NH4HF2 as fluorinating agent. Fluorination causes a decrease of sodium content in the parent phase with the concurrent formation of the minor phases of Na2CO3 and NaF. The structure of NaxCoO2 in both powders is refined in P63/mmc space group. The results of the Rietveld refinement combined with the findings from the XPS measurements confirm the Na0.76CoO2 and Na0.44CoO1.96F0.04 stoichiometries for the pristine and fluorinated powders, respectively, which indicates that 4 at.% of fluorine ions per formula unit are incorporated in the structure. Preliminary electrochemical investigations have revealed an improved charge/discharge performance. The influence of fluorination on morphology and magnetic properties has also been examined. © 2018 Elsevier B.V.
T2  - Journal of Alloys and Compounds
T1  - Effects of fluorination on the structure, magnetic and electrochemical properties of the P2-type NaxCoO2 powder
VL  - 774
SP  - 30
EP  - 37
DO  - 10.1016/j.jallcom.2018.09.372
ER  - 
@article{
author = "Jugović, Dragana and Milović, Miloš and Popović, Maja and Kusigerski, Vladan and Škapin, Srečo Davor and Rakočević, Zlatko Lj. and Mitrić, Miodrag",
year = "2019",
abstract = "The main goal of this research has been to investigate for the first time the effects of fluorination on the crystal structure, magnetic, and electrochemical properties of the P2-type NaxCoO2 powder. Sodium cobalt oxide with a P2-type structure is synthesized by a modified solid-state reaction consisting of alternating processes of rapid heating up to 750 °C and rapid cooling to the room temperature. The obtained powder is fluorinated using a gas-solid reaction with NH4HF2 as fluorinating agent. Fluorination causes a decrease of sodium content in the parent phase with the concurrent formation of the minor phases of Na2CO3 and NaF. The structure of NaxCoO2 in both powders is refined in P63/mmc space group. The results of the Rietveld refinement combined with the findings from the XPS measurements confirm the Na0.76CoO2 and Na0.44CoO1.96F0.04 stoichiometries for the pristine and fluorinated powders, respectively, which indicates that 4 at.% of fluorine ions per formula unit are incorporated in the structure. Preliminary electrochemical investigations have revealed an improved charge/discharge performance. The influence of fluorination on morphology and magnetic properties has also been examined. © 2018 Elsevier B.V.",
journal = "Journal of Alloys and Compounds",
title = "Effects of fluorination on the structure, magnetic and electrochemical properties of the P2-type NaxCoO2 powder",
volume = "774",
pages = "30-37",
doi = "10.1016/j.jallcom.2018.09.372"
}
Jugović, D., Milović, M., Popović, M., Kusigerski, V., Škapin, S. D., Rakočević, Z. Lj.,& Mitrić, M.. (2019). Effects of fluorination on the structure, magnetic and electrochemical properties of the P2-type NaxCoO2 powder. in Journal of Alloys and Compounds, 774, 30-37.
https://doi.org/10.1016/j.jallcom.2018.09.372
Jugović D, Milović M, Popović M, Kusigerski V, Škapin SD, Rakočević ZL, Mitrić M. Effects of fluorination on the structure, magnetic and electrochemical properties of the P2-type NaxCoO2 powder. in Journal of Alloys and Compounds. 2019;774:30-37.
doi:10.1016/j.jallcom.2018.09.372 .
Jugović, Dragana, Milović, Miloš, Popović, Maja, Kusigerski, Vladan, Škapin, Srečo Davor, Rakočević, Zlatko Lj., Mitrić, Miodrag, "Effects of fluorination on the structure, magnetic and electrochemical properties of the P2-type NaxCoO2 powder" in Journal of Alloys and Compounds, 774 (2019):30-37,
https://doi.org/10.1016/j.jallcom.2018.09.372 . .
15
10
13

Magnetic properties and heating efficacy of magnesium doped magnetite nanoparticles obtained by co-precipitation method

Kusigerski, Vladan; Illés, Erzsébet; Blanuša, Jovan; Gyergyek, Sašo; Bošković, Marko; Perović, Marija M.; Spasojević, Vojislav

(2019)

TY  - JOUR
AU  - Kusigerski, Vladan
AU  - Illés, Erzsébet
AU  - Blanuša, Jovan
AU  - Gyergyek, Sašo
AU  - Bošković, Marko
AU  - Perović, Marija M.
AU  - Spasojević, Vojislav
PY  - 2019
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/7983
AB  - Ferrofluids based on magnesium substituted magnetite nanoparticles MgxFe3−xO4 (x = 0.1; 0.2; 0.4) were synthesised by a chemical co-precipitation method. Their physical properties have been compared with those of the magnetite based ferrofluid obtained by the same synthesis route. Both XRD and TEM studies showed particle size decrease with the increased Mg content while DLS experiments pointed to the more prominent aggregation of Mg-containing nanoparticles. Magnetic properties investigation conducted on the powder (i.e. dried) specimens showed decrease of magnetization values with increased Mg content except for the lowest concentration of x = 0.1 where substantial saturation magnetization rise of about 40% was recorded at room temperature. Heating abilities of the studied ferrofluids under the applied AC fields (SAR values) also showed decreasing trend with the increased Mg content even for x = 0.1 sample despite its elevated magnetization value. This trend has been understood as a consequence of the changed intrinsic nanoparticle properties such as size and magnetic anisotropy, as well as contribution of a collective behaviour due to an increased nanoparticle aggregation in Mg-doped systems.
T2  - Journal of Magnetism and Magnetic Materials
T1  - Magnetic properties and heating efficacy of magnesium doped magnetite nanoparticles obtained by co-precipitation method
VL  - 475
SP  - 470
EP  - 478
DO  - 10.1016/j.jmmm.2018.11.127
ER  - 
@article{
author = "Kusigerski, Vladan and Illés, Erzsébet and Blanuša, Jovan and Gyergyek, Sašo and Bošković, Marko and Perović, Marija M. and Spasojević, Vojislav",
year = "2019",
abstract = "Ferrofluids based on magnesium substituted magnetite nanoparticles MgxFe3−xO4 (x = 0.1; 0.2; 0.4) were synthesised by a chemical co-precipitation method. Their physical properties have been compared with those of the magnetite based ferrofluid obtained by the same synthesis route. Both XRD and TEM studies showed particle size decrease with the increased Mg content while DLS experiments pointed to the more prominent aggregation of Mg-containing nanoparticles. Magnetic properties investigation conducted on the powder (i.e. dried) specimens showed decrease of magnetization values with increased Mg content except for the lowest concentration of x = 0.1 where substantial saturation magnetization rise of about 40% was recorded at room temperature. Heating abilities of the studied ferrofluids under the applied AC fields (SAR values) also showed decreasing trend with the increased Mg content even for x = 0.1 sample despite its elevated magnetization value. This trend has been understood as a consequence of the changed intrinsic nanoparticle properties such as size and magnetic anisotropy, as well as contribution of a collective behaviour due to an increased nanoparticle aggregation in Mg-doped systems.",
journal = "Journal of Magnetism and Magnetic Materials",
title = "Magnetic properties and heating efficacy of magnesium doped magnetite nanoparticles obtained by co-precipitation method",
volume = "475",
pages = "470-478",
doi = "10.1016/j.jmmm.2018.11.127"
}
Kusigerski, V., Illés, E., Blanuša, J., Gyergyek, S., Bošković, M., Perović, M. M.,& Spasojević, V.. (2019). Magnetic properties and heating efficacy of magnesium doped magnetite nanoparticles obtained by co-precipitation method. in Journal of Magnetism and Magnetic Materials, 475, 470-478.
https://doi.org/10.1016/j.jmmm.2018.11.127
Kusigerski V, Illés E, Blanuša J, Gyergyek S, Bošković M, Perović MM, Spasojević V. Magnetic properties and heating efficacy of magnesium doped magnetite nanoparticles obtained by co-precipitation method. in Journal of Magnetism and Magnetic Materials. 2019;475:470-478.
doi:10.1016/j.jmmm.2018.11.127 .
Kusigerski, Vladan, Illés, Erzsébet, Blanuša, Jovan, Gyergyek, Sašo, Bošković, Marko, Perović, Marija M., Spasojević, Vojislav, "Magnetic properties and heating efficacy of magnesium doped magnetite nanoparticles obtained by co-precipitation method" in Journal of Magnetism and Magnetic Materials, 475 (2019):470-478,
https://doi.org/10.1016/j.jmmm.2018.11.127 . .
45
21
44

Experimental Protocols for Measuring Properties of Nanoparticles Dispersed in Fluids

Omelyanchik, Alexander; Knežević, Nikola; Rodionova, Valeria; Salvador, Maria; Peddis, Davide; Varvaro, Gaspare; Laureti, Sara; Mraković, Ana Đ.; Kusigerski, Vladan; Illes, Erzsebet

(IEEE, 2018)

TY  - CONF
AU  - Omelyanchik, Alexander
AU  - Knežević, Nikola
AU  - Rodionova, Valeria
AU  - Salvador, Maria
AU  - Peddis, Davide
AU  - Varvaro, Gaspare
AU  - Laureti, Sara
AU  - Mraković, Ana Đ.
AU  - Kusigerski, Vladan
AU  - Illes, Erzsebet
PY  - 2018
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/8749
AB  - Investigating magnetic properties of nanoparticles dispersed in a fluid is catching an increasing attention for their wide range of applications; however, a careful magnetic characterization requires low temperatures and vacuum conditions which represent a critical issue for a correct sample handling. In this paper, several experimental protocols to investigate low temperature magnetic properties of magnetic nanoparticles dispersed in fluid are described. In particular, by investigating interparticle interaction by remanence techniques at low temperature, some insight about particle aggregation in fluids has been given. © 2018 IEEE.
PB  - IEEE
C3  - 2018 IEEE 8th International Conference Nanomaterials: Application & Properties (NAP)
T1  - Experimental Protocols for Measuring Properties of Nanoparticles Dispersed in Fluids
SP  - 1
EP  - 5
DO  - 10.1109/NAP.2018.8915059
ER  - 
@conference{
author = "Omelyanchik, Alexander and Knežević, Nikola and Rodionova, Valeria and Salvador, Maria and Peddis, Davide and Varvaro, Gaspare and Laureti, Sara and Mraković, Ana Đ. and Kusigerski, Vladan and Illes, Erzsebet",
year = "2018",
abstract = "Investigating magnetic properties of nanoparticles dispersed in a fluid is catching an increasing attention for their wide range of applications; however, a careful magnetic characterization requires low temperatures and vacuum conditions which represent a critical issue for a correct sample handling. In this paper, several experimental protocols to investigate low temperature magnetic properties of magnetic nanoparticles dispersed in fluid are described. In particular, by investigating interparticle interaction by remanence techniques at low temperature, some insight about particle aggregation in fluids has been given. © 2018 IEEE.",
publisher = "IEEE",
journal = "2018 IEEE 8th International Conference Nanomaterials: Application & Properties (NAP)",
title = "Experimental Protocols for Measuring Properties of Nanoparticles Dispersed in Fluids",
pages = "1-5",
doi = "10.1109/NAP.2018.8915059"
}
Omelyanchik, A., Knežević, N., Rodionova, V., Salvador, M., Peddis, D., Varvaro, G., Laureti, S., Mraković, A. Đ., Kusigerski, V.,& Illes, E.. (2018). Experimental Protocols for Measuring Properties of Nanoparticles Dispersed in Fluids. in 2018 IEEE 8th International Conference Nanomaterials: Application & Properties (NAP)
IEEE., 1-5.
https://doi.org/10.1109/NAP.2018.8915059
Omelyanchik A, Knežević N, Rodionova V, Salvador M, Peddis D, Varvaro G, Laureti S, Mraković AĐ, Kusigerski V, Illes E. Experimental Protocols for Measuring Properties of Nanoparticles Dispersed in Fluids. in 2018 IEEE 8th International Conference Nanomaterials: Application & Properties (NAP). 2018;:1-5.
doi:10.1109/NAP.2018.8915059 .
Omelyanchik, Alexander, Knežević, Nikola, Rodionova, Valeria, Salvador, Maria, Peddis, Davide, Varvaro, Gaspare, Laureti, Sara, Mraković, Ana Đ., Kusigerski, Vladan, Illes, Erzsebet, "Experimental Protocols for Measuring Properties of Nanoparticles Dispersed in Fluids" in 2018 IEEE 8th International Conference Nanomaterials: Application & Properties (NAP) (2018):1-5,
https://doi.org/10.1109/NAP.2018.8915059 . .
2
2

Selective magnetic GMA based potential sorbents for molybdenum and rhenium sorption

Marković, Bojana M.; Vuković, Zorica M.; Spasojević, Vojislav; Kusigerski, Vladan; Pavlović, Vladimir B.; Onjia, Antonije E.; Nastasović, Aleksandra B.

