Perović, Marija M.

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Authority KeyName Variants
orcid::0000-0002-0088-7612
  • Perović, Marija M. (30)
Projects
Magnetic and radionuclide labeled nanostructured materials for medical applications Croatian Science Foundation [IP-2016-06-8254]
Strukturne i magnetne osobine nanočestičnih i polikristalnih oksida retkih zemalja i 3d metala. SK-SRB-18-0066
21-58-53046 Bilateral Croatian-Chinese scientific project “Iron oxide nanostructures for environmental and energy applications”
bilateral Croatian-Chinese scientific project "Synthesis and characterization of iron oxide nanoparticles and nanofibers and their application in environmental catalysis" bilateral Croatian-Serbian [IP-2016-06-8254]
Bilateral Croatian-Serbian scientific project bilateral Croatian-Serbian scientific project " Nanostructured iron oxides for environmental applications"
Bilateral Croatian-Serbian scientific project “Nanostructured iron oxides for environmental applications” Bilateral Serbia-Slovenia [06-00-118/2018-09/32/02]
Bilateral Serbia-Slovenia [BI-RS/18-19-031] Bilateral Serbia-Slovenia projects (projects No. 451-03-38/2016-09/26 and 06-00-118/2018-09/32/02)
CENN Nanocenter for the use of Transmission Electron Microscope Jeol [JEM-2100] COST Action TD1402-RADIOMAG
Croatian Centre of Excellence for Advanced Materials and Sensing Devices Croatian Science Foundation [IP-2016-06-825]
Croatian Science Foundation (IP-2016-06-8254) ERDF EU [VEGA02/0132/16, ITMS26220120047, SKSRB-2013-0050]
Hungarian Academy of Sciences [LP2013-59 - ‘Lendület’ (Momentum) Program] Strengthening of the MagBioVin Research and Innovation Team for Development of Novel Approaches for Tumour Therapy based on Nanostructured Materials
Nanostructured Functional and Composite Materials in Catalytic and Sorption Processes ITMS: 26220220186
MAD Sk-Pl Ministry of Education, Science and Technological Development of the Republic of Serbia
Ministry of Science and Education of the Republic of Croatia Ministry of Science and Environmental Protection of Serbia [141027]
Ministry of Science and Technology of the People's Republic of China (bilateral Croatian-Serbian and Croatian-Chinese scientific projects) National Research, Development and Innovation Fund [NKFIH FK 124460]

Author's Bibliography

Magnetocaloric effect in La0.70Ag0.25MnO3+δ magnetic nanoparticles

Zentková, M.; Kovalik, M.; Mihalik, M.; Csach, K.; Gamzatov, A.G.; Aliev, A.M.; Iľkovič, S.; Fitta, M.; Perović, Marija M.; Mihalik, M.

(2022)

TY  - JOUR
AU  - Zentková, M.
AU  - Kovalik, M.
AU  - Mihalik, M.
AU  - Csach, K.
AU  - Gamzatov, A.G.
AU  - Aliev, A.M.
AU  - Iľkovič, S.
AU  - Fitta, M.
AU  - Perović, Marija M.
AU  - Mihalik, M.
PY  - 2022
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/10129
AB  - Experimental study of magnetocaloric effect (MCE) was performed by direct and indirect methods on La0.70Ag0.25MnO3+δ nanoparticles with rhombohedral LaAlO3 – type crystal structure (R3¯c space group – No. 167, hP30). The content of oxygen was modified by annealing at 800 °C/48h in different atmosphere (air, O2 and Ar). The Curie temperature TC increases from 250 K to 319.5 K and to 322.9 K with the content of oxygen. The adiabatic temperature change ΔT(4T) = 1.52 K, the change of magnetic entropy −ΔSmax(4T) = 3.96 Jkg−1K−1 and the relative cooling power RCT(4T) = 172 J/kg are maximal for sample treated in Ar and decrease with oxygen content. The frequency dependence of ΔT (f) and the shape of maximum in ΔT (T) and −ΔSmax (T) indicate relaxation processes and presence of magnetic inhomogeneities which are present mostly in sample treated in Ar. The samples demonstrate the stability of the MCE up to 1000 cycles of switching on and off the magnetic field without any signs of degradation
T2  - Journal of Magnetism and Magnetic Materials
T1  - Magnetocaloric effect in La0.70Ag0.25MnO3+δ magnetic nanoparticles
VL  - 549
SP  - 169002
DO  - 10.1016/j.jmmm.2021.169002
ER  - 
@article{
author = "Zentková, M. and Kovalik, M. and Mihalik, M. and Csach, K. and Gamzatov, A.G. and Aliev, A.M. and Iľkovič, S. and Fitta, M. and Perović, Marija M. and Mihalik, M.",
year = "2022",
abstract = "Experimental study of magnetocaloric effect (MCE) was performed by direct and indirect methods on La0.70Ag0.25MnO3+δ nanoparticles with rhombohedral LaAlO3 – type crystal structure (R3¯c space group – No. 167, hP30). The content of oxygen was modified by annealing at 800 °C/48h in different atmosphere (air, O2 and Ar). The Curie temperature TC increases from 250 K to 319.5 K and to 322.9 K with the content of oxygen. The adiabatic temperature change ΔT(4T) = 1.52 K, the change of magnetic entropy −ΔSmax(4T) = 3.96 Jkg−1K−1 and the relative cooling power RCT(4T) = 172 J/kg are maximal for sample treated in Ar and decrease with oxygen content. The frequency dependence of ΔT (f) and the shape of maximum in ΔT (T) and −ΔSmax (T) indicate relaxation processes and presence of magnetic inhomogeneities which are present mostly in sample treated in Ar. The samples demonstrate the stability of the MCE up to 1000 cycles of switching on and off the magnetic field without any signs of degradation",
journal = "Journal of Magnetism and Magnetic Materials",
title = "Magnetocaloric effect in La0.70Ag0.25MnO3+δ magnetic nanoparticles",
volume = "549",
pages = "169002",
doi = "10.1016/j.jmmm.2021.169002"
}
Zentková, M., Kovalik, M., Mihalik, M., Csach, K., Gamzatov, A.G., Aliev, A.M., Iľkovič, S., Fitta, M., Perović, M. M.,& Mihalik, M.. (2022). Magnetocaloric effect in La0.70Ag0.25MnO3+δ magnetic nanoparticles. in Journal of Magnetism and Magnetic Materials, 549, 169002.
https://doi.org/10.1016/j.jmmm.2021.169002
Zentková M, Kovalik M, Mihalik M, Csach K, Gamzatov A, Aliev A, Iľkovič S, Fitta M, Perović MM, Mihalik M. Magnetocaloric effect in La0.70Ag0.25MnO3+δ magnetic nanoparticles. in Journal of Magnetism and Magnetic Materials. 2022;549:169002.
doi:10.1016/j.jmmm.2021.169002 .
Zentková, M., Kovalik, M., Mihalik, M., Csach, K., Gamzatov, A.G., Aliev, A.M., Iľkovič, S., Fitta, M., Perović, Marija M., Mihalik, M., "Magnetocaloric effect in La0.70Ag0.25MnO3+δ magnetic nanoparticles" in Journal of Magnetism and Magnetic Materials, 549 (2022):169002,
https://doi.org/10.1016/j.jmmm.2021.169002 . .
1

Influence of Sn doping on the structural, magnetic, optical and photocatalytic properties of hematite (α-Fe2O3) nanoparticles

Popov, Nina; Ristić, Mira; Bošković, Marko; Perović, Marija M.; Musić, Svetozar; Stanković, Dalibor M.; Krehula, Stjepko

(2022)

