TY  - JOUR
AU  - Maletić, Marina
AU  - Kalijadis, Ana
AU  - Lazović, Vladimir
AU  - Trifunović, Snežana
AU  - Babić, Biljana M.
AU  - Dapčević, Aleksandra
AU  - Kovač, Janez
AU  - Vukčević, Marija
PY  - 2023
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/10693
AB  - N-doped TiO2/carbon composites (TiO2/CN) with different nitrogen content, were obtained starting from titanium isopropoxide and glucose, and by varying the amount of melamine, added to starting reaction mixture. For comparison, an undoped sample (TiO2/C) was also prepared. Structural and surface characteristics were determined through scanning electron microscopy, thermogravimetric analysis, elemental analysis, Fourier transform infrared spectroscopy, X-ray photoelectron spectroscopy, X-ray diffraction and nitrogen adsorption–desorption isotherms. The photocatalytic activity of TiO2/CN composites was examined via photocatalytic degradation of methylene blue and multiclass pharmaceuticals from water solution. It was found that N doping of TiO2/carbon composites induced changes in structural and surface characteristics of TiO2/CN composites, improving their adsorption, but decreasing photocatalytic efficiency. Nevertheless, TiO2/CN0.05 composite obtained by the hydrothermal synthesis in the presence of glucose and 0.05 g melamine showed the highest efficiency for removing selected pharmaceuticals and methylene blue from aqueous solutions through the combined processes of adsorption in the dark, and photocatalytic degradation under UV and visible irradiation.
T2  - Journal of the Serbian Chemical Society
T1  - Influence of N doping on structural and photocatalytic properties of hydrothermally synthesized TiO2/carbon composites
VL  - 88
IS  - 2
SP  - 183
EP  - 197
DO  - 10.2298/JSC220608079M
ER  - 

@article{
author = "Maletić, Marina and Kalijadis, Ana and Lazović, Vladimir and Trifunović, Snežana and Babić, Biljana M. and Dapčević, Aleksandra and Kovač, Janez and Vukčević, Marija",
year = "2023",
abstract = "N-doped TiO2/carbon composites (TiO2/CN) with different nitrogen content, were obtained starting from titanium isopropoxide and glucose, and by varying the amount of melamine, added to starting reaction mixture. For comparison, an undoped sample (TiO2/C) was also prepared. Structural and surface characteristics were determined through scanning electron microscopy, thermogravimetric analysis, elemental analysis, Fourier transform infrared spectroscopy, X-ray photoelectron spectroscopy, X-ray diffraction and nitrogen adsorption–desorption isotherms. The photocatalytic activity of TiO2/CN composites was examined via photocatalytic degradation of methylene blue and multiclass pharmaceuticals from water solution. It was found that N doping of TiO2/carbon composites induced changes in structural and surface characteristics of TiO2/CN composites, improving their adsorption, but decreasing photocatalytic efficiency. Nevertheless, TiO2/CN0.05 composite obtained by the hydrothermal synthesis in the presence of glucose and 0.05 g melamine showed the highest efficiency for removing selected pharmaceuticals and methylene blue from aqueous solutions through the combined processes of adsorption in the dark, and photocatalytic degradation under UV and visible irradiation.",
journal = "Journal of the Serbian Chemical Society",
title = "Influence of N doping on structural and photocatalytic properties of hydrothermally synthesized TiO2/carbon composites",
volume = "88",
number = "2",
pages = "183-197",
doi = "10.2298/JSC220608079M"
}

Maletić, M., Kalijadis, A., Lazović, V., Trifunović, S., Babić, B. M., Dapčević, A., Kovač, J.,& Vukčević, M.. (2023). Influence of N doping on structural and photocatalytic properties of hydrothermally synthesized TiO2/carbon composites. in Journal of the Serbian Chemical Society, 88(2), 183-197.
https://doi.org/10.2298/JSC220608079M

Maletić M, Kalijadis A, Lazović V, Trifunović S, Babić BM, Dapčević A, Kovač J, Vukčević M. Influence of N doping on structural and photocatalytic properties of hydrothermally synthesized TiO2/carbon composites. in Journal of the Serbian Chemical Society. 2023;88(2):183-197.
doi:10.2298/JSC220608079M .

Maletić, Marina, Kalijadis, Ana, Lazović, Vladimir, Trifunović, Snežana, Babić, Biljana M., Dapčević, Aleksandra, Kovač, Janez, Vukčević, Marija, "Influence of N doping on structural and photocatalytic properties of hydrothermally synthesized TiO2/carbon composites" in Journal of the Serbian Chemical Society, 88, no. 2 (2023):183-197,
https://doi.org/10.2298/JSC220608079M . .