(2017)

TY  - JOUR
AU  - Marković, Bojana M.
AU  - Vuković, Zorica M.
AU  - Spasojević, Vojislav
AU  - Kusigerski, Vladan
AU  - Pavlović, Vladimir B.
AU  - Onjia, Antonije E.
AU  - Nastasović, Aleksandra B.
PY  - 2017
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/1494
AB  - Magnetic macroporous crosslinked copolymer glycidyl methacrylate (GMA) and ethylene glycol dimethacrylate (EGDMA) samples with different magnetite content were prepared by suspension copolymerization and functionalized with diethylene triamine. Samples were characterized by elemental analysis, mercury porosimetry, Fourier transform infrared spectroscopy (FTIR) analysis, scanning electron microscopy with energy-dispersive X-ray spectroscopy, transmission electron microscopy, SQUID magnetometry and X-ray photoelectron spectroscopy (XPS). The selected amino-functionalized sample was tested as a potential sorbent for the Mo(VI) and Re(VII) oxyanions from aqueous solutions. The influence of pH, ionic strength and possible interfering of cations and anions was investigated. Equilibrium data were analyzed with Langmuir, Freundlich and Tempkin adsorption isotherm models. Sorption studies were carried out in a batch competitive experiments, in the pH range 1-8, at 298 K. Obtained results indicate that 92% of Re(VII) and 98% of Mo(VI) were sorbed at pH 2. (C) 2017 Elsevier B. V. All rights reserved.
T2  - Journal of Alloys and Compounds
T1  - Selective magnetic GMA based potential sorbents for molybdenum and rhenium sorption
VL  - 705
SP  - 38
EP  - 50
DO  - 10.1016/j.jallcom.2017.02.108
ER  - 
@article{
author = "Marković, Bojana M. and Vuković, Zorica M. and Spasojević, Vojislav and Kusigerski, Vladan and Pavlović, Vladimir B. and Onjia, Antonije E. and Nastasović, Aleksandra B.",
year = "2017",
abstract = "Magnetic macroporous crosslinked copolymer glycidyl methacrylate (GMA) and ethylene glycol dimethacrylate (EGDMA) samples with different magnetite content were prepared by suspension copolymerization and functionalized with diethylene triamine. Samples were characterized by elemental analysis, mercury porosimetry, Fourier transform infrared spectroscopy (FTIR) analysis, scanning electron microscopy with energy-dispersive X-ray spectroscopy, transmission electron microscopy, SQUID magnetometry and X-ray photoelectron spectroscopy (XPS). The selected amino-functionalized sample was tested as a potential sorbent for the Mo(VI) and Re(VII) oxyanions from aqueous solutions. The influence of pH, ionic strength and possible interfering of cations and anions was investigated. Equilibrium data were analyzed with Langmuir, Freundlich and Tempkin adsorption isotherm models. Sorption studies were carried out in a batch competitive experiments, in the pH range 1-8, at 298 K. Obtained results indicate that 92% of Re(VII) and 98% of Mo(VI) were sorbed at pH 2. (C) 2017 Elsevier B. V. All rights reserved.",
journal = "Journal of Alloys and Compounds",
title = "Selective magnetic GMA based potential sorbents for molybdenum and rhenium sorption",
volume = "705",
pages = "38-50",
doi = "10.1016/j.jallcom.2017.02.108"
}
Marković, B. M., Vuković, Z. M., Spasojević, V., Kusigerski, V., Pavlović, V. B., Onjia, A. E.,& Nastasović, A. B.. (2017). Selective magnetic GMA based potential sorbents for molybdenum and rhenium sorption. in Journal of Alloys and Compounds, 705, 38-50.
https://doi.org/10.1016/j.jallcom.2017.02.108
Marković BM, Vuković ZM, Spasojević V, Kusigerski V, Pavlović VB, Onjia AE, Nastasović AB. Selective magnetic GMA based potential sorbents for molybdenum and rhenium sorption. in Journal of Alloys and Compounds. 2017;705:38-50.
doi:10.1016/j.jallcom.2017.02.108 .
Marković, Bojana M., Vuković, Zorica M., Spasojević, Vojislav, Kusigerski, Vladan, Pavlović, Vladimir B., Onjia, Antonije E., Nastasović, Aleksandra B., "Selective magnetic GMA based potential sorbents for molybdenum and rhenium sorption" in Journal of Alloys and Compounds, 705 (2017):38-50,
https://doi.org/10.1016/j.jallcom.2017.02.108 . .
29
21
29

Exchange Bias Effect in NdFeO3 System of Nanoparticles

Vavra, M.; Zentkova, M.; Mihalik, M.; Mihalik, Jr., M.; Lazurova, J.; Girman, V.; Perović, Marija M.; Kusigerski, Vladan; Roupcova, P.; Jagličić, Zvonko

(2017)

TY  - JOUR
AU  - Vavra, M.
AU  - Zentkova, M.
AU  - Mihalik, M.
AU  - Mihalik, Jr., M.
AU  - Lazurova, J.
AU  - Girman, V.
AU  - Perović, Marija M.
AU  - Kusigerski, Vladan
AU  - Roupcova, P.
AU  - Jagličić, Zvonko
PY  - 2017
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/7162
AB  - We study the effect of nanometric size on the crystal structure, magnetic environment of iron and magnetization in NdFeO3 system of nanoparticles. The average particle size of NdFeO3 nanoparticles increases with annealing at 600 degrees C from about 15 nm to 40 nm, The smallest particles on annealed sample have size approximately 30 nm and typically have character of single crystalline samples. All samples adopt orthorhombic crystal structure, space group Prima with lattice parameters a = 5.5817 angstrom, b = 7.7663 angstrom and c = 5.456 angstrom for as prepared sample. The presence of superparamagnetic particles was indicated by the Mossbauer measurements. The reduction of dimensionality induces a decrease of T-N1 from 691 K to 544 K. The shift of magnetic hysteresis loop in vertical and horizontal direction was observed at low temperatures after cooling in magnetic field. We attribute such behaviour to exchange bias effect and discuss in the frame of core shellmodel.
T2  - Acta Physica Polonica A
T1  - Exchange Bias Effect in NdFeO3 System of Nanoparticles
VL  - 131
IS  - 4
SP  - 869
EP  - 871
DO  - 10.12693/APhysPolA.131.869
ER  - 
@article{
author = "Vavra, M. and Zentkova, M. and Mihalik, M. and Mihalik, Jr., M. and Lazurova, J. and Girman, V. and Perović, Marija M. and Kusigerski, Vladan and Roupcova, P. and Jagličić, Zvonko",
year = "2017",
abstract = "We study the effect of nanometric size on the crystal structure, magnetic environment of iron and magnetization in NdFeO3 system of nanoparticles. The average particle size of NdFeO3 nanoparticles increases with annealing at 600 degrees C from about 15 nm to 40 nm, The smallest particles on annealed sample have size approximately 30 nm and typically have character of single crystalline samples. All samples adopt orthorhombic crystal structure, space group Prima with lattice parameters a = 5.5817 angstrom, b = 7.7663 angstrom and c = 5.456 angstrom for as prepared sample. The presence of superparamagnetic particles was indicated by the Mossbauer measurements. The reduction of dimensionality induces a decrease of T-N1 from 691 K to 544 K. The shift of magnetic hysteresis loop in vertical and horizontal direction was observed at low temperatures after cooling in magnetic field. We attribute such behaviour to exchange bias effect and discuss in the frame of core shellmodel.",
journal = "Acta Physica Polonica A",
title = "Exchange Bias Effect in NdFeO3 System of Nanoparticles",
volume = "131",
number = "4",
pages = "869-871",
doi = "10.12693/APhysPolA.131.869"
}
Vavra, M., Zentkova, M., Mihalik, M., Mihalik, Jr., M., Lazurova, J., Girman, V., Perović, M. M., Kusigerski, V., Roupcova, P.,& Jagličić, Z.. (2017). Exchange Bias Effect in NdFeO3 System of Nanoparticles. in Acta Physica Polonica A, 131(4), 869-871.
https://doi.org/10.12693/APhysPolA.131.869
Vavra M, Zentkova M, Mihalik M, Mihalik JM, Lazurova J, Girman V, Perović MM, Kusigerski V, Roupcova P, Jagličić Z. Exchange Bias Effect in NdFeO3 System of Nanoparticles. in Acta Physica Polonica A. 2017;131(4):869-871.
doi:10.12693/APhysPolA.131.869 .
Vavra, M., Zentkova, M., Mihalik, M., Mihalik, Jr., M., Lazurova, J., Girman, V., Perović, Marija M., Kusigerski, Vladan, Roupcova, P., Jagličić, Zvonko, "Exchange Bias Effect in NdFeO3 System of Nanoparticles" in Acta Physica Polonica A, 131, no. 4 (2017):869-871,
https://doi.org/10.12693/APhysPolA.131.869 . .
6
3
7

Design of novel magnetic nanostructures for targeted tumour therapy - MagBioVin Project

Illés, Erzsébet; Knežević, Nikola; Mraković, Ana Đ.; Antić, Bratislav; Perović, Marija M.; Bošković, Marko; Kusigerski, Vladan; Vranješ-Đurić, Sanja; Peddis, Davide; Spasojević, Vojislav; Szytula, A.