TY  - JOUR
AU  - Popov, Nina
AU  - Ristić, Mira
AU  - Bošković, Marko
AU  - Perović, Marija M.
AU  - Musić, Svetozar
AU  - Stanković, Dalibor M.
AU  - Krehula, Stjepko
PY  - 2022
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/9929
AB  - Sn-doped hematite (α-Fe2O3) nanoparticles of fairly uniform and Sn-dependent size and shape were synthesized via a simple combination of hydrothermal co-precipitation and calcination. The effects of Sn doping on the unit cell size, crystallinity, particle size and shape, as well as the magnetic, optical and photocatalytic properties of hematite nanoparticles were analyzed. The incorporation of Sn4+ ions into the crystal structure of hematite was confirmed by determination of the unit cell expansion due to the replacement of octahedrally coordinated Fe3+ ions by significantly larger Sn4+ ions, as well as a substantially reduced hyperfine magnetic field due to magnetic dilution upon the substitution of non-magnetic Sn4+ ions for magnetic high-spin Fe3+ ions. Sn doping caused a decrease in length and width and an increase in thickness of elongated hematite nanoparticles. Fairly uniform Sn-doped hematite nanoellipsoids or nanocuboids were formed, depending on the Sn content. Temperature dependence of magnetization measurements showed the disappearance of the magnetic phase transition (Morin transition) in hematite upon Sn doping. Magnetic coercivity decreased upon Sn doping due to a decrease in shape anisotropy induced by the change in particle shape from nanorods to nanoellipsoids and nanocuboids. The optical and electronic properties of hematite nanoparticles were significantly affected by Sn doping – the absorption edge was shifted to higher wavelengths, while direct and indirect optical band gaps narrowed with the increasing Sn4+-for-Fe3+ substitution. Sn-doped hematite nanoellipsoids containing 4.3 mol% Sn exhibited a substantial visible light photocatalytic activity in the heterogeneous photo-Fenton process, but this activity significantly decreased with higher Sn doping.
T2  - Journal of Physics and Chemistry of Solids
T1  - Influence of Sn doping on the structural, magnetic, optical and photocatalytic properties of hematite (α-Fe2O3) nanoparticles
VL  - 161
SP  - 110372
DO  - 10.1016/j.jpcs.2021.110372
ER  - 
@article{
author = "Popov, Nina and Ristić, Mira and Bošković, Marko and Perović, Marija M. and Musić, Svetozar and Stanković, Dalibor M. and Krehula, Stjepko",
year = "2022",
abstract = "Sn-doped hematite (α-Fe2O3) nanoparticles of fairly uniform and Sn-dependent size and shape were synthesized via a simple combination of hydrothermal co-precipitation and calcination. The effects of Sn doping on the unit cell size, crystallinity, particle size and shape, as well as the magnetic, optical and photocatalytic properties of hematite nanoparticles were analyzed. The incorporation of Sn4+ ions into the crystal structure of hematite was confirmed by determination of the unit cell expansion due to the replacement of octahedrally coordinated Fe3+ ions by significantly larger Sn4+ ions, as well as a substantially reduced hyperfine magnetic field due to magnetic dilution upon the substitution of non-magnetic Sn4+ ions for magnetic high-spin Fe3+ ions. Sn doping caused a decrease in length and width and an increase in thickness of elongated hematite nanoparticles. Fairly uniform Sn-doped hematite nanoellipsoids or nanocuboids were formed, depending on the Sn content. Temperature dependence of magnetization measurements showed the disappearance of the magnetic phase transition (Morin transition) in hematite upon Sn doping. Magnetic coercivity decreased upon Sn doping due to a decrease in shape anisotropy induced by the change in particle shape from nanorods to nanoellipsoids and nanocuboids. The optical and electronic properties of hematite nanoparticles were significantly affected by Sn doping – the absorption edge was shifted to higher wavelengths, while direct and indirect optical band gaps narrowed with the increasing Sn4+-for-Fe3+ substitution. Sn-doped hematite nanoellipsoids containing 4.3 mol% Sn exhibited a substantial visible light photocatalytic activity in the heterogeneous photo-Fenton process, but this activity significantly decreased with higher Sn doping.",
journal = "Journal of Physics and Chemistry of Solids",
title = "Influence of Sn doping on the structural, magnetic, optical and photocatalytic properties of hematite (α-Fe2O3) nanoparticles",
volume = "161",
pages = "110372",
doi = "10.1016/j.jpcs.2021.110372"
}
Popov, N., Ristić, M., Bošković, M., Perović, M. M., Musić, S., Stanković, D. M.,& Krehula, S.. (2022). Influence of Sn doping on the structural, magnetic, optical and photocatalytic properties of hematite (α-Fe2O3) nanoparticles. in Journal of Physics and Chemistry of Solids, 161, 110372.
https://doi.org/10.1016/j.jpcs.2021.110372
Popov N, Ristić M, Bošković M, Perović MM, Musić S, Stanković DM, Krehula S. Influence of Sn doping on the structural, magnetic, optical and photocatalytic properties of hematite (α-Fe2O3) nanoparticles. in Journal of Physics and Chemistry of Solids. 2022;161:110372.
doi:10.1016/j.jpcs.2021.110372 .
Popov, Nina, Ristić, Mira, Bošković, Marko, Perović, Marija M., Musić, Svetozar, Stanković, Dalibor M., Krehula, Stjepko, "Influence of Sn doping on the structural, magnetic, optical and photocatalytic properties of hematite (α-Fe2O3) nanoparticles" in Journal of Physics and Chemistry of Solids, 161 (2022):110372,
https://doi.org/10.1016/j.jpcs.2021.110372 . .
6
1
3

Effect of Ru3+ ions on the formation, structural, magnetic and optical properties of hematite (α-Fe2O3) nanorods

Popov, Nina; Bošković, Marko; Perović, Marija M.; Zadro, Krešo; Gilja, Vanja; Kratofil Krenula, Ljerka; Robić, Marko; Marijan, Marciuš; Ristić, Mira; Musić, Svetozar; Stanković, Dalibor M.; Krehula, Stjepko

(2021)