TY  - JOUR
AU  - Kalijadis, Ana
AU  - Maletić, Marina M.
AU  - Bjelajac, Anđelika Z.
AU  - Babić, Biljana M.
AU  - Minović-Arsić, Tamara
AU  - Vukčević, Marija M.
PY  - 2022
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/10339
AB  - In this study, the influence of boron doping on structural and surface properties of carbon material synthesized by a hydrothermal method was investigated, and the obtained results were compared with the previously published influence that boron has on characteristics of carbonized boron-doped hydrothermal carbons (CHTCB). Hydrothermal carbons doped with boron (HTCB) were obtained by the hydrothermal synthesis of glucose solutions with different nominal concentrations of boric acid. It was found that glucose based hydrothermal carbon does not have developed porosity, and the presence of boron in their structure has insignificant influence on it. On the contrary, additional carbonization increases the specific surface area of the undoped sample, while an increase in boron content drastically decreases the specific surface area. Boron doping leads to a decrease in the amount of surface oxygen groups, for both, hydrothermally synthesized and additionally carbonized materials. Raman analysis showed that the boron content does not affect a structural arrangement of the HTCB samples, and Raman structural parameters show a higher degree of disorder, compared to the CHTCB samples. Comparison of structural and surface characteristics of hydrothermal carbons and carbonized materials contributes to the study of the so far, insufficiently clarified influence that boron incorporation has on the material characteristics. © 2022 Serbian Chemical Society. All rights reserved.
T2  - Journal of the Serbian Chemical Society
T1  - Influence of boron doping on characteristics of glucose-based hydrothermal carbons
VL  - 87
IS  - 6
SP  - 749
EP  - 760
DO  - 10.2298/JSC211011001K
ER  - 

@article{
author = "Kalijadis, Ana and Maletić, Marina M. and Bjelajac, Anđelika Z. and Babić, Biljana M. and Minović-Arsić, Tamara and Vukčević, Marija M.",
year = "2022",
abstract = "In this study, the influence of boron doping on structural and surface properties of carbon material synthesized by a hydrothermal method was investigated, and the obtained results were compared with the previously published influence that boron has on characteristics of carbonized boron-doped hydrothermal carbons (CHTCB). Hydrothermal carbons doped with boron (HTCB) were obtained by the hydrothermal synthesis of glucose solutions with different nominal concentrations of boric acid. It was found that glucose based hydrothermal carbon does not have developed porosity, and the presence of boron in their structure has insignificant influence on it. On the contrary, additional carbonization increases the specific surface area of the undoped sample, while an increase in boron content drastically decreases the specific surface area. Boron doping leads to a decrease in the amount of surface oxygen groups, for both, hydrothermally synthesized and additionally carbonized materials. Raman analysis showed that the boron content does not affect a structural arrangement of the HTCB samples, and Raman structural parameters show a higher degree of disorder, compared to the CHTCB samples. Comparison of structural and surface characteristics of hydrothermal carbons and carbonized materials contributes to the study of the so far, insufficiently clarified influence that boron incorporation has on the material characteristics. © 2022 Serbian Chemical Society. All rights reserved.",
journal = "Journal of the Serbian Chemical Society",
title = "Influence of boron doping on characteristics of glucose-based hydrothermal carbons",
volume = "87",
number = "6",
pages = "749-760",
doi = "10.2298/JSC211011001K"
}

Kalijadis, A., Maletić, M. M., Bjelajac, A. Z., Babić, B. M., Minović-Arsić, T.,& Vukčević, M. M.. (2022). Influence of boron doping on characteristics of glucose-based hydrothermal carbons. in Journal of the Serbian Chemical Society, 87(6), 749-760.
https://doi.org/10.2298/JSC211011001K

Kalijadis A, Maletić MM, Bjelajac AZ, Babić BM, Minović-Arsić T, Vukčević MM. Influence of boron doping on characteristics of glucose-based hydrothermal carbons. in Journal of the Serbian Chemical Society. 2022;87(6):749-760.
doi:10.2298/JSC211011001K .

Kalijadis, Ana, Maletić, Marina M., Bjelajac, Anđelika Z., Babić, Biljana M., Minović-Arsić, Tamara, Vukčević, Marija M., "Influence of boron doping on characteristics of glucose-based hydrothermal carbons" in Journal of the Serbian Chemical Society, 87, no. 6 (2022):749-760,
https://doi.org/10.2298/JSC211011001K . .