(2016)

TY  - CONF
AU  - Illés, Erzsébet
AU  - Knežević, Nikola
AU  - Mraković, Ana Đ.
AU  - Antić, Bratislav
AU  - Perović, Marija M.
AU  - Bošković, Marko
AU  - Kusigerski, Vladan
AU  - Vranješ-Đurić, Sanja
AU  - Peddis, Davide
AU  - Spasojević, Vojislav
AU  - Szytula, A.
PY  - 2016
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/10828
AB  - We present here some recent research advancements and opportunities within the FP7-ERA Chairs MagBioVin project. The project aims to design various novel magnetic nanoarchitectures (e.g. bimagnetic and polymeric core-shell systems, nanoparticles embedded in mesoporous silica and radiolabeled nanostructures) for application in targeted treatment and diagnostics of cancer. The magnetic core of these nanomaterials allows the selective treatment of tumor tissues (i.e. targeted drug-delivery, localized magnetic hyperthermia) by magnetic field. Attachment of radionuclides (e.g. 90Y, 99mTc, 134I) to the nanoparticles opens the possibilities for imaging and internal radiotherapy. Magnetic nanoparticles (MNPs), i.e. iron oxides and spinel ferrites, were synthesized by different methods and coated by several compounds (e.g. citrate, polymers, silica, BSA) to increase their biocompatibility. The composition and morphology of the nanomaterials is characterized by XRD, TEM imaging and infrared spectroscopy, while their magnetic properties were studied by SQUID magnetometry and Mössbauer spectroscopy. Magnetic hyperthermia effects were monitored by DM100 device equipped with DM1, 2 and 3 applicators (nB nanoScale Biomagnetics). This unique setup allows us to monitor the heating efficiency development in cell cultures and small animals (e.g. mice, rats) as well. The current results showed that the MNPs can be successfully labeled with 90Y and 99mTc. The drug loading and release properties of MNPs are studied by HPLC using doxorubicin as the drug. In vitro and in vivo (animal model) applicability of the synthesized nanomaterials regarding toxicity, biodistribution and anti-cancer efficacy is explored for targeted cancer treatment.
C3  - Clinical Chemistry and Laboratory Medicine
T1  - Design of novel magnetic nanostructures for targeted tumour therapy - MagBioVin Project
VL  - 54
IS  - 10
SP  - eA187
DO  - 10.1515/cclm-2016-0583
ER  - 
@conference{
author = "Illés, Erzsébet and Knežević, Nikola and Mraković, Ana Đ. and Antić, Bratislav and Perović, Marija M. and Bošković, Marko and Kusigerski, Vladan and Vranješ-Đurić, Sanja and Peddis, Davide and Spasojević, Vojislav and Szytula, A.",
year = "2016",
abstract = "We present here some recent research advancements and opportunities within the FP7-ERA Chairs MagBioVin project. The project aims to design various novel magnetic nanoarchitectures (e.g. bimagnetic and polymeric core-shell systems, nanoparticles embedded in mesoporous silica and radiolabeled nanostructures) for application in targeted treatment and diagnostics of cancer. The magnetic core of these nanomaterials allows the selective treatment of tumor tissues (i.e. targeted drug-delivery, localized magnetic hyperthermia) by magnetic field. Attachment of radionuclides (e.g. 90Y, 99mTc, 134I) to the nanoparticles opens the possibilities for imaging and internal radiotherapy. Magnetic nanoparticles (MNPs), i.e. iron oxides and spinel ferrites, were synthesized by different methods and coated by several compounds (e.g. citrate, polymers, silica, BSA) to increase their biocompatibility. The composition and morphology of the nanomaterials is characterized by XRD, TEM imaging and infrared spectroscopy, while their magnetic properties were studied by SQUID magnetometry and Mössbauer spectroscopy. Magnetic hyperthermia effects were monitored by DM100 device equipped with DM1, 2 and 3 applicators (nB nanoScale Biomagnetics). This unique setup allows us to monitor the heating efficiency development in cell cultures and small animals (e.g. mice, rats) as well. The current results showed that the MNPs can be successfully labeled with 90Y and 99mTc. The drug loading and release properties of MNPs are studied by HPLC using doxorubicin as the drug. In vitro and in vivo (animal model) applicability of the synthesized nanomaterials regarding toxicity, biodistribution and anti-cancer efficacy is explored for targeted cancer treatment.",
journal = "Clinical Chemistry and Laboratory Medicine",
title = "Design of novel magnetic nanostructures for targeted tumour therapy - MagBioVin Project",
volume = "54",
number = "10",
pages = "eA187",
doi = "10.1515/cclm-2016-0583"
}
Illés, E., Knežević, N., Mraković, A. Đ., Antić, B., Perović, M. M., Bošković, M., Kusigerski, V., Vranješ-Đurić, S., Peddis, D., Spasojević, V.,& Szytula, A.. (2016). Design of novel magnetic nanostructures for targeted tumour therapy - MagBioVin Project. in Clinical Chemistry and Laboratory Medicine, 54(10), eA187.
https://doi.org/10.1515/cclm-2016-0583
Illés E, Knežević N, Mraković AĐ, Antić B, Perović MM, Bošković M, Kusigerski V, Vranješ-Đurić S, Peddis D, Spasojević V, Szytula A. Design of novel magnetic nanostructures for targeted tumour therapy - MagBioVin Project. in Clinical Chemistry and Laboratory Medicine. 2016;54(10):eA187.
doi:10.1515/cclm-2016-0583 .
Illés, Erzsébet, Knežević, Nikola, Mraković, Ana Đ., Antić, Bratislav, Perović, Marija M., Bošković, Marko, Kusigerski, Vladan, Vranješ-Đurić, Sanja, Peddis, Davide, Spasojević, Vojislav, Szytula, A., "Design of novel magnetic nanostructures for targeted tumour therapy - MagBioVin Project" in Clinical Chemistry and Laboratory Medicine, 54, no. 10 (2016):eA187,
https://doi.org/10.1515/cclm-2016-0583 . .

Structural and magnetic properties of mechanochemically synthesized LaFe1-xCrxO3 (x = 0.5 and 0.75)

Jugović, Dragana; Bradarić, Ivica; Jovalekić, Čedomir; Barudžija, Tanja; Kusigerski, Vladan; Mitrić, Miodrag

(Belgrade : Materials Research Society of Serbia, 2016)

TY  - CONF
AU  - Jugović, Dragana
AU  - Bradarić, Ivica
AU  - Jovalekić, Čedomir
AU  - Barudžija, Tanja
AU  - Kusigerski, Vladan
AU  - Mitrić, Miodrag
PY  - 2016
UR  - http://dais.sanu.ac.rs/123456789/897
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/7554
AB  - Perovskite oxides with the composition LaFe1-xCrxO3 (x = 0.5 and 0.75) have been studied. The samples have been prepared using the mechanochemical treatment. A mixture of crystalline La(OH)3, Fe2O3 and Cr2O3 powders in stoichiometric ratio was mechanochemically treated in a planetary ball mill up to 40 h of milling. The mechanochemical formation of the LaFe1-xCrxO3 perovskite phase was followed by X-ray diffraction and magnetization measurements. The Rietveld refinement of the XRD data shows that the compounds crystallize in an orthorhombic perovskite structure with a random distribution of the Fe and Cr cations at the B sublattice. All structural and microstructural parameters were analyzed. In addition, magnetic measurements for LaFe0.5Cr0.5O3 show clear antiferromagnetic ordering bellow 250 K, which supports above conclusion of random distribution of Fe and Cr cations.
PB  - Belgrade : Materials Research Society of Serbia
C3  - YUCOMAT 2016 : 18th Annual Conference YUCOMAT 2016 : programme and the book of abstracts; September 5-10, Herceg Novi
T1  - Structural and magnetic properties of mechanochemically synthesized LaFe1-xCrxO3 (x = 0.5 and 0.75)
SP  - 57
EP  - 57
UR  - https://hdl.handle.net/21.15107/rcub_vinar_7554
ER  - 
@conference{
author = "Jugović, Dragana and Bradarić, Ivica and Jovalekić, Čedomir and Barudžija, Tanja and Kusigerski, Vladan and Mitrić, Miodrag",
year = "2016",
abstract = "Perovskite oxides with the composition LaFe1-xCrxO3 (x = 0.5 and 0.75) have been studied. The samples have been prepared using the mechanochemical treatment. A mixture of crystalline La(OH)3, Fe2O3 and Cr2O3 powders in stoichiometric ratio was mechanochemically treated in a planetary ball mill up to 40 h of milling. The mechanochemical formation of the LaFe1-xCrxO3 perovskite phase was followed by X-ray diffraction and magnetization measurements. The Rietveld refinement of the XRD data shows that the compounds crystallize in an orthorhombic perovskite structure with a random distribution of the Fe and Cr cations at the B sublattice. All structural and microstructural parameters were analyzed. In addition, magnetic measurements for LaFe0.5Cr0.5O3 show clear antiferromagnetic ordering bellow 250 K, which supports above conclusion of random distribution of Fe and Cr cations.",
publisher = "Belgrade : Materials Research Society of Serbia",
journal = "YUCOMAT 2016 : 18th Annual Conference YUCOMAT 2016 : programme and the book of abstracts; September 5-10, Herceg Novi",
title = "Structural and magnetic properties of mechanochemically synthesized LaFe1-xCrxO3 (x = 0.5 and 0.75)",
pages = "57-57",
url = "https://hdl.handle.net/21.15107/rcub_vinar_7554"
}
Jugović, D., Bradarić, I., Jovalekić, Č., Barudžija, T., Kusigerski, V.,& Mitrić, M.. (2016). Structural and magnetic properties of mechanochemically synthesized LaFe1-xCrxO3 (x = 0.5 and 0.75). in YUCOMAT 2016 : 18th Annual Conference YUCOMAT 2016 : programme and the book of abstracts; September 5-10, Herceg Novi
Belgrade : Materials Research Society of Serbia., 57-57.
https://hdl.handle.net/21.15107/rcub_vinar_7554
Jugović D, Bradarić I, Jovalekić Č, Barudžija T, Kusigerski V, Mitrić M. Structural and magnetic properties of mechanochemically synthesized LaFe1-xCrxO3 (x = 0.5 and 0.75). in YUCOMAT 2016 : 18th Annual Conference YUCOMAT 2016 : programme and the book of abstracts; September 5-10, Herceg Novi. 2016;:57-57.
https://hdl.handle.net/21.15107/rcub_vinar_7554 .
Jugović, Dragana, Bradarić, Ivica, Jovalekić, Čedomir, Barudžija, Tanja, Kusigerski, Vladan, Mitrić, Miodrag, "Structural and magnetic properties of mechanochemically synthesized LaFe1-xCrxO3 (x = 0.5 and 0.75)" in YUCOMAT 2016 : 18th Annual Conference YUCOMAT 2016 : programme and the book of abstracts; September 5-10, Herceg Novi (2016):57-57,
https://hdl.handle.net/21.15107/rcub_vinar_7554 .