TY  - JOUR
AU  - Popov, Nina
AU  - Bošković, Marko
AU  - Perović, Marija M.
AU  - Zadro, Krešo
AU  - Gilja, Vanja
AU  - Kratofil Krenula, Ljerka
AU  - Robić, Marko
AU  - Marijan, Marciuš
AU  - Ristić, Mira
AU  - Musić, Svetozar
AU  - Stanković, Dalibor M.
AU  - Krehula, Stjepko
PY  - 2021
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/9882
AB  - Nanosized hematite (α-Fe2O3) is a widely investigated material due to its favourable properties (chemically stable, environmentally safe, inexpensive) and very good performance in several advanced applications. Properties and performance of hematite nanoparticles can be adjusted and improved by modification of particle size and shape, as well as by substitution of Fe3+ ions in the crystal structure of hematite with other metal ions. Ru3+ ions are potentially suitable metal ions for the substitution of Fe3+ ions in hematite because of the same charge and similar ionic radii. In the present work, the effects of Ru3+ ions on the formation and properties of hematite nanorods prepared by combination of hydrothermal precipitation and calcination were investigated. The influence of the molar fraction of Ru3+ ions in the hydrothermal precipitation system on the formation and properties of iron oxide phases was studied. Single-phase goethite (α-FeOOH) nanorods containing incorporated Ru3+ ions were formed in the presence of low levels of Ru3+ ions (<3 mol%), while at higher levels (4 and 5 mol% Ru) hematite nanocylinders, consisting of self-assembled and fused nanoparticles, were obtained. The mechanism of the formation of these iron oxide nanostructures in the presence of Ru3+ ions was explained and compared with the effect of other metal cations reported in the literature. Ru-doped hematite nanorods were formed after calcination of Ru-doped goethite nanorods at 500 °C. A gradual elongation of hematite nanorods with increased Ru doping to highly elongated Ru-doped hematite nanoneedles at 2 mol% Ru was observed and explained. The influence of the Ru doping level on the magnetic properties of hematite nanorods was investigated using Mössbauer spectroscopy and magnetic measurements. Temperature of the transition between antiferromagnetic (AFM) and weakly ferromagnetic (WFM) spin ordering state (Morin transition) gradually rose with increasing Ru3+-for-Fe3+ substitution in hematite. Besides, magnetization of the WFM hematite gradually decreased with Ru doping which was attributed to the reduced canting of two almost antiparallel spin sublattices in this phase. The optical band gap in hematite nanorods was found to get gradually narrower with increased Ru doping due to the modified electronic structure.
T2  - Journal of magnetism and magnetic materials
T2  - Journal of magnetism and magnetic materials
T1  - Effect of Ru3+ ions on the formation, structural, magnetic and optical properties of hematite (α-Fe2O3) nanorods
VL  - 538
SP  - 168316
EP  - 168321
DO  - 10.1016/j.jmmm.2021.168316
ER  - 
@article{
author = "Popov, Nina and Bošković, Marko and Perović, Marija M. and Zadro, Krešo and Gilja, Vanja and Kratofil Krenula, Ljerka and Robić, Marko and Marijan, Marciuš and Ristić, Mira and Musić, Svetozar and Stanković, Dalibor M. and Krehula, Stjepko",
year = "2021",
abstract = "Nanosized hematite (α-Fe2O3) is a widely investigated material due to its favourable properties (chemically stable, environmentally safe, inexpensive) and very good performance in several advanced applications. Properties and performance of hematite nanoparticles can be adjusted and improved by modification of particle size and shape, as well as by substitution of Fe3+ ions in the crystal structure of hematite with other metal ions. Ru3+ ions are potentially suitable metal ions for the substitution of Fe3+ ions in hematite because of the same charge and similar ionic radii. In the present work, the effects of Ru3+ ions on the formation and properties of hematite nanorods prepared by combination of hydrothermal precipitation and calcination were investigated. The influence of the molar fraction of Ru3+ ions in the hydrothermal precipitation system on the formation and properties of iron oxide phases was studied. Single-phase goethite (α-FeOOH) nanorods containing incorporated Ru3+ ions were formed in the presence of low levels of Ru3+ ions (<3 mol%), while at higher levels (4 and 5 mol% Ru) hematite nanocylinders, consisting of self-assembled and fused nanoparticles, were obtained. The mechanism of the formation of these iron oxide nanostructures in the presence of Ru3+ ions was explained and compared with the effect of other metal cations reported in the literature. Ru-doped hematite nanorods were formed after calcination of Ru-doped goethite nanorods at 500 °C. A gradual elongation of hematite nanorods with increased Ru doping to highly elongated Ru-doped hematite nanoneedles at 2 mol% Ru was observed and explained. The influence of the Ru doping level on the magnetic properties of hematite nanorods was investigated using Mössbauer spectroscopy and magnetic measurements. Temperature of the transition between antiferromagnetic (AFM) and weakly ferromagnetic (WFM) spin ordering state (Morin transition) gradually rose with increasing Ru3+-for-Fe3+ substitution in hematite. Besides, magnetization of the WFM hematite gradually decreased with Ru doping which was attributed to the reduced canting of two almost antiparallel spin sublattices in this phase. The optical band gap in hematite nanorods was found to get gradually narrower with increased Ru doping due to the modified electronic structure.",
journal = "Journal of magnetism and magnetic materials, Journal of magnetism and magnetic materials",
title = "Effect of Ru3+ ions on the formation, structural, magnetic and optical properties of hematite (α-Fe2O3) nanorods",
volume = "538",
pages = "168316-168321",
doi = "10.1016/j.jmmm.2021.168316"
}
Popov, N., Bošković, M., Perović, M. M., Zadro, K., Gilja, V., Kratofil Krenula, L., Robić, M., Marijan, M., Ristić, M., Musić, S., Stanković, D. M.,& Krehula, S.. (2021). Effect of Ru3+ ions on the formation, structural, magnetic and optical properties of hematite (α-Fe2O3) nanorods. in Journal of magnetism and magnetic materials, 538, 168316-168321.
https://doi.org/10.1016/j.jmmm.2021.168316
Popov N, Bošković M, Perović MM, Zadro K, Gilja V, Kratofil Krenula L, Robić M, Marijan M, Ristić M, Musić S, Stanković DM, Krehula S. Effect of Ru3+ ions on the formation, structural, magnetic and optical properties of hematite (α-Fe2O3) nanorods. in Journal of magnetism and magnetic materials. 2021;538:168316-168321.
doi:10.1016/j.jmmm.2021.168316 .
Popov, Nina, Bošković, Marko, Perović, Marija M., Zadro, Krešo, Gilja, Vanja, Kratofil Krenula, Ljerka, Robić, Marko, Marijan, Marciuš, Ristić, Mira, Musić, Svetozar, Stanković, Dalibor M., Krehula, Stjepko, "Effect of Ru3+ ions on the formation, structural, magnetic and optical properties of hematite (α-Fe2O3) nanorods" in Journal of magnetism and magnetic materials, 538 (2021):168316-168321,
https://doi.org/10.1016/j.jmmm.2021.168316 . .
1
2
2

Search for high temperature memory effects in magnetic nanoparticles

Perović, Marija M.; Bošković, Marko; Kusigerski, Vladan B.; Jagličić, Zvonko; Blanuša, Jovan; Spasojević, Vojislav; Pizurova, Nadežda; Schneeweiss, Oldřich B.

(2021)