Corrigendum: Effects of sintering on the structural, micro structural and magnetic properties of nanoparticle manganite Ca1-xGdxMnO3 (x=0.05, 0.1, 0.15, 0.2) (vol 41, pg 14964, 2015)

Rosić, Milena; Kljajević, Ljiljana M.; Jordanov, Dragana; Stoiljković, Milovan; Kusigerski, Vladan; Spasojević, Vojislav; Matović, Branko

(Elsevier, 2016)

TY  - JOUR
AU  - Rosić, Milena
AU  - Kljajević, Ljiljana M.
AU  - Jordanov, Dragana
AU  - Stoiljković, Milovan
AU  - Kusigerski, Vladan
AU  - Spasojević, Vojislav
AU  - Matović, Branko
PY  - 2016
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/980
AB  - Nanocrystalline manganites Ca1−xGdxMnO3 (x=0.05, 0.1, 0.15, and 0.2) were synthesized by a modified glycine-nitrate procedure and subjected to a systematic investigation regarding the effects of calcination and sintering on their structural, microstructural and magnetic properties. Thermal treatments of the green bodies were carried out by the conventional sintering (CS) method and the effects were monitored by different experimental techniques (XRD, ICP, FTIR, SEM, and EDS). The obtained results showed that induced structural/microstructural changes were not simple functions of the dopant concentration x and that they were influenced by different material-specific processes. Magnetism of the final bulk powders have been investigated by SQUID-magnetometry and correlated with samples composition and structural/microstructural properties.
PB  - Elsevier
T2  - Ceramics International
T1  - Corrigendum: Effects of sintering on the structural, micro structural and magnetic properties of nanoparticle manganite Ca1-xGdxMnO3 (x=0.05, 0.1, 0.15, 0.2) (vol 41, pg 14964, 2015)
VL  - 42
IS  - 6
SP  - 7895
EP  - 7895
DO  - 10.1016/j.ceramint.2016.01.134
ER  - 
@article{
author = "Rosić, Milena and Kljajević, Ljiljana M. and Jordanov, Dragana and Stoiljković, Milovan and Kusigerski, Vladan and Spasojević, Vojislav and Matović, Branko",
year = "2016",
abstract = "Nanocrystalline manganites Ca1−xGdxMnO3 (x=0.05, 0.1, 0.15, and 0.2) were synthesized by a modified glycine-nitrate procedure and subjected to a systematic investigation regarding the effects of calcination and sintering on their structural, microstructural and magnetic properties. Thermal treatments of the green bodies were carried out by the conventional sintering (CS) method and the effects were monitored by different experimental techniques (XRD, ICP, FTIR, SEM, and EDS). The obtained results showed that induced structural/microstructural changes were not simple functions of the dopant concentration x and that they were influenced by different material-specific processes. Magnetism of the final bulk powders have been investigated by SQUID-magnetometry and correlated with samples composition and structural/microstructural properties.",
publisher = "Elsevier",
journal = "Ceramics International",
title = "Corrigendum: Effects of sintering on the structural, micro structural and magnetic properties of nanoparticle manganite Ca1-xGdxMnO3 (x=0.05, 0.1, 0.15, 0.2) (vol 41, pg 14964, 2015)",
volume = "42",
number = "6",
pages = "7895-7895",
doi = "10.1016/j.ceramint.2016.01.134"
}
Rosić, M., Kljajević, L. M., Jordanov, D., Stoiljković, M., Kusigerski, V., Spasojević, V.,& Matović, B.. (2016). Corrigendum: Effects of sintering on the structural, micro structural and magnetic properties of nanoparticle manganite Ca1-xGdxMnO3 (x=0.05, 0.1, 0.15, 0.2) (vol 41, pg 14964, 2015). in Ceramics International
Elsevier., 42(6), 7895-7895.
https://doi.org/10.1016/j.ceramint.2016.01.134
Rosić M, Kljajević LM, Jordanov D, Stoiljković M, Kusigerski V, Spasojević V, Matović B. Corrigendum: Effects of sintering on the structural, micro structural and magnetic properties of nanoparticle manganite Ca1-xGdxMnO3 (x=0.05, 0.1, 0.15, 0.2) (vol 41, pg 14964, 2015). in Ceramics International. 2016;42(6):7895-7895.
doi:10.1016/j.ceramint.2016.01.134 .
Rosić, Milena, Kljajević, Ljiljana M., Jordanov, Dragana, Stoiljković, Milovan, Kusigerski, Vladan, Spasojević, Vojislav, Matović, Branko, "Corrigendum: Effects of sintering on the structural, micro structural and magnetic properties of nanoparticle manganite Ca1-xGdxMnO3 (x=0.05, 0.1, 0.15, 0.2) (vol 41, pg 14964, 2015)" in Ceramics International, 42, no. 6 (2016):7895-7895,
https://doi.org/10.1016/j.ceramint.2016.01.134 . .

Development of Novel Approaches for Tumour Therapy based on Nanostructured Materials - MagBioVin Project

Knežević, Nikola; Illés, E.; Mraković, Ana; Perović, Marija; Bošković, Marko; Kusigerski, Vladan; Vranješ-Đurić, Sanja; Peddis, D.; Spasojević, Vojislav; Szytula, Andrzej

(2016)

TY  - CONF
AU  - Knežević, Nikola
AU  - Illés, E.
AU  - Mraković, Ana
AU  - Perović, Marija
AU  - Bošković, Marko
AU  - Kusigerski, Vladan
AU  - Vranješ-Đurić, Sanja
AU  - Peddis, D.
AU  - Spasojević, Vojislav
AU  - Szytula, Andrzej
PY  - 2016
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/10829
UR  - https://nanosymposiumatuclan.files.wordpress.com/2015/09/conference-abstract-proceedings_post-symposium-version.pdf
AB  - Research advancements and opportunities by the FP7-ERA Chairs project MagBioVin are spotlighted.[1] Topic of the project is the design of different novel magnetic nanoarchitectures (e.g. bimagnetic and polymeric core-shell systems, nanoparticles embedded in mesoporous silica structures, and radiolabeled nanostructures)[2–4] for application in targeted treatment and diagnostics of cancer. These nanomaterials posses the ability for selective treatment of tumor tissues by the targeting with magnetic field.[5,6] Alternating magnetic field also provides the means for hyperthermia-induced cancer treatment.[7]Attachment of radionuclides to the synthesized nanoparticles is explored for the purpose of imaging and internal radiotherapy.[8,9] Magnetic characteristics of the prepared nanomaterials is done by SQUID magnetometry and Mössbauer spectroscopy. Structural characterization of the investigated nanomaterials is performed by XRD, TEM imaging, DRIFT spectroscopy, and nitrogen sorption analysis. Magnetic hyperthermia effects are monitored by using commercial setup (nB nanoScale Biomagnetics) which includes applicators for cell cultures and small animals. In vitro and in vivo (animal model) applicability of the synthesized nanomaterials regarding toxicity, biodistribution and anticancer efficacy is explored for targeted cancer treatment.
C3  - Functional Nanomaterials in Industrial Applications: Academic-Industry Meet, Conference Abstract Proceedings
T1  - Development of Novel Approaches for Tumour Therapy based on Nanostructured Materials - MagBioVin Project
SP  - 61
UR  - https://hdl.handle.net/21.15107/rcub_vinar_10829
ER  - 
@conference{
author = "Knežević, Nikola and Illés, E. and Mraković, Ana and Perović, Marija and Bošković, Marko and Kusigerski, Vladan and Vranješ-Đurić, Sanja and Peddis, D. and Spasojević, Vojislav and Szytula, Andrzej",
year = "2016",
abstract = "Research advancements and opportunities by the FP7-ERA Chairs project MagBioVin are spotlighted.[1] Topic of the project is the design of different novel magnetic nanoarchitectures (e.g. bimagnetic and polymeric core-shell systems, nanoparticles embedded in mesoporous silica structures, and radiolabeled nanostructures)[2–4] for application in targeted treatment and diagnostics of cancer. These nanomaterials posses the ability for selective treatment of tumor tissues by the targeting with magnetic field.[5,6] Alternating magnetic field also provides the means for hyperthermia-induced cancer treatment.[7]Attachment of radionuclides to the synthesized nanoparticles is explored for the purpose of imaging and internal radiotherapy.[8,9] Magnetic characteristics of the prepared nanomaterials is done by SQUID magnetometry and Mössbauer spectroscopy. Structural characterization of the investigated nanomaterials is performed by XRD, TEM imaging, DRIFT spectroscopy, and nitrogen sorption analysis. Magnetic hyperthermia effects are monitored by using commercial setup (nB nanoScale Biomagnetics) which includes applicators for cell cultures and small animals. In vitro and in vivo (animal model) applicability of the synthesized nanomaterials regarding toxicity, biodistribution and anticancer efficacy is explored for targeted cancer treatment.",
journal = "Functional Nanomaterials in Industrial Applications: Academic-Industry Meet, Conference Abstract Proceedings",
title = "Development of Novel Approaches for Tumour Therapy based on Nanostructured Materials - MagBioVin Project",
pages = "61",
url = "https://hdl.handle.net/21.15107/rcub_vinar_10829"
}
Knežević, N., Illés, E., Mraković, A., Perović, M., Bošković, M., Kusigerski, V., Vranješ-Đurić, S., Peddis, D., Spasojević, V.,& Szytula, A.. (2016). Development of Novel Approaches for Tumour Therapy based on Nanostructured Materials - MagBioVin Project. in Functional Nanomaterials in Industrial Applications: Academic-Industry Meet, Conference Abstract Proceedings, 61.
https://hdl.handle.net/21.15107/rcub_vinar_10829
Knežević N, Illés E, Mraković A, Perović M, Bošković M, Kusigerski V, Vranješ-Đurić S, Peddis D, Spasojević V, Szytula A. Development of Novel Approaches for Tumour Therapy based on Nanostructured Materials - MagBioVin Project. in Functional Nanomaterials in Industrial Applications: Academic-Industry Meet, Conference Abstract Proceedings. 2016;:61.
https://hdl.handle.net/21.15107/rcub_vinar_10829 .
Knežević, Nikola, Illés, E., Mraković, Ana, Perović, Marija, Bošković, Marko, Kusigerski, Vladan, Vranješ-Đurić, Sanja, Peddis, D., Spasojević, Vojislav, Szytula, Andrzej, "Development of Novel Approaches for Tumour Therapy based on Nanostructured Materials - MagBioVin Project" in Functional Nanomaterials in Industrial Applications: Academic-Industry Meet, Conference Abstract Proceedings (2016):61,
https://hdl.handle.net/21.15107/rcub_vinar_10829 .

Structural and magnetic properties of hydrothermally synthesized beta-MnO2 and alpha-KxMnO2 nanorods

Barudžija, Tanja; Kusigerski, Vladan; Cvjetićanin, Nikola; Šorgić, Saša; Perović, Marija M.; Mitrić, Miodrag

(Elsevier, 2016)

TY  - JOUR
AU  - Barudžija, Tanja
AU  - Kusigerski, Vladan
AU  - Cvjetićanin, Nikola
AU  - Šorgić, Saša
AU  - Perović, Marija M.
AU  - Mitrić, Miodrag
PY  - 2016
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/920
AB  - Hydrothermal synthesis was applied for obtaining different manganese dioxide polymorphs whose morphology, structure and magnetic properties were thoroughly investigated. Variations in the synthesis pathways lead to the formation of tetragonal rutile-type beta-MnO2 and two tetragonal hollandite-type alpha-KxMnO2 samples with different concentration of potassium cations (x = 0.15 and 0.18). SEM images showed nanorod shape of all specimens, while microstructure characterization done by XRD measurements revealed that crystallites have an elongated rod-like shape and, hence, it confirmed the anisotropic morphology. Magnetic ordering of beta-MnO2 is antiferromagnetic below 93 K, while both alpha-KxMnO2 samples possess more complicated low-temperature behaviour of the reentrant spin-glass type: the onset of the spin-glass like state occurs at temperatures below the weak ferromagnetic ordering. (C) 2016 Elsevier B.V. All rights reserved.
PB  - Elsevier
T2  - Journal of Alloys and Compounds
T1  - Structural and magnetic properties of hydrothermally synthesized beta-MnO2 and alpha-KxMnO2 nanorods
VL  - 665
SP  - 261
EP  - 270
DO  - 10.1016/j.jallcom.2016.01.024
ER  - 
@article{
author = "Barudžija, Tanja and Kusigerski, Vladan and Cvjetićanin, Nikola and Šorgić, Saša and Perović, Marija M. and Mitrić, Miodrag",
year = "2016",
abstract = "Hydrothermal synthesis was applied for obtaining different manganese dioxide polymorphs whose morphology, structure and magnetic properties were thoroughly investigated. Variations in the synthesis pathways lead to the formation of tetragonal rutile-type beta-MnO2 and two tetragonal hollandite-type alpha-KxMnO2 samples with different concentration of potassium cations (x = 0.15 and 0.18). SEM images showed nanorod shape of all specimens, while microstructure characterization done by XRD measurements revealed that crystallites have an elongated rod-like shape and, hence, it confirmed the anisotropic morphology. Magnetic ordering of beta-MnO2 is antiferromagnetic below 93 K, while both alpha-KxMnO2 samples possess more complicated low-temperature behaviour of the reentrant spin-glass type: the onset of the spin-glass like state occurs at temperatures below the weak ferromagnetic ordering. (C) 2016 Elsevier B.V. All rights reserved.",
publisher = "Elsevier",
journal = "Journal of Alloys and Compounds",
title = "Structural and magnetic properties of hydrothermally synthesized beta-MnO2 and alpha-KxMnO2 nanorods",
volume = "665",
pages = "261-270",
doi = "10.1016/j.jallcom.2016.01.024"
}
Barudžija, T., Kusigerski, V., Cvjetićanin, N., Šorgić, S., Perović, M. M.,& Mitrić, M.. (2016). Structural and magnetic properties of hydrothermally synthesized beta-MnO2 and alpha-KxMnO2 nanorods. in Journal of Alloys and Compounds
Elsevier., 665, 261-270.
https://doi.org/10.1016/j.jallcom.2016.01.024
Barudžija T, Kusigerski V, Cvjetićanin N, Šorgić S, Perović MM, Mitrić M. Structural and magnetic properties of hydrothermally synthesized beta-MnO2 and alpha-KxMnO2 nanorods. in Journal of Alloys and Compounds. 2016;665:261-270.
doi:10.1016/j.jallcom.2016.01.024 .
Barudžija, Tanja, Kusigerski, Vladan, Cvjetićanin, Nikola, Šorgić, Saša, Perović, Marija M., Mitrić, Miodrag, "Structural and magnetic properties of hydrothermally synthesized beta-MnO2 and alpha-KxMnO2 nanorods" in Journal of Alloys and Compounds, 665 (2016):261-270,
https://doi.org/10.1016/j.jallcom.2016.01.024 . .
22
18
24

Experimental evidence for simultaneous relaxation processes in super spin glass gamma-Fe2O3 nanoparticle system

Nikolić, Violeta N.; Perović, Marija M.; Kusigerski, Vladan; Bošković, Marko; Mraković, Ana Đ.; Blanuša, Jovan; Spasojević, Vojislav

(2015)

TY  - JOUR
AU  - Nikolić, Violeta N.
AU  - Perović, Marija M.
AU  - Kusigerski, Vladan
AU  - Bošković, Marko
AU  - Mraković, Ana Đ.
AU  - Blanuša, Jovan
AU  - Spasojević, Vojislav
PY  - 2015
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/561
AB  - Spherical gamma-Fe2O3 nanoparticles with the narrow size distribution of (5 +/- 1) nm were synthesized by the method of thermal decomposition from iron acetyl acetonate precursor. The existence of super spin-glass state at low temperatures and in low applied magnetic fields was confirmed by DC magnetization measurements on a SQUID magnetometer. The comprehensive investigation of magnetic relaxation dynamics in low-temperature region was conducted through the measurements of single-stop and multiple stop ZFC memory effects, ZFC magnetization relaxation, and AC susceptibility measurements. The experimental findings revealed the peculiar change of magnetic relaxation dynamics at T approximate to 10 K, which arose as a consequence of simultaneous existence of different relaxation processes in Fe2O3 nanoparticle system. Complementarity of the applied measurements was utilized in order to single out distinct relaxation processes as well as to elucidate complex relaxation mechanisms in the investigated interacting nanoparticle system.
T2  - Journal of Nanoparticle Research
T1  - Experimental evidence for simultaneous relaxation processes in super spin glass gamma-Fe2O3 nanoparticle system
VL  - 17
IS  - 3
DO  - 10.1007/s11051-015-2952-2
ER  - 
@article{
author = "Nikolić, Violeta N. and Perović, Marija M. and Kusigerski, Vladan and Bošković, Marko and Mraković, Ana Đ. and Blanuša, Jovan and Spasojević, Vojislav",
year = "2015",
abstract = "Spherical gamma-Fe2O3 nanoparticles with the narrow size distribution of (5 +/- 1) nm were synthesized by the method of thermal decomposition from iron acetyl acetonate precursor. The existence of super spin-glass state at low temperatures and in low applied magnetic fields was confirmed by DC magnetization measurements on a SQUID magnetometer. The comprehensive investigation of magnetic relaxation dynamics in low-temperature region was conducted through the measurements of single-stop and multiple stop ZFC memory effects, ZFC magnetization relaxation, and AC susceptibility measurements. The experimental findings revealed the peculiar change of magnetic relaxation dynamics at T approximate to 10 K, which arose as a consequence of simultaneous existence of different relaxation processes in Fe2O3 nanoparticle system. Complementarity of the applied measurements was utilized in order to single out distinct relaxation processes as well as to elucidate complex relaxation mechanisms in the investigated interacting nanoparticle system.",
journal = "Journal of Nanoparticle Research",
title = "Experimental evidence for simultaneous relaxation processes in super spin glass gamma-Fe2O3 nanoparticle system",
volume = "17",
number = "3",
doi = "10.1007/s11051-015-2952-2"
}
Nikolić, V. N., Perović, M. M., Kusigerski, V., Bošković, M., Mraković, A. Đ., Blanuša, J.,& Spasojević, V.. (2015). Experimental evidence for simultaneous relaxation processes in super spin glass gamma-Fe2O3 nanoparticle system. in Journal of Nanoparticle Research, 17(3).
https://doi.org/10.1007/s11051-015-2952-2
Nikolić VN, Perović MM, Kusigerski V, Bošković M, Mraković AĐ, Blanuša J, Spasojević V. Experimental evidence for simultaneous relaxation processes in super spin glass gamma-Fe2O3 nanoparticle system. in Journal of Nanoparticle Research. 2015;17(3).
doi:10.1007/s11051-015-2952-2 .
Nikolić, Violeta N., Perović, Marija M., Kusigerski, Vladan, Bošković, Marko, Mraković, Ana Đ., Blanuša, Jovan, Spasojević, Vojislav, "Experimental evidence for simultaneous relaxation processes in super spin glass gamma-Fe2O3 nanoparticle system" in Journal of Nanoparticle Research, 17, no. 3 (2015),
https://doi.org/10.1007/s11051-015-2952-2 . .
4
3
3

The glassy behaviour of poorly crystalline Fe2O3 nanorods obtained by thermal decomposition of ferrous oxalate

Perović, Marija M.; Kusigerski, Vladan; Mraković, Ana Đ.; Spasojević, Vojislav; Blanuša, Jovan; Nikolić, Violeta N.; Schneeweiss, Oldřich B.; David, B.; Pizurova, Nadežda

(2015)

TY  - JOUR
AU  - Perović, Marija M.
AU  - Kusigerski, Vladan
AU  - Mraković, Ana Đ.
AU  - Spasojević, Vojislav
AU  - Blanuša, Jovan
AU  - Nikolić, Violeta N.
AU  - Schneeweiss, Oldřich B.
AU  - David, B.
AU  - Pizurova, Nadežda
PY  - 2015
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/429
AB  - Nanorod ferrous oxalate dihydrate (FeC2O4 x 2H(2)O) which had been synthesized by the microemulsion method, was used as a precursor in the thermal decomposition process performed in air atmosphere. The formation of nanocrystalline hematite as the final product was preceded by the appearence of an intermediate product. Comprehensive study comprising several complementary techniques (x-ray diffraction, transmission electron microscopy, selected area electron diffraction, thermogravimetric/differential thermal analyses and SQUID magnetometry) confirmed that the intermediate product corresponds to the poorly crystalline Fe2O3. Due to the specific nanorod shape and poorly crystalline structure, the investigated Fe2O3 showed high coercive field value of similar to 0.5 T at 5 K. Special attention in this study was devoted to the peculiar magnetic properties of poorly crystalline Fe2O3, which were thoroughly investigated by employing sophisticated experimental procedures such as relaxation of thermoremanent magnetization for different cooling fields, zero field and field cooled memory effects as well as aging experiments for different waiting times. At low temperatures and weak applied magnetic fields, the investigated system behaves similarly to spin glasses, manifesting slow, collective relaxation dynamics of magnetic moments through memory, rejuvenation and aging effects.
T2  - Nanotechnology
T1  - The glassy behaviour of poorly crystalline Fe2O3 nanorods obtained by thermal decomposition of ferrous oxalate
VL  - 26
IS  - 11
DO  - 10.1088/0957-4484/26/11/115705
ER  - 
@article{
author = "Perović, Marija M. and Kusigerski, Vladan and Mraković, Ana Đ. and Spasojević, Vojislav and Blanuša, Jovan and Nikolić, Violeta N. and Schneeweiss, Oldřich B. and David, B. and Pizurova, Nadežda",
year = "2015",
abstract = "Nanorod ferrous oxalate dihydrate (FeC2O4 x 2H(2)O) which had been synthesized by the microemulsion method, was used as a precursor in the thermal decomposition process performed in air atmosphere. The formation of nanocrystalline hematite as the final product was preceded by the appearence of an intermediate product. Comprehensive study comprising several complementary techniques (x-ray diffraction, transmission electron microscopy, selected area electron diffraction, thermogravimetric/differential thermal analyses and SQUID magnetometry) confirmed that the intermediate product corresponds to the poorly crystalline Fe2O3. Due to the specific nanorod shape and poorly crystalline structure, the investigated Fe2O3 showed high coercive field value of similar to 0.5 T at 5 K. Special attention in this study was devoted to the peculiar magnetic properties of poorly crystalline Fe2O3, which were thoroughly investigated by employing sophisticated experimental procedures such as relaxation of thermoremanent magnetization for different cooling fields, zero field and field cooled memory effects as well as aging experiments for different waiting times. At low temperatures and weak applied magnetic fields, the investigated system behaves similarly to spin glasses, manifesting slow, collective relaxation dynamics of magnetic moments through memory, rejuvenation and aging effects.",
journal = "Nanotechnology",
title = "The glassy behaviour of poorly crystalline Fe2O3 nanorods obtained by thermal decomposition of ferrous oxalate",
volume = "26",
number = "11",
doi = "10.1088/0957-4484/26/11/115705"
}
Perović, M. M., Kusigerski, V., Mraković, A. Đ., Spasojević, V., Blanuša, J., Nikolić, V. N., Schneeweiss, O. B., David, B.,& Pizurova, N.. (2015). The glassy behaviour of poorly crystalline Fe2O3 nanorods obtained by thermal decomposition of ferrous oxalate. in Nanotechnology, 26(11).
https://doi.org/10.1088/0957-4484/26/11/115705
Perović MM, Kusigerski V, Mraković AĐ, Spasojević V, Blanuša J, Nikolić VN, Schneeweiss OB, David B, Pizurova N. The glassy behaviour of poorly crystalline Fe2O3 nanorods obtained by thermal decomposition of ferrous oxalate. in Nanotechnology. 2015;26(11).
doi:10.1088/0957-4484/26/11/115705 .
Perović, Marija M., Kusigerski, Vladan, Mraković, Ana Đ., Spasojević, Vojislav, Blanuša, Jovan, Nikolić, Violeta N., Schneeweiss, Oldřich B., David, B., Pizurova, Nadežda, "The glassy behaviour of poorly crystalline Fe2O3 nanorods obtained by thermal decomposition of ferrous oxalate" in Nanotechnology, 26, no. 11 (2015),
https://doi.org/10.1088/0957-4484/26/11/115705 . .
6
4
5