TY  - JOUR
AU  - Perović, Marija M.
AU  - Bošković, Marko
AU  - Kusigerski, Vladan B.
AU  - Jagličić, Zvonko
AU  - Blanuša, Jovan
AU  - Spasojević, Vojislav
AU  - Pizurova, Nadežda
AU  - Schneeweiss, Oldřich B.
PY  - 2021
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/9674
AB  - Nanoparticle materials have become a promising candidate for a new kind of storage media based on thermally induced memory effects due to the possibility to tailor their magnetic properties and behaviour. In this study, we have investigated whether the magnetic memory effects could appear at high, industry accessible temperatures including the possibility of thermal data inscription. Investigated iron oxide nanoparticles were synthesized by poliol method, which has been modified in order to allow control of particle agglomeration and consequently magnetic properties. Structure, morphology and the degree of nanoparticle agglomeration were studied by X-Ray diffraction, Transmission Electron Microscopy and Dynamic Light Scattering techniques, while magnetic properties as well as memory effects were measured on a commercial SQUID-based magnetometer. Results of the study confirmed that in super spin glass magnetite nanoparticles, magnetic memory effects can be observed up to 200 K which represents much higher temperatures in comparison to those achieved in spin glasses and other glassy materials. Procedures of writing and reading (inscribing and retrieving) of digital information in such a material were demonstrated and discussed in details.
T2  - Journal of Alloys and Compounds
T1  - Search for high temperature memory effects in magnetic nanoparticles
VL  - 855
SP  - 157523
DO  - 10.1016/j.jallcom.2020.157523
ER  - 
@article{
author = "Perović, Marija M. and Bošković, Marko and Kusigerski, Vladan B. and Jagličić, Zvonko and Blanuša, Jovan and Spasojević, Vojislav and Pizurova, Nadežda and Schneeweiss, Oldřich B.",
year = "2021",
abstract = "Nanoparticle materials have become a promising candidate for a new kind of storage media based on thermally induced memory effects due to the possibility to tailor their magnetic properties and behaviour. In this study, we have investigated whether the magnetic memory effects could appear at high, industry accessible temperatures including the possibility of thermal data inscription. Investigated iron oxide nanoparticles were synthesized by poliol method, which has been modified in order to allow control of particle agglomeration and consequently magnetic properties. Structure, morphology and the degree of nanoparticle agglomeration were studied by X-Ray diffraction, Transmission Electron Microscopy and Dynamic Light Scattering techniques, while magnetic properties as well as memory effects were measured on a commercial SQUID-based magnetometer. Results of the study confirmed that in super spin glass magnetite nanoparticles, magnetic memory effects can be observed up to 200 K which represents much higher temperatures in comparison to those achieved in spin glasses and other glassy materials. Procedures of writing and reading (inscribing and retrieving) of digital information in such a material were demonstrated and discussed in details.",
journal = "Journal of Alloys and Compounds",
title = "Search for high temperature memory effects in magnetic nanoparticles",
volume = "855",
pages = "157523",
doi = "10.1016/j.jallcom.2020.157523"
}
Perović, M. M., Bošković, M., Kusigerski, V. B., Jagličić, Z., Blanuša, J., Spasojević, V., Pizurova, N.,& Schneeweiss, O. B.. (2021). Search for high temperature memory effects in magnetic nanoparticles. in Journal of Alloys and Compounds, 855, 157523.
https://doi.org/10.1016/j.jallcom.2020.157523
Perović MM, Bošković M, Kusigerski VB, Jagličić Z, Blanuša J, Spasojević V, Pizurova N, Schneeweiss OB. Search for high temperature memory effects in magnetic nanoparticles. in Journal of Alloys and Compounds. 2021;855:157523.
doi:10.1016/j.jallcom.2020.157523 .
Perović, Marija M., Bošković, Marko, Kusigerski, Vladan B., Jagličić, Zvonko, Blanuša, Jovan, Spasojević, Vojislav, Pizurova, Nadežda, Schneeweiss, Oldřich B., "Search for high temperature memory effects in magnetic nanoparticles" in Journal of Alloys and Compounds, 855 (2021):157523,
https://doi.org/10.1016/j.jallcom.2020.157523 . .

Influence of low-spin Co3+ for high-spin Fe3+ substitution on the structural, magnetic, optical and catalytic properties of hematite (α-Fe2O3) nanorods

Popov, Nina; Bošković, Marko; Perović, Marija M.; Németh, Zoltán; Wang, Junhu; Kuang, Zhichong; Reissner, Michael; Kuzmann, Ernő; Homonnay, Zoltán; Kubuki, Shiro; Marciuš, Marijan; Ristić, Mira; Musić, Svetozar; Stanković, Dalibor M.; Krehula, Stjepko

(2021)

TY  - JOUR
AU  - Popov, Nina
AU  - Bošković, Marko
AU  - Perović, Marija M.
AU  - Németh, Zoltán
AU  - Wang, Junhu
AU  - Kuang, Zhichong
AU  - Reissner, Michael
AU  - Kuzmann, Ernő
AU  - Homonnay, Zoltán
AU  - Kubuki, Shiro
AU  - Marciuš, Marijan
AU  - Ristić, Mira
AU  - Musić, Svetozar
AU  - Stanković, Dalibor M.
AU  - Krehula, Stjepko
PY  - 2021
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/9516
AB  - Pure hematite nanorods and very long and thin cobalt-doped hematite nanorods (nanoneedles) were prepared by a combined precipitation and annealing method. The influence of the level of cobalt doping on different properties of hematite nanorods was investigated. Incorporation of cobalt in the form of low-spin Co3+ ions into the structure of hematite by substitution for high-spin Fe3+ ions was proved by determination of a significant unit cell contraction by powder X-ray diffraction (PXRD) and characteristic positions of the absorption edge in X-ray absorption near edge structure (XANES) spectra and peaks in X-ray emission (XES) spectra. Cobalt doping caused a gradual elongation and thinning of hematite nanorods – very long and thin 1D nanoparticles (nanoneedles) were formed in the presence of 10 and 12 mol% Co. Magnetic measurements showed a strong increase in low-temperature remanent magnetization and coercivity upon cobalt doping, as well as a disappearance of the Morin transition, which was also confirmed by Mössbauer spectroscopy. Cobalt doping significantly affected optical properties of hematite nanorods – absorption in the visible and NIR ranges increased, which was accompanied by narrowing of the optical band gap. Compared with pure hematite nanorods cobalt-doped hematite nanoneedles showed a significantly better electrocatalytic activity for the oxygen evolution reaction (OER). © 2020 Elsevier Ltd
T2  - Journal of Physics and Chemistry of Solids
T1  - Influence of low-spin Co3+ for high-spin Fe3+ substitution on the structural, magnetic, optical and catalytic properties of hematite (α-Fe2O3) nanorods
VL  - 152
SP  - 109929
DO  - 10.1016/j.jpcs.2020.109929
ER  - 
@article{
author = "Popov, Nina and Bošković, Marko and Perović, Marija M. and Németh, Zoltán and Wang, Junhu and Kuang, Zhichong and Reissner, Michael and Kuzmann, Ernő and Homonnay, Zoltán and Kubuki, Shiro and Marciuš, Marijan and Ristić, Mira and Musić, Svetozar and Stanković, Dalibor M. and Krehula, Stjepko",
year = "2021",
abstract = "Pure hematite nanorods and very long and thin cobalt-doped hematite nanorods (nanoneedles) were prepared by a combined precipitation and annealing method. The influence of the level of cobalt doping on different properties of hematite nanorods was investigated. Incorporation of cobalt in the form of low-spin Co3+ ions into the structure of hematite by substitution for high-spin Fe3+ ions was proved by determination of a significant unit cell contraction by powder X-ray diffraction (PXRD) and characteristic positions of the absorption edge in X-ray absorption near edge structure (XANES) spectra and peaks in X-ray emission (XES) spectra. Cobalt doping caused a gradual elongation and thinning of hematite nanorods – very long and thin 1D nanoparticles (nanoneedles) were formed in the presence of 10 and 12 mol% Co. Magnetic measurements showed a strong increase in low-temperature remanent magnetization and coercivity upon cobalt doping, as well as a disappearance of the Morin transition, which was also confirmed by Mössbauer spectroscopy. Cobalt doping significantly affected optical properties of hematite nanorods – absorption in the visible and NIR ranges increased, which was accompanied by narrowing of the optical band gap. Compared with pure hematite nanorods cobalt-doped hematite nanoneedles showed a significantly better electrocatalytic activity for the oxygen evolution reaction (OER). © 2020 Elsevier Ltd",
journal = "Journal of Physics and Chemistry of Solids",
title = "Influence of low-spin Co3+ for high-spin Fe3+ substitution on the structural, magnetic, optical and catalytic properties of hematite (α-Fe2O3) nanorods",
volume = "152",
pages = "109929",
doi = "10.1016/j.jpcs.2020.109929"
}
Popov, N., Bošković, M., Perović, M. M., Németh, Z., Wang, J., Kuang, Z., Reissner, M., Kuzmann, E., Homonnay, Z., Kubuki, S., Marciuš, M., Ristić, M., Musić, S., Stanković, D. M.,& Krehula, S.. (2021). Influence of low-spin Co3+ for high-spin Fe3+ substitution on the structural, magnetic, optical and catalytic properties of hematite (α-Fe2O3) nanorods. in Journal of Physics and Chemistry of Solids, 152, 109929.
https://doi.org/10.1016/j.jpcs.2020.109929
Popov N, Bošković M, Perović MM, Németh Z, Wang J, Kuang Z, Reissner M, Kuzmann E, Homonnay Z, Kubuki S, Marciuš M, Ristić M, Musić S, Stanković DM, Krehula S. Influence of low-spin Co3+ for high-spin Fe3+ substitution on the structural, magnetic, optical and catalytic properties of hematite (α-Fe2O3) nanorods. in Journal of Physics and Chemistry of Solids. 2021;152:109929.
doi:10.1016/j.jpcs.2020.109929 .
Popov, Nina, Bošković, Marko, Perović, Marija M., Németh, Zoltán, Wang, Junhu, Kuang, Zhichong, Reissner, Michael, Kuzmann, Ernő, Homonnay, Zoltán, Kubuki, Shiro, Marciuš, Marijan, Ristić, Mira, Musić, Svetozar, Stanković, Dalibor M., Krehula, Stjepko, "Influence of low-spin Co3+ for high-spin Fe3+ substitution on the structural, magnetic, optical and catalytic properties of hematite (α-Fe2O3) nanorods" in Journal of Physics and Chemistry of Solids, 152 (2021):109929,
https://doi.org/10.1016/j.jpcs.2020.109929 . .
4
2
3