Correlation between morphology and magnetic properties of electrochemically produced cobalt powder particles

Maksimović, Vesna; Nikolić, Nebojša D.; Kusigerski, Vladan; Blanuša, Jovan

(2015)

TY  - JOUR
AU  - Maksimović, Vesna
AU  - Nikolić, Nebojša D.
AU  - Kusigerski, Vladan
AU  - Blanuša, Jovan
PY  - 2015
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/453
AB  - Cobalt 3D powder particles were successfully prepared by galvanostatic electrodeposition. The electrodeposited cobalt powders were characterized by X-ray diffraction (XRD) analysis, scanning electron microscopy (SEM), energy dispersive spectroscopy (EDS) and SQUID magnetometry. It was shown that the morphology, structure and magnetic properties of cobalt particles were closely associated and could be easily controlled by adjusting the electrodeposition process parameters. The morphology of cobalt powder particles was strongly affected by the hydrogen evolution reaction as a parallel reaction to cobalt electrodeposition. Depending on the applied current density, two types of powder particles were formed: dendrites at lower and spongy-like particles at higher current densities. Morphologies and structures of powder particles were correlated with their magnetic properties, and compared with those of the bulk cobalt. In comparison with the properties of bulk cobalt, the obtained 3D structutes exhibited a decreased saturation magnetization (M-S), but an enhanced coercivity (H-C), which was explained by their peculiar morphology.
T2  - Journal of the Serbian Chemical Society
T1  - Correlation between morphology and magnetic properties of electrochemically produced cobalt powder particles
VL  - 80
IS  - 2
SP  - 197
EP  - 207
DO  - 10.2298/JSC200814104M
ER  - 
@article{
author = "Maksimović, Vesna and Nikolić, Nebojša D. and Kusigerski, Vladan and Blanuša, Jovan",
year = "2015",
abstract = "Cobalt 3D powder particles were successfully prepared by galvanostatic electrodeposition. The electrodeposited cobalt powders were characterized by X-ray diffraction (XRD) analysis, scanning electron microscopy (SEM), energy dispersive spectroscopy (EDS) and SQUID magnetometry. It was shown that the morphology, structure and magnetic properties of cobalt particles were closely associated and could be easily controlled by adjusting the electrodeposition process parameters. The morphology of cobalt powder particles was strongly affected by the hydrogen evolution reaction as a parallel reaction to cobalt electrodeposition. Depending on the applied current density, two types of powder particles were formed: dendrites at lower and spongy-like particles at higher current densities. Morphologies and structures of powder particles were correlated with their magnetic properties, and compared with those of the bulk cobalt. In comparison with the properties of bulk cobalt, the obtained 3D structutes exhibited a decreased saturation magnetization (M-S), but an enhanced coercivity (H-C), which was explained by their peculiar morphology.",
journal = "Journal of the Serbian Chemical Society",
title = "Correlation between morphology and magnetic properties of electrochemically produced cobalt powder particles",
volume = "80",
number = "2",
pages = "197-207",
doi = "10.2298/JSC200814104M"
}
Maksimović, V., Nikolić, N. D., Kusigerski, V.,& Blanuša, J.. (2015). Correlation between morphology and magnetic properties of electrochemically produced cobalt powder particles. in Journal of the Serbian Chemical Society, 80(2), 197-207.
https://doi.org/10.2298/JSC200814104M
Maksimović V, Nikolić ND, Kusigerski V, Blanuša J. Correlation between morphology and magnetic properties of electrochemically produced cobalt powder particles. in Journal of the Serbian Chemical Society. 2015;80(2):197-207.
doi:10.2298/JSC200814104M .
Maksimović, Vesna, Nikolić, Nebojša D., Kusigerski, Vladan, Blanuša, Jovan, "Correlation between morphology and magnetic properties of electrochemically produced cobalt powder particles" in Journal of the Serbian Chemical Society, 80, no. 2 (2015):197-207,
https://doi.org/10.2298/JSC200814104M . .
1
14
15
19

Effects of sintering on the structural, micro structural and magnetic properties of nanoparticle manganite Ca1-xGdxMnO3 (x=0.05, 0.1, 0.15, 0.2)

Rosić, Milena; Kljaljevic, Ljiljana; Jordanov, Dragana; Stoiljković, Milovan; Kusigerski, Vladan; Spasojević, Vojislav; Matović, Branko

(2015)

TY  - JOUR
AU  - Rosić, Milena
AU  - Kljaljevic, Ljiljana
AU  - Jordanov, Dragana
AU  - Stoiljković, Milovan
AU  - Kusigerski, Vladan
AU  - Spasojević, Vojislav
AU  - Matović, Branko
PY  - 2015
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/772
AB  - Nanocrystalline manganites Ca1-xGdxMnO3 (x=0.05, 0.1, 0.15, and 0.2) were synthesized by a modified glycine-nitrate procedure and subjected to a systematic investigation regarding the effects of calcination and sintering on their structural, microstructural and magnetic properties. Thermal treatments of the green bodies were carried out by the conventional sintering (CS) method and the effects were monitored by different experimental techniques (XRD, ICP, FTIR, SEM, and EDS). The obtained results showed that induced structural/microstructural changes were not simple functions of the dopant concentration x and that they were influenced by different material-specific processes. Magnetism of the final bulk powders have been investigated by SQUID-magnetometry and correlated with samples composition and structural/microstructural properties. (C) 2015 Elsevier Ltd and Techna Group S.r.l. All rights reserved.
T2  - Ceramics International
T1  - Effects of sintering on the structural, micro structural and magnetic properties of nanoparticle manganite Ca1-xGdxMnO3 (x=0.05, 0.1, 0.15, 0.2)
VL  - 41
IS  - 10
SP  - 14964
EP  - 14972
DO  - 10.1016/j.ceramint.2015.08.041
ER  - 
@article{
author = "Rosić, Milena and Kljaljevic, Ljiljana and Jordanov, Dragana and Stoiljković, Milovan and Kusigerski, Vladan and Spasojević, Vojislav and Matović, Branko",
year = "2015",
abstract = "Nanocrystalline manganites Ca1-xGdxMnO3 (x=0.05, 0.1, 0.15, and 0.2) were synthesized by a modified glycine-nitrate procedure and subjected to a systematic investigation regarding the effects of calcination and sintering on their structural, microstructural and magnetic properties. Thermal treatments of the green bodies were carried out by the conventional sintering (CS) method and the effects were monitored by different experimental techniques (XRD, ICP, FTIR, SEM, and EDS). The obtained results showed that induced structural/microstructural changes were not simple functions of the dopant concentration x and that they were influenced by different material-specific processes. Magnetism of the final bulk powders have been investigated by SQUID-magnetometry and correlated with samples composition and structural/microstructural properties. (C) 2015 Elsevier Ltd and Techna Group S.r.l. All rights reserved.",
journal = "Ceramics International",
title = "Effects of sintering on the structural, micro structural and magnetic properties of nanoparticle manganite Ca1-xGdxMnO3 (x=0.05, 0.1, 0.15, 0.2)",
volume = "41",
number = "10",
pages = "14964-14972",
doi = "10.1016/j.ceramint.2015.08.041"
}
Rosić, M., Kljaljevic, L., Jordanov, D., Stoiljković, M., Kusigerski, V., Spasojević, V.,& Matović, B.. (2015). Effects of sintering on the structural, micro structural and magnetic properties of nanoparticle manganite Ca1-xGdxMnO3 (x=0.05, 0.1, 0.15, 0.2). in Ceramics International, 41(10), 14964-14972.
https://doi.org/10.1016/j.ceramint.2015.08.041
Rosić M, Kljaljevic L, Jordanov D, Stoiljković M, Kusigerski V, Spasojević V, Matović B. Effects of sintering on the structural, micro structural and magnetic properties of nanoparticle manganite Ca1-xGdxMnO3 (x=0.05, 0.1, 0.15, 0.2). in Ceramics International. 2015;41(10):14964-14972.
doi:10.1016/j.ceramint.2015.08.041 .
Rosić, Milena, Kljaljevic, Ljiljana, Jordanov, Dragana, Stoiljković, Milovan, Kusigerski, Vladan, Spasojević, Vojislav, Matović, Branko, "Effects of sintering on the structural, micro structural and magnetic properties of nanoparticle manganite Ca1-xGdxMnO3 (x=0.05, 0.1, 0.15, 0.2)" in Ceramics International, 41, no. 10 (2015):14964-14972,
https://doi.org/10.1016/j.ceramint.2015.08.041 . .
14
10
14

Magnetic Properties and Mossbauer spectroscopy of NdFe(1-x)MnxO(3)

Lazurova, J.; Mihalik, M.; Mihalik, Jr., M.; Vavra, M.; Zentkova, M.; Briancin, J.; Perović, Marija M.; Kusigerski, Vladan; Schneeweiss, Oldřich B.; Roupcova, P.; Kamenev, K. V.; Misek, M.; Jagličić, Zvonko

(2015)

TY  - CONF
AU  - Lazurova, J.
AU  - Mihalik, M.
AU  - Mihalik, Jr., M.
AU  - Vavra, M.
AU  - Zentkova, M.
AU  - Briancin, J.
AU  - Perović, Marija M.
AU  - Kusigerski, Vladan
AU  - Schneeweiss, Oldřich B.
AU  - Roupcova, P.
AU  - Kamenev, K. V.
AU  - Misek, M.
AU  - Jagličić, Zvonko
PY  - 2015
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/7067
AB  - The effect of particle reduction to nanoscale size and substitution of Mn3+ ions for Fe3+ ions on the crystal structure, lattice dynamics, Mossbauer spectra and magnetic properties in NdFe(1-x)MnxO(3) compounds have been studied. X-ray powder diffraction and Raman spectroscopy revealed that the Jahn-Teller distortion of lattice dominates for samples with x GT 0.4. The average particle size of NdFeO3 nanoparticles (NAP) increases with annealing at 600 degrees C from about 15 nm to 25 nm. The presence of superparamagnetic particles was indicated by Mossbauer measurements in NdFeO3 NAP system. Sextets in NdFe(1-x)MnxO(3) Mssbauer spectra can be modelled with several local environments of Fe3+ induced by substitution. The reduction of dimensionality and the substitution induce a decrease of the Neel temperature T-Nl from 691 K to 544 K for NAP or to 356 K for x = 0.4, however the temperature of spin reorientation T-SR increases with substitution. The saturated magnetization obtained at 1.9 K increases and ferromagnetic component is removed below T-SR with the substitution.
C3  - Journal of Physics: Conference Series
T1  - Magnetic Properties and Mossbauer spectroscopy of NdFe(1-x)MnxO(3)
VL  - 592
DO  - 10.1088/1742-6596/592/1/012117
ER  - 
@conference{
author = "Lazurova, J. and Mihalik, M. and Mihalik, Jr., M. and Vavra, M. and Zentkova, M. and Briancin, J. and Perović, Marija M. and Kusigerski, Vladan and Schneeweiss, Oldřich B. and Roupcova, P. and Kamenev, K. V. and Misek, M. and Jagličić, Zvonko",
year = "2015",
abstract = "The effect of particle reduction to nanoscale size and substitution of Mn3+ ions for Fe3+ ions on the crystal structure, lattice dynamics, Mossbauer spectra and magnetic properties in NdFe(1-x)MnxO(3) compounds have been studied. X-ray powder diffraction and Raman spectroscopy revealed that the Jahn-Teller distortion of lattice dominates for samples with x GT 0.4. The average particle size of NdFeO3 nanoparticles (NAP) increases with annealing at 600 degrees C from about 15 nm to 25 nm. The presence of superparamagnetic particles was indicated by Mossbauer measurements in NdFeO3 NAP system. Sextets in NdFe(1-x)MnxO(3) Mssbauer spectra can be modelled with several local environments of Fe3+ induced by substitution. The reduction of dimensionality and the substitution induce a decrease of the Neel temperature T-Nl from 691 K to 544 K for NAP or to 356 K for x = 0.4, however the temperature of spin reorientation T-SR increases with substitution. The saturated magnetization obtained at 1.9 K increases and ferromagnetic component is removed below T-SR with the substitution.",
journal = "Journal of Physics: Conference Series",
title = "Magnetic Properties and Mossbauer spectroscopy of NdFe(1-x)MnxO(3)",
volume = "592",
doi = "10.1088/1742-6596/592/1/012117"
}
Lazurova, J., Mihalik, M., Mihalik, Jr., M., Vavra, M., Zentkova, M., Briancin, J., Perović, M. M., Kusigerski, V., Schneeweiss, O. B., Roupcova, P., Kamenev, K. V., Misek, M.,& Jagličić, Z.. (2015). Magnetic Properties and Mossbauer spectroscopy of NdFe(1-x)MnxO(3). in Journal of Physics: Conference Series, 592.
https://doi.org/10.1088/1742-6596/592/1/012117
Lazurova J, Mihalik M, Mihalik JM, Vavra M, Zentkova M, Briancin J, Perović MM, Kusigerski V, Schneeweiss OB, Roupcova P, Kamenev KV, Misek M, Jagličić Z. Magnetic Properties and Mossbauer spectroscopy of NdFe(1-x)MnxO(3). in Journal of Physics: Conference Series. 2015;592.
doi:10.1088/1742-6596/592/1/012117 .
Lazurova, J., Mihalik, M., Mihalik, Jr., M., Vavra, M., Zentkova, M., Briancin, J., Perović, Marija M., Kusigerski, Vladan, Schneeweiss, Oldřich B., Roupcova, P., Kamenev, K. V., Misek, M., Jagličić, Zvonko, "Magnetic Properties and Mossbauer spectroscopy of NdFe(1-x)MnxO(3)" in Journal of Physics: Conference Series, 592 (2015),
https://doi.org/10.1088/1742-6596/592/1/012117 . .
12
11
13

Crystal structure and magnetic properties of Y-2(Cu1-xMgx)(2)O-5 obtained by SHS method

Gebrel, Z.; Blanuša, Jovan; Kusigerski, Vladan; Spasojević, Vojislav; Mraković, Ana Đ.; Perović, Marija M.; Alqat, A.

(2014)

TY  - JOUR
AU  - Gebrel, Z.
AU  - Blanuša, Jovan
AU  - Kusigerski, Vladan
AU  - Spasojević, Vojislav
AU  - Mraković, Ana Đ.
AU  - Perović, Marija M.
AU  - Alqat, A.
PY  - 2014
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/5714
AB  - The single-phase polycrystalline samples of Y-2(Cu1-xMgx)(2)O-5, x = 0.0, 0.05, 0.15 were successfully synthesized by a modified self-propagating high temperature synthesis. Effects of Mg+2 substitution for Cu+2 in metamagnetic Y2Cu2O5 on its crystal structure and magnetic properties have been analyzed by X-ray diffraction and magnetic measurements performed within 2-300 K range. Mg doping was found to introduce small distortions in the main intradimmer superexchange paths so that ferromagnetic correlations decrease with Mg concentration. More significant impact of Cu substitution was found on the low temperature magnetism due to the breaking of infinite Cu-O chains. The formation of finite size chains introduces low temperature paramagnetic contribution and reduction in Neel temperature. Overall results give a strong indication that the antiferromagnetic ordering as well as metamagnetism persists up to the 15% of the Mg concentration. (C) 2013 Elsevier B.V. All rights reserved.
T2  - Journal of Alloys and Compounds
T1  - Crystal structure and magnetic properties of Y-2(Cu1-xMgx)(2)O-5 obtained by SHS method
VL  - 582
SP  - 186
EP  - 189
DO  - 10.1016/j.jallcom.2013.08.033
ER  - 
@article{
author = "Gebrel, Z. and Blanuša, Jovan and Kusigerski, Vladan and Spasojević, Vojislav and Mraković, Ana Đ. and Perović, Marija M. and Alqat, A.",
year = "2014",
abstract = "The single-phase polycrystalline samples of Y-2(Cu1-xMgx)(2)O-5, x = 0.0, 0.05, 0.15 were successfully synthesized by a modified self-propagating high temperature synthesis. Effects of Mg+2 substitution for Cu+2 in metamagnetic Y2Cu2O5 on its crystal structure and magnetic properties have been analyzed by X-ray diffraction and magnetic measurements performed within 2-300 K range. Mg doping was found to introduce small distortions in the main intradimmer superexchange paths so that ferromagnetic correlations decrease with Mg concentration. More significant impact of Cu substitution was found on the low temperature magnetism due to the breaking of infinite Cu-O chains. The formation of finite size chains introduces low temperature paramagnetic contribution and reduction in Neel temperature. Overall results give a strong indication that the antiferromagnetic ordering as well as metamagnetism persists up to the 15% of the Mg concentration. (C) 2013 Elsevier B.V. All rights reserved.",
journal = "Journal of Alloys and Compounds",
title = "Crystal structure and magnetic properties of Y-2(Cu1-xMgx)(2)O-5 obtained by SHS method",
volume = "582",
pages = "186-189",
doi = "10.1016/j.jallcom.2013.08.033"
}
Gebrel, Z., Blanuša, J., Kusigerski, V., Spasojević, V., Mraković, A. Đ., Perović, M. M.,& Alqat, A.. (2014). Crystal structure and magnetic properties of Y-2(Cu1-xMgx)(2)O-5 obtained by SHS method. in Journal of Alloys and Compounds, 582, 186-189.
https://doi.org/10.1016/j.jallcom.2013.08.033
Gebrel Z, Blanuša J, Kusigerski V, Spasojević V, Mraković AĐ, Perović MM, Alqat A. Crystal structure and magnetic properties of Y-2(Cu1-xMgx)(2)O-5 obtained by SHS method. in Journal of Alloys and Compounds. 2014;582:186-189.
doi:10.1016/j.jallcom.2013.08.033 .
Gebrel, Z., Blanuša, Jovan, Kusigerski, Vladan, Spasojević, Vojislav, Mraković, Ana Đ., Perović, Marija M., Alqat, A., "Crystal structure and magnetic properties of Y-2(Cu1-xMgx)(2)O-5 obtained by SHS method" in Journal of Alloys and Compounds, 582 (2014):186-189,
https://doi.org/10.1016/j.jallcom.2013.08.033 . .

Magnetic Properties of NdFe0.9Mn0.1O3

Zentkova, M.; Lazurova, J.; Kovač, Janez; Mihalik, M.; Mihalik, Jr., M.; Briancin, J.; Fitta, M.; Kusigerski, Vladan

(2014)

TY  - JOUR
AU  - Zentkova, M.
AU  - Lazurova, J.
AU  - Kovač, Janez
AU  - Mihalik, M.
AU  - Mihalik, Jr., M.
AU  - Briancin, J.
AU  - Fitta, M.
AU  - Kusigerski, Vladan
PY  - 2014
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/7034
AB  - In our paper we study effect of Mn for Fe substitution on magnetic properties of NdFex-1MnxO3 compounds for x = 0 and 0.1, which have been grown by the OFZ technique. The Neel temperature decreases from T-N1 = 691 K to T-N1 = 621 K, and the anomaly in AC susceptibility, related to spin reorientation, vanishes with Mn substitution. Low temperature heat capacity measurement for sample with x = 0.1 revealed that substitution of Mn for Fe shifts a Schottky-type anomaly at T-sh to higher temperatures. Another anomaly is generated by doping at T-max = 11 K. The anomaly is smeared out by magnetic field, confirming its magnetic origin.
T2  - Acta Physica Polonica A
T1  - Magnetic Properties of NdFe0.9Mn0.1O3
VL  - 126
IS  - 1
SP  - 306
EP  - 307
DO  - 10.12693/APhysPolA.126.306
ER  - 
@article{
author = "Zentkova, M. and Lazurova, J. and Kovač, Janez and Mihalik, M. and Mihalik, Jr., M. and Briancin, J. and Fitta, M. and Kusigerski, Vladan",
year = "2014",
abstract = "In our paper we study effect of Mn for Fe substitution on magnetic properties of NdFex-1MnxO3 compounds for x = 0 and 0.1, which have been grown by the OFZ technique. The Neel temperature decreases from T-N1 = 691 K to T-N1 = 621 K, and the anomaly in AC susceptibility, related to spin reorientation, vanishes with Mn substitution. Low temperature heat capacity measurement for sample with x = 0.1 revealed that substitution of Mn for Fe shifts a Schottky-type anomaly at T-sh to higher temperatures. Another anomaly is generated by doping at T-max = 11 K. The anomaly is smeared out by magnetic field, confirming its magnetic origin.",
journal = "Acta Physica Polonica A",
title = "Magnetic Properties of NdFe0.9Mn0.1O3",
volume = "126",
number = "1",
pages = "306-307",
doi = "10.12693/APhysPolA.126.306"
}
Zentkova, M., Lazurova, J., Kovač, J., Mihalik, M., Mihalik, Jr., M., Briancin, J., Fitta, M.,& Kusigerski, V.. (2014). Magnetic Properties of NdFe0.9Mn0.1O3. in Acta Physica Polonica A, 126(1), 306-307.
https://doi.org/10.12693/APhysPolA.126.306
Zentkova M, Lazurova J, Kovač J, Mihalik M, Mihalik JM, Briancin J, Fitta M, Kusigerski V. Magnetic Properties of NdFe0.9Mn0.1O3. in Acta Physica Polonica A. 2014;126(1):306-307.
doi:10.12693/APhysPolA.126.306 .
Zentkova, M., Lazurova, J., Kovač, Janez, Mihalik, M., Mihalik, Jr., M., Briancin, J., Fitta, M., Kusigerski, Vladan, "Magnetic Properties of NdFe0.9Mn0.1O3" in Acta Physica Polonica A, 126, no. 1 (2014):306-307,
https://doi.org/10.12693/APhysPolA.126.306 . .
8
5
6

An ac susceptibility study of spin dynamics in a super spin glass nanoparticle La0.7Ca0.3MnO3 system: simultaneous relaxation processes

Perović, Marija M.; Kusigerski, Vladan; Spasojević, Vojislav; Mraković, Ana Đ.; Blanuša, Jovan; Zentkova, M.; Mihalik, M.