Magnetic memory effect in hollandite-type α-K MnO2 monocrystalline nanorods

Barudžija, Tanja; Perović, Marija M.; Bošković, Marko; Cvjetićanin, Nikola; Gyergyek, Sašo; Mitrić, Miodrag

(2020)

TY  - JOUR
AU  - Barudžija, Tanja
AU  - Perović, Marija M.
AU  - Bošković, Marko
AU  - Cvjetićanin, Nikola
AU  - Gyergyek, Sašo
AU  - Mitrić, Miodrag
PY  - 2020
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/8743
AB  - Memory effect due to spin-glass state below about 20 K has been illustrated in the hollandite-type α-KxMnO2 monocrystalline nanorods by systematic magnetization measurements including temperature- and time-dependent magnetization curves in low fields. In this work, we succeeded in writing, reading, and deleting 8-bits digital information in the investigated system. These results show that α-KxMnO2 is a good candidate material for a thermal memory cell. The phenomenological droplet model was used in the description of the observed memory effect, whose origin in α-KxMnO2 is associated with bulk properties, doping and frustration. © 2019 Elsevier B.V.
T2  - Journal of Alloys and Compounds
T1  - Magnetic memory effect in hollandite-type α-K MnO2 monocrystalline nanorods
VL  - 820
SP  - 153406
DO  - 10.1016/j.jallcom.2019.153406
ER  - 
@article{
author = "Barudžija, Tanja and Perović, Marija M. and Bošković, Marko and Cvjetićanin, Nikola and Gyergyek, Sašo and Mitrić, Miodrag",
year = "2020",
abstract = "Memory effect due to spin-glass state below about 20 K has been illustrated in the hollandite-type α-KxMnO2 monocrystalline nanorods by systematic magnetization measurements including temperature- and time-dependent magnetization curves in low fields. In this work, we succeeded in writing, reading, and deleting 8-bits digital information in the investigated system. These results show that α-KxMnO2 is a good candidate material for a thermal memory cell. The phenomenological droplet model was used in the description of the observed memory effect, whose origin in α-KxMnO2 is associated with bulk properties, doping and frustration. © 2019 Elsevier B.V.",
journal = "Journal of Alloys and Compounds",
title = "Magnetic memory effect in hollandite-type α-K MnO2 monocrystalline nanorods",
volume = "820",
pages = "153406",
doi = "10.1016/j.jallcom.2019.153406"
}
Barudžija, T., Perović, M. M., Bošković, M., Cvjetićanin, N., Gyergyek, S.,& Mitrić, M.. (2020). Magnetic memory effect in hollandite-type α-K MnO2 monocrystalline nanorods. in Journal of Alloys and Compounds, 820, 153406.
https://doi.org/10.1016/j.jallcom.2019.153406
Barudžija T, Perović MM, Bošković M, Cvjetićanin N, Gyergyek S, Mitrić M. Magnetic memory effect in hollandite-type α-K MnO2 monocrystalline nanorods. in Journal of Alloys and Compounds. 2020;820:153406.
doi:10.1016/j.jallcom.2019.153406 .
Barudžija, Tanja, Perović, Marija M., Bošković, Marko, Cvjetićanin, Nikola, Gyergyek, Sašo, Mitrić, Miodrag, "Magnetic memory effect in hollandite-type α-K MnO2 monocrystalline nanorods" in Journal of Alloys and Compounds, 820 (2020):153406,
https://doi.org/10.1016/j.jallcom.2019.153406 . .
2
2
2

Crystal Structure and Magnetocaloric Effect of La0.80Ag0.15MnO3 Nanoparticles

Zentkova, M.; Mihalik, Marian; Mihalik, Jr., M.; Kovalik, M; Perović, Marija M.; Vavra, M.; Briančin, J.

(2020)

TY  - JOUR
AU  - Zentkova, M.
AU  - Mihalik, Marian
AU  - Mihalik, Jr., M.
AU  - Kovalik, M
AU  - Perović, Marija M.
AU  - Vavra, M.
AU  - Briančin, J.
PY  - 2020
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/9085
AB  - Annealing of_ non stoichiometric La0.80Ag0.15MnO3 nanoparticles leads to the change of the crystal symmetry from Pnma to R3c and to almost doubling of its Curie temperature from 117 K to 317 K. This effect is due to the releasing of lattice distortions and strengthening of double exchange interaction. The large values of the magnetocaloric entropy of the order of ∆S = 6.19 J/(kg K) were observedat ∆µ0H = 5 T and T = 315 K.
T2  - Acta Physica Polonica A
T1  - Crystal Structure and Magnetocaloric Effect of La0.80Ag0.15MnO3 Nanoparticles
VL  - 137
IS  - 5
SP  - 900
EP  - 903
DO  - 10.12693/APhysPolA.137.900
ER  - 
@article{
author = "Zentkova, M. and Mihalik, Marian and Mihalik, Jr., M. and Kovalik, M and Perović, Marija M. and Vavra, M. and Briančin, J.",
year = "2020",
abstract = "Annealing of_ non stoichiometric La0.80Ag0.15MnO3 nanoparticles leads to the change of the crystal symmetry from Pnma to R3c and to almost doubling of its Curie temperature from 117 K to 317 K. This effect is due to the releasing of lattice distortions and strengthening of double exchange interaction. The large values of the magnetocaloric entropy of the order of ∆S = 6.19 J/(kg K) were observedat ∆µ0H = 5 T and T = 315 K.",
journal = "Acta Physica Polonica A",
title = "Crystal Structure and Magnetocaloric Effect of La0.80Ag0.15MnO3 Nanoparticles",
volume = "137",
number = "5",
pages = "900-903",
doi = "10.12693/APhysPolA.137.900"
}
Zentkova, M., Mihalik, M., Mihalik, Jr., M., Kovalik, M., Perović, M. M., Vavra, M.,& Briančin, J.. (2020). Crystal Structure and Magnetocaloric Effect of La0.80Ag0.15MnO3 Nanoparticles. in Acta Physica Polonica A, 137(5), 900-903.
https://doi.org/10.12693/APhysPolA.137.900
Zentkova M, Mihalik M, Mihalik JM, Kovalik M, Perović MM, Vavra M, Briančin J. Crystal Structure and Magnetocaloric Effect of La0.80Ag0.15MnO3 Nanoparticles. in Acta Physica Polonica A. 2020;137(5):900-903.
doi:10.12693/APhysPolA.137.900 .
Zentkova, M., Mihalik, Marian, Mihalik, Jr., M., Kovalik, M, Perović, Marija M., Vavra, M., Briančin, J., "Crystal Structure and Magnetocaloric Effect of La0.80Ag0.15MnO3 Nanoparticles" in Acta Physica Polonica A, 137, no. 5 (2020):900-903,
https://doi.org/10.12693/APhysPolA.137.900 . .
1
1

Magnetic properties and heating efficacy of magnesium doped magnetite nanoparticles obtained by co-precipitation method

Kusigerski, Vladan; Illés, Erzsébet; Blanuša, Jovan; Gyergyek, Sašo; Bošković, Marko; Perović, Marija M.; Spasojević, Vojislav

(2019)

TY  - JOUR
AU  - Kusigerski, Vladan
AU  - Illés, Erzsébet
AU  - Blanuša, Jovan
AU  - Gyergyek, Sašo
AU  - Bošković, Marko
AU  - Perović, Marija M.
AU  - Spasojević, Vojislav
PY  - 2019
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/7983
AB  - Ferrofluids based on magnesium substituted magnetite nanoparticles MgxFe3−xO4 (x = 0.1; 0.2; 0.4) were synthesised by a chemical co-precipitation method. Their physical properties have been compared with those of the magnetite based ferrofluid obtained by the same synthesis route. Both XRD and TEM studies showed particle size decrease with the increased Mg content while DLS experiments pointed to the more prominent aggregation of Mg-containing nanoparticles. Magnetic properties investigation conducted on the powder (i.e. dried) specimens showed decrease of magnetization values with increased Mg content except for the lowest concentration of x = 0.1 where substantial saturation magnetization rise of about 40% was recorded at room temperature. Heating abilities of the studied ferrofluids under the applied AC fields (SAR values) also showed decreasing trend with the increased Mg content even for x = 0.1 sample despite its elevated magnetization value. This trend has been understood as a consequence of the changed intrinsic nanoparticle properties such as size and magnetic anisotropy, as well as contribution of a collective behaviour due to an increased nanoparticle aggregation in Mg-doped systems.
T2  - Journal of Magnetism and Magnetic Materials
T1  - Magnetic properties and heating efficacy of magnesium doped magnetite nanoparticles obtained by co-precipitation method
VL  - 475
SP  - 470
EP  - 478
DO  - 10.1016/j.jmmm.2018.11.127
ER  - 
@article{
author = "Kusigerski, Vladan and Illés, Erzsébet and Blanuša, Jovan and Gyergyek, Sašo and Bošković, Marko and Perović, Marija M. and Spasojević, Vojislav",
year = "2019",
abstract = "Ferrofluids based on magnesium substituted magnetite nanoparticles MgxFe3−xO4 (x = 0.1; 0.2; 0.4) were synthesised by a chemical co-precipitation method. Their physical properties have been compared with those of the magnetite based ferrofluid obtained by the same synthesis route. Both XRD and TEM studies showed particle size decrease with the increased Mg content while DLS experiments pointed to the more prominent aggregation of Mg-containing nanoparticles. Magnetic properties investigation conducted on the powder (i.e. dried) specimens showed decrease of magnetization values with increased Mg content except for the lowest concentration of x = 0.1 where substantial saturation magnetization rise of about 40% was recorded at room temperature. Heating abilities of the studied ferrofluids under the applied AC fields (SAR values) also showed decreasing trend with the increased Mg content even for x = 0.1 sample despite its elevated magnetization value. This trend has been understood as a consequence of the changed intrinsic nanoparticle properties such as size and magnetic anisotropy, as well as contribution of a collective behaviour due to an increased nanoparticle aggregation in Mg-doped systems.",
journal = "Journal of Magnetism and Magnetic Materials",
title = "Magnetic properties and heating efficacy of magnesium doped magnetite nanoparticles obtained by co-precipitation method",
volume = "475",
pages = "470-478",
doi = "10.1016/j.jmmm.2018.11.127"
}
Kusigerski, V., Illés, E., Blanuša, J., Gyergyek, S., Bošković, M., Perović, M. M.,& Spasojević, V.. (2019). Magnetic properties and heating efficacy of magnesium doped magnetite nanoparticles obtained by co-precipitation method. in Journal of Magnetism and Magnetic Materials, 475, 470-478.
https://doi.org/10.1016/j.jmmm.2018.11.127
Kusigerski V, Illés E, Blanuša J, Gyergyek S, Bošković M, Perović MM, Spasojević V. Magnetic properties and heating efficacy of magnesium doped magnetite nanoparticles obtained by co-precipitation method. in Journal of Magnetism and Magnetic Materials. 2019;475:470-478.
doi:10.1016/j.jmmm.2018.11.127 .
Kusigerski, Vladan, Illés, Erzsébet, Blanuša, Jovan, Gyergyek, Sašo, Bošković, Marko, Perović, Marija M., Spasojević, Vojislav, "Magnetic properties and heating efficacy of magnesium doped magnetite nanoparticles obtained by co-precipitation method" in Journal of Magnetism and Magnetic Materials, 475 (2019):470-478,
https://doi.org/10.1016/j.jmmm.2018.11.127 . .
27
21
21

Influence of Fe(III) doping on the crystal structure and properties of hydrothermally prepared β-Ni(OH) 2 nanostructures

Krehula, Stjepko; Ristić, Mira; Wu, Chuchu; Li, Xuning; Jiang, Luhua; Wang, Junhu H.; Sun, Gongquan; Zhang, Tao; Perović, Marija M.; Bošković, Marko; Antić, Bratislav; Kratofil Krehula, Ljerka; Kobzi, Balazs; Kubuki, Shiro; Musić, Svetozar

(2018)