(2013)

TY  - JOUR
AU  - Perović, Marija M.
AU  - Kusigerski, Vladan
AU  - Spasojević, Vojislav
AU  - Mraković, Ana Đ.
AU  - Blanuša, Jovan
AU  - Zentkova, M.
AU  - Mihalik, M.
PY  - 2013
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/5395
AB  - In this paper, we present the results of a systematic study of nonequilibrium dynamics in a strongly interacting super spin glass (SSG) nanoparticle La0.7Ca0.3MnO3 system by alternating current (ac) susceptibility measurements. Cole-Cole analysis of the obtained data revealed the simultaneous existence of two separated relaxation processes, which can be assigned to the relaxation of different magnetic entities. Along with the expected relaxation of the collective SSG phase, the existence of individual, nonagglomerated particles, which do not take part in the collective phase and relax independently, was proposed. A full dynamical scaling analysis was performed in order to elucidate the nature of the transition to a low-temperature SSG state in the interacting La0.7Ca0.3MnO3 nanoparticle sample.
T2  - Journal of Physics. D: Applied Physics
T1  - An ac susceptibility study of spin dynamics in a super spin glass nanoparticle La0.7Ca0.3MnO3 system: simultaneous relaxation processes
VL  - 46
IS  - 16
DO  - 10.1088/0022-3727/46/16/165001
ER  - 
@article{
author = "Perović, Marija M. and Kusigerski, Vladan and Spasojević, Vojislav and Mraković, Ana Đ. and Blanuša, Jovan and Zentkova, M. and Mihalik, M.",
year = "2013",
abstract = "In this paper, we present the results of a systematic study of nonequilibrium dynamics in a strongly interacting super spin glass (SSG) nanoparticle La0.7Ca0.3MnO3 system by alternating current (ac) susceptibility measurements. Cole-Cole analysis of the obtained data revealed the simultaneous existence of two separated relaxation processes, which can be assigned to the relaxation of different magnetic entities. Along with the expected relaxation of the collective SSG phase, the existence of individual, nonagglomerated particles, which do not take part in the collective phase and relax independently, was proposed. A full dynamical scaling analysis was performed in order to elucidate the nature of the transition to a low-temperature SSG state in the interacting La0.7Ca0.3MnO3 nanoparticle sample.",
journal = "Journal of Physics. D: Applied Physics",
title = "An ac susceptibility study of spin dynamics in a super spin glass nanoparticle La0.7Ca0.3MnO3 system: simultaneous relaxation processes",
volume = "46",
number = "16",
doi = "10.1088/0022-3727/46/16/165001"
}
Perović, M. M., Kusigerski, V., Spasojević, V., Mraković, A. Đ., Blanuša, J., Zentkova, M.,& Mihalik, M.. (2013). An ac susceptibility study of spin dynamics in a super spin glass nanoparticle La0.7Ca0.3MnO3 system: simultaneous relaxation processes. in Journal of Physics. D: Applied Physics, 46(16).
https://doi.org/10.1088/0022-3727/46/16/165001
Perović MM, Kusigerski V, Spasojević V, Mraković AĐ, Blanuša J, Zentkova M, Mihalik M. An ac susceptibility study of spin dynamics in a super spin glass nanoparticle La0.7Ca0.3MnO3 system: simultaneous relaxation processes. in Journal of Physics. D: Applied Physics. 2013;46(16).
doi:10.1088/0022-3727/46/16/165001 .
Perović, Marija M., Kusigerski, Vladan, Spasojević, Vojislav, Mraković, Ana Đ., Blanuša, Jovan, Zentkova, M., Mihalik, M., "An ac susceptibility study of spin dynamics in a super spin glass nanoparticle La0.7Ca0.3MnO3 system: simultaneous relaxation processes" in Journal of Physics. D: Applied Physics, 46, no. 16 (2013),
https://doi.org/10.1088/0022-3727/46/16/165001 . .
15
12
17

Modified self-propagating high-temperature synthesis of nanosized La0.7Ca0.3MnO3

Mraković, Ana Đ.; Blanuša, Jovan; Primc, Darinka; Perović, Marija M.; Jagličić, Zvonko; Kusigerski, Vladan; Spasojević, Vojislav

(2013)

TY  - JOUR
AU  - Mraković, Ana Đ.
AU  - Blanuša, Jovan
AU  - Primc, Darinka
AU  - Perović, Marija M.
AU  - Jagličić, Zvonko
AU  - Kusigerski, Vladan
AU  - Spasojević, Vojislav
PY  - 2013
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/5463
AB  - A modified solid-state combustion route was developed for the preparation of nanocrystalline manganite La0.7Ca0.3MnO3 in a single-step process, using metal nitrates and glucose/KNO3 redox mixture. The obtained sample was found to crystallize within O type of orthorhombic perovskite structure (space group Pnma), without the presence of other structural phases or impurities. Nanoparticles are found to have particle size in the range 12-35 nm, and to be highly crystalline without the presence of amorphous surface layer. Magnetic measurements show that nanoparticles display bulk-like magnetic properties, with ferromagnetic phase transition at 125 K and the absence of superparamagnetic or spin-glass behavior. (C) 2012 Elsevier Ltd and Techna Group S.r.l. All rights reserved.
T2  - Ceramics International
T1  - Modified self-propagating high-temperature synthesis of nanosized La0.7Ca0.3MnO3
VL  - 39
IS  - 4
SP  - 3771
EP  - 3777
DO  - 10.1016/j.ceramint.2012.10.216
ER  - 
@article{
author = "Mraković, Ana Đ. and Blanuša, Jovan and Primc, Darinka and Perović, Marija M. and Jagličić, Zvonko and Kusigerski, Vladan and Spasojević, Vojislav",
year = "2013",
abstract = "A modified solid-state combustion route was developed for the preparation of nanocrystalline manganite La0.7Ca0.3MnO3 in a single-step process, using metal nitrates and glucose/KNO3 redox mixture. The obtained sample was found to crystallize within O type of orthorhombic perovskite structure (space group Pnma), without the presence of other structural phases or impurities. Nanoparticles are found to have particle size in the range 12-35 nm, and to be highly crystalline without the presence of amorphous surface layer. Magnetic measurements show that nanoparticles display bulk-like magnetic properties, with ferromagnetic phase transition at 125 K and the absence of superparamagnetic or spin-glass behavior. (C) 2012 Elsevier Ltd and Techna Group S.r.l. All rights reserved.",
journal = "Ceramics International",
title = "Modified self-propagating high-temperature synthesis of nanosized La0.7Ca0.3MnO3",
volume = "39",
number = "4",
pages = "3771-3777",
doi = "10.1016/j.ceramint.2012.10.216"
}
Mraković, A. Đ., Blanuša, J., Primc, D., Perović, M. M., Jagličić, Z., Kusigerski, V.,& Spasojević, V.. (2013). Modified self-propagating high-temperature synthesis of nanosized La0.7Ca0.3MnO3. in Ceramics International, 39(4), 3771-3777.
https://doi.org/10.1016/j.ceramint.2012.10.216
Mraković AĐ, Blanuša J, Primc D, Perović MM, Jagličić Z, Kusigerski V, Spasojević V. Modified self-propagating high-temperature synthesis of nanosized La0.7Ca0.3MnO3. in Ceramics International. 2013;39(4):3771-3777.
doi:10.1016/j.ceramint.2012.10.216 .
Mraković, Ana Đ., Blanuša, Jovan, Primc, Darinka, Perović, Marija M., Jagličić, Zvonko, Kusigerski, Vladan, Spasojević, Vojislav, "Modified self-propagating high-temperature synthesis of nanosized La0.7Ca0.3MnO3" in Ceramics International, 39, no. 4 (2013):3771-3777,
https://doi.org/10.1016/j.ceramint.2012.10.216 . .
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Combustion synthesis as a novel approach in preparation of polycrystalline Y2Cu2O5

Gebrel, Z.; Blanuša, Jovan; Spasojević, Vojislav; Kusigerski, Vladan; Mraković, Ana Đ.; Alqat, A.; Perović, Marija M.

(2013)

TY  - JOUR
AU  - Gebrel, Z.
AU  - Blanuša, Jovan
AU  - Spasojević, Vojislav
AU  - Kusigerski, Vladan
AU  - Mraković, Ana Đ.
AU  - Alqat, A.
AU  - Perović, Marija M.
PY  - 2013
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/5515
AB  - Polycrystalline samples of Y2Cu2O5 were for the first time sintered from precursors obtained by two combustion routes - the glycine-nitrate method (sample S1) and a modified self-propagating high-temperature synthesis (sample S2). The detailed X-ray diffraction analysis has confirmed that both samples are well crystallized and single phase, with the high crystallization degree and cation ordering within a Cu sublattice. Magnetic characterization has shown magnetic behavior typical of pure Y2Cu2O5. The distinctive advantages of these new synthesis routes in comparison to the ceramic sintering are in simplification of the overall procedure as well as in a significant reduction of synthesis duration from several days down to 31 h (S1) or 12 h (S2). (C) 2013 Elsevier B.V. All rights reserved.
T2  - Journal of Alloys and Compounds
T1  - Combustion synthesis as a novel approach in preparation of polycrystalline Y2Cu2O5
VL  - 568
SP  - 55
EP  - 59
DO  - 10.1016/j.jallcom.2013.03.133
ER  - 
@article{
author = "Gebrel, Z. and Blanuša, Jovan and Spasojević, Vojislav and Kusigerski, Vladan and Mraković, Ana Đ. and Alqat, A. and Perović, Marija M.",
year = "2013",
abstract = "Polycrystalline samples of Y2Cu2O5 were for the first time sintered from precursors obtained by two combustion routes - the glycine-nitrate method (sample S1) and a modified self-propagating high-temperature synthesis (sample S2). The detailed X-ray diffraction analysis has confirmed that both samples are well crystallized and single phase, with the high crystallization degree and cation ordering within a Cu sublattice. Magnetic characterization has shown magnetic behavior typical of pure Y2Cu2O5. The distinctive advantages of these new synthesis routes in comparison to the ceramic sintering are in simplification of the overall procedure as well as in a significant reduction of synthesis duration from several days down to 31 h (S1) or 12 h (S2). (C) 2013 Elsevier B.V. All rights reserved.",
journal = "Journal of Alloys and Compounds",
title = "Combustion synthesis as a novel approach in preparation of polycrystalline Y2Cu2O5",
volume = "568",
pages = "55-59",
doi = "10.1016/j.jallcom.2013.03.133"
}
Gebrel, Z., Blanuša, J., Spasojević, V., Kusigerski, V., Mraković, A. Đ., Alqat, A.,& Perović, M. M.. (2013). Combustion synthesis as a novel approach in preparation of polycrystalline Y2Cu2O5. in Journal of Alloys and Compounds, 568, 55-59.
https://doi.org/10.1016/j.jallcom.2013.03.133
Gebrel Z, Blanuša J, Spasojević V, Kusigerski V, Mraković AĐ, Alqat A, Perović MM. Combustion synthesis as a novel approach in preparation of polycrystalline Y2Cu2O5. in Journal of Alloys and Compounds. 2013;568:55-59.
doi:10.1016/j.jallcom.2013.03.133 .
Gebrel, Z., Blanuša, Jovan, Spasojević, Vojislav, Kusigerski, Vladan, Mraković, Ana Đ., Alqat, A., Perović, Marija M., "Combustion synthesis as a novel approach in preparation of polycrystalline Y2Cu2O5" in Journal of Alloys and Compounds, 568 (2013):55-59,
https://doi.org/10.1016/j.jallcom.2013.03.133 . .
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