TY  - JOUR
AU  - Krehula, Stjepko
AU  - Ristić, Mira
AU  - Wu, Chuchu
AU  - Li, Xuning
AU  - Jiang, Luhua
AU  - Wang, Junhu H.
AU  - Sun, Gongquan
AU  - Zhang, Tao
AU  - Perović, Marija M.
AU  - Bošković, Marko
AU  - Antić, Bratislav
AU  - Kratofil Krehula, Ljerka
AU  - Kobzi, Balazs
AU  - Kubuki, Shiro
AU  - Musić, Svetozar
PY  - 2018
UR  - http://linkinghub.elsevier.com/retrieve/pii/S0925838818313197
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/7744
AB  - This paper systematically examines the influence of the level of Fe(III) doping on the crystal structure and other properties of Ni(OH)(2). Reference beta-Ni(OH)(2) and Fe-doped Ni(OH)(2) samples were synthesized by hydrothermal precipitation of mixed Ni(II) and Fe(III) nitrate aqueous solutions in a highly alkaline medium. The samples were investigated using X-ray powder diffraction (XRPD), scanning and transmission electron microscopy (FE-SEM and TEM), energy dispersive X-ray spectroscopy (EDS), Mossbauer spectroscopy, magnetic measurements, Fourier transform infrared (FT-IR) spectroscopy, ultraviolet-visible-near infrared (UV-Vis-NIR) spectroscopy, thermogravimetric analysis (TGA) and electrochemical measurements. Incorporation of Fe in beta-Ni(OH)(2) by cation substitution was confirmed from the shifts in position of XRPD lines due to the difference in the ionic radius of Fe3+ and Ni-2. The Fe-3-for-Ni2+ substitution in beta-Ni(OH)(2) caused formation of an interstratifled structure with beta-Ni(OH)(2) and alpha-Ni(OH)(2) structural units interconnected within the same structural layers and crystallites. Mossbauer spectra revealed the presence of Fe3+ ions in highly distorted octahedral sites, presumably at the boundary between the alpha-Ni(OH)(2) and beta-Ni(OH)(2) structural units within the same structural layer. Electrochemical measurements showed significant increase in oxygen evolution reaction (OER) catalytic activity of Fe-doped Ni(OH)(2) compared to pure phase. (C) 2018 Elsevier B.V. All rights reserved.
T2  - Journal of Alloys and Compounds
T1  - Influence of Fe(III) doping on the crystal structure and properties of hydrothermally prepared β-Ni(OH) 2 nanostructures
VL  - 750
SP  - 687
EP  - 695
DO  - 10.1016/j.jallcom.2018.04.032
ER  - 
@article{
author = "Krehula, Stjepko and Ristić, Mira and Wu, Chuchu and Li, Xuning and Jiang, Luhua and Wang, Junhu H. and Sun, Gongquan and Zhang, Tao and Perović, Marija M. and Bošković, Marko and Antić, Bratislav and Kratofil Krehula, Ljerka and Kobzi, Balazs and Kubuki, Shiro and Musić, Svetozar",
year = "2018",
abstract = "This paper systematically examines the influence of the level of Fe(III) doping on the crystal structure and other properties of Ni(OH)(2). Reference beta-Ni(OH)(2) and Fe-doped Ni(OH)(2) samples were synthesized by hydrothermal precipitation of mixed Ni(II) and Fe(III) nitrate aqueous solutions in a highly alkaline medium. The samples were investigated using X-ray powder diffraction (XRPD), scanning and transmission electron microscopy (FE-SEM and TEM), energy dispersive X-ray spectroscopy (EDS), Mossbauer spectroscopy, magnetic measurements, Fourier transform infrared (FT-IR) spectroscopy, ultraviolet-visible-near infrared (UV-Vis-NIR) spectroscopy, thermogravimetric analysis (TGA) and electrochemical measurements. Incorporation of Fe in beta-Ni(OH)(2) by cation substitution was confirmed from the shifts in position of XRPD lines due to the difference in the ionic radius of Fe3+ and Ni-2. The Fe-3-for-Ni2+ substitution in beta-Ni(OH)(2) caused formation of an interstratifled structure with beta-Ni(OH)(2) and alpha-Ni(OH)(2) structural units interconnected within the same structural layers and crystallites. Mossbauer spectra revealed the presence of Fe3+ ions in highly distorted octahedral sites, presumably at the boundary between the alpha-Ni(OH)(2) and beta-Ni(OH)(2) structural units within the same structural layer. Electrochemical measurements showed significant increase in oxygen evolution reaction (OER) catalytic activity of Fe-doped Ni(OH)(2) compared to pure phase. (C) 2018 Elsevier B.V. All rights reserved.",
journal = "Journal of Alloys and Compounds",
title = "Influence of Fe(III) doping on the crystal structure and properties of hydrothermally prepared β-Ni(OH) 2 nanostructures",
volume = "750",
pages = "687-695",
doi = "10.1016/j.jallcom.2018.04.032"
}
Krehula, S., Ristić, M., Wu, C., Li, X., Jiang, L., Wang, J. H., Sun, G., Zhang, T., Perović, M. M., Bošković, M., Antić, B., Kratofil Krehula, L., Kobzi, B., Kubuki, S.,& Musić, S.. (2018). Influence of Fe(III) doping on the crystal structure and properties of hydrothermally prepared β-Ni(OH) 2 nanostructures. in Journal of Alloys and Compounds, 750, 687-695.
https://doi.org/10.1016/j.jallcom.2018.04.032
Krehula S, Ristić M, Wu C, Li X, Jiang L, Wang JH, Sun G, Zhang T, Perović MM, Bošković M, Antić B, Kratofil Krehula L, Kobzi B, Kubuki S, Musić S. Influence of Fe(III) doping on the crystal structure and properties of hydrothermally prepared β-Ni(OH) 2 nanostructures. in Journal of Alloys and Compounds. 2018;750:687-695.
doi:10.1016/j.jallcom.2018.04.032 .
Krehula, Stjepko, Ristić, Mira, Wu, Chuchu, Li, Xuning, Jiang, Luhua, Wang, Junhu H., Sun, Gongquan, Zhang, Tao, Perović, Marija M., Bošković, Marko, Antić, Bratislav, Kratofil Krehula, Ljerka, Kobzi, Balazs, Kubuki, Shiro, Musić, Svetozar, "Influence of Fe(III) doping on the crystal structure and properties of hydrothermally prepared β-Ni(OH) 2 nanostructures" in Journal of Alloys and Compounds, 750 (2018):687-695,
https://doi.org/10.1016/j.jallcom.2018.04.032 . .
21
20
21

Synthesis and Properties of Ni-doped Goethite and Ni-doped Hematite Nanorods

Krehula, Stjepko; Ristić, Mira; Mitar, Ivana; Wu, Chuchu; Li, Xuning; Jiang, Luhua; Wang, Junhu H.; Sun, Gongquan; Zhang, Tao; Perović, Marija M.; Bošković, Marko; Antić, Bratislav; Musić, Svetozar

(2018)

TY  - JOUR
AU  - Krehula, Stjepko
AU  - Ristić, Mira
AU  - Mitar, Ivana
AU  - Wu, Chuchu
AU  - Li, Xuning
AU  - Jiang, Luhua
AU  - Wang, Junhu H.
AU  - Sun, Gongquan
AU  - Zhang, Tao
AU  - Perović, Marija M.
AU  - Bošković, Marko
AU  - Antić, Bratislav
AU  - Musić, Svetozar
PY  - 2018
UR  - https://hrcak.srce.hr/file/309798
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/8100
AB  - Ni-doped goethite (α-FeOOH) nanorods were synthesized from mixed Fe(III)-Ni(II) nitrate solutions with various Ni/(Ni+Fe) ratios (0, 5, 10, 20, 33 and 50 mol % Ni) by hydrothermal precipitation in a highly alkaline medium using the strong organic alkali, tetramethylammonium hydroxide (TMAH). Ni-doped hematite (α-Fe2O3) nanorods were obtained by calcination of Ni-doped goethite nanorods at 400 °C. The Ni 2+ -for-Fe 3+ substitution in goethite and hematite was confirmed by determination of the unit cell expansion (due to the difference in the ionic radii of Fe 3+ and Ni 2+ ) using XRPD and determination of the reduction of a hyperfine magnetic field (due to the difference in magnetic moments of Fe 3+ and Ni 2+ ) using Mössbauer spectroscopy. Single-phase goethite nanorods were found in samples containing 0 or 5 mol % Ni. A higher Ni content in the precipitation system (10 mol % or more) resulted in a higher Ni 2+ -for-Fe 3+ substitution in goethite, and larger Ni-doped goethite nanorods, though with the presence of low crystalline Ni-containing ferrihydrite and Ni ferrite (NiFe2O4) as additional phases. Significant changes in FT-IR and UV-Vis-NIR spectra of prepared samples were observed with increasing Ni content. Electrochemical measurements of samples showed a strong increase in oxygen evolution reaction (OER) electrocatalytic activity with increasing Ni content. © 2018 Croatian Chemical Society. All Rights Reserved.
T2  - Croatica Chemica Acta
T1  - Synthesis and Properties of Ni-doped Goethite and Ni-doped Hematite Nanorods
VL  - 91
IS  - 3
SP  - 389
EP  - 401
DO  - 10.5562/cca3402
ER  - 
@article{
author = "Krehula, Stjepko and Ristić, Mira and Mitar, Ivana and Wu, Chuchu and Li, Xuning and Jiang, Luhua and Wang, Junhu H. and Sun, Gongquan and Zhang, Tao and Perović, Marija M. and Bošković, Marko and Antić, Bratislav and Musić, Svetozar",
year = "2018",
abstract = "Ni-doped goethite (α-FeOOH) nanorods were synthesized from mixed Fe(III)-Ni(II) nitrate solutions with various Ni/(Ni+Fe) ratios (0, 5, 10, 20, 33 and 50 mol % Ni) by hydrothermal precipitation in a highly alkaline medium using the strong organic alkali, tetramethylammonium hydroxide (TMAH). Ni-doped hematite (α-Fe2O3) nanorods were obtained by calcination of Ni-doped goethite nanorods at 400 °C. The Ni 2+ -for-Fe 3+ substitution in goethite and hematite was confirmed by determination of the unit cell expansion (due to the difference in the ionic radii of Fe 3+ and Ni 2+ ) using XRPD and determination of the reduction of a hyperfine magnetic field (due to the difference in magnetic moments of Fe 3+ and Ni 2+ ) using Mössbauer spectroscopy. Single-phase goethite nanorods were found in samples containing 0 or 5 mol % Ni. A higher Ni content in the precipitation system (10 mol % or more) resulted in a higher Ni 2+ -for-Fe 3+ substitution in goethite, and larger Ni-doped goethite nanorods, though with the presence of low crystalline Ni-containing ferrihydrite and Ni ferrite (NiFe2O4) as additional phases. Significant changes in FT-IR and UV-Vis-NIR spectra of prepared samples were observed with increasing Ni content. Electrochemical measurements of samples showed a strong increase in oxygen evolution reaction (OER) electrocatalytic activity with increasing Ni content. © 2018 Croatian Chemical Society. All Rights Reserved.",
journal = "Croatica Chemica Acta",
title = "Synthesis and Properties of Ni-doped Goethite and Ni-doped Hematite Nanorods",
volume = "91",
number = "3",
pages = "389-401",
doi = "10.5562/cca3402"
}
Krehula, S., Ristić, M., Mitar, I., Wu, C., Li, X., Jiang, L., Wang, J. H., Sun, G., Zhang, T., Perović, M. M., Bošković, M., Antić, B.,& Musić, S.. (2018). Synthesis and Properties of Ni-doped Goethite and Ni-doped Hematite Nanorods. in Croatica Chemica Acta, 91(3), 389-401.
https://doi.org/10.5562/cca3402
Krehula S, Ristić M, Mitar I, Wu C, Li X, Jiang L, Wang JH, Sun G, Zhang T, Perović MM, Bošković M, Antić B, Musić S. Synthesis and Properties of Ni-doped Goethite and Ni-doped Hematite Nanorods. in Croatica Chemica Acta. 2018;91(3):389-401.
doi:10.5562/cca3402 .
Krehula, Stjepko, Ristić, Mira, Mitar, Ivana, Wu, Chuchu, Li, Xuning, Jiang, Luhua, Wang, Junhu H., Sun, Gongquan, Zhang, Tao, Perović, Marija M., Bošković, Marko, Antić, Bratislav, Musić, Svetozar, "Synthesis and Properties of Ni-doped Goethite and Ni-doped Hematite Nanorods" in Croatica Chemica Acta, 91, no. 3 (2018):389-401,
https://doi.org/10.5562/cca3402 . .
7
6
6

Exchange Bias Effect in NdFeO3 System of Nanoparticles

Vavra, M.; Zentkova, M.; Mihalik, M.; Mihalik, Jr., M.; Lazurova, J.; Girman, V.; Perović, Marija M.; Kusigerski, Vladan; Roupcova, P.; Jaglicic, Z.

(2017)

TY  - JOUR
AU  - Vavra, M.
AU  - Zentkova, M.
AU  - Mihalik, M.
AU  - Mihalik, Jr., M.
AU  - Lazurova, J.
AU  - Girman, V.
AU  - Perović, Marija M.
AU  - Kusigerski, Vladan
AU  - Roupcova, P.
AU  - Jaglicic, Z.
PY  - 2017
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/7162
AB  - We study the effect of nanometric size on the crystal structure, magnetic environment of iron and magnetization in NdFeO3 system of nanoparticles. The average particle size of NdFeO3 nanoparticles increases with annealing at 600 degrees C from about 15 nm to 40 nm, The smallest particles on annealed sample have size approximately 30 nm and typically have character of single crystalline samples. All samples adopt orthorhombic crystal structure, space group Prima with lattice parameters a = 5.5817 angstrom, b = 7.7663 angstrom and c = 5.456 angstrom for as prepared sample. The presence of superparamagnetic particles was indicated by the Mossbauer measurements. The reduction of dimensionality induces a decrease of T-N1 from 691 K to 544 K. The shift of magnetic hysteresis loop in vertical and horizontal direction was observed at low temperatures after cooling in magnetic field. We attribute such behaviour to exchange bias effect and discuss in the frame of core shellmodel.
T2  - Acta Physica Polonica. Series A: General Physics, Physics of Condensed Matter, Optics and Quantum Electronics, Atomic and Molecular Physics, Applied Physics
T1  - Exchange Bias Effect in NdFeO3 System of Nanoparticles
VL  - 131
IS  - 4
SP  - 869
EP  - 871
DO  - 10.12693/APhysPolA.131.869
ER  - 
@article{
author = "Vavra, M. and Zentkova, M. and Mihalik, M. and Mihalik, Jr., M. and Lazurova, J. and Girman, V. and Perović, Marija M. and Kusigerski, Vladan and Roupcova, P. and Jaglicic, Z.",
year = "2017",
abstract = "We study the effect of nanometric size on the crystal structure, magnetic environment of iron and magnetization in NdFeO3 system of nanoparticles. The average particle size of NdFeO3 nanoparticles increases with annealing at 600 degrees C from about 15 nm to 40 nm, The smallest particles on annealed sample have size approximately 30 nm and typically have character of single crystalline samples. All samples adopt orthorhombic crystal structure, space group Prima with lattice parameters a = 5.5817 angstrom, b = 7.7663 angstrom and c = 5.456 angstrom for as prepared sample. The presence of superparamagnetic particles was indicated by the Mossbauer measurements. The reduction of dimensionality induces a decrease of T-N1 from 691 K to 544 K. The shift of magnetic hysteresis loop in vertical and horizontal direction was observed at low temperatures after cooling in magnetic field. We attribute such behaviour to exchange bias effect and discuss in the frame of core shellmodel.",
journal = "Acta Physica Polonica. Series A: General Physics, Physics of Condensed Matter, Optics and Quantum Electronics, Atomic and Molecular Physics, Applied Physics",
title = "Exchange Bias Effect in NdFeO3 System of Nanoparticles",
volume = "131",
number = "4",
pages = "869-871",
doi = "10.12693/APhysPolA.131.869"
}
Vavra, M., Zentkova, M., Mihalik, M., Mihalik, Jr., M., Lazurova, J., Girman, V., Perović, M. M., Kusigerski, V., Roupcova, P.,& Jaglicic, Z.. (2017). Exchange Bias Effect in NdFeO3 System of Nanoparticles. in Acta Physica Polonica. Series A: General Physics, Physics of Condensed Matter, Optics and Quantum Electronics, Atomic and Molecular Physics, Applied Physics, 131(4), 869-871.
https://doi.org/10.12693/APhysPolA.131.869
Vavra M, Zentkova M, Mihalik M, Mihalik JM, Lazurova J, Girman V, Perović MM, Kusigerski V, Roupcova P, Jaglicic Z. Exchange Bias Effect in NdFeO3 System of Nanoparticles. in Acta Physica Polonica. Series A: General Physics, Physics of Condensed Matter, Optics and Quantum Electronics, Atomic and Molecular Physics, Applied Physics. 2017;131(4):869-871.
doi:10.12693/APhysPolA.131.869 .
Vavra, M., Zentkova, M., Mihalik, M., Mihalik, Jr., M., Lazurova, J., Girman, V., Perović, Marija M., Kusigerski, Vladan, Roupcova, P., Jaglicic, Z., "Exchange Bias Effect in NdFeO3 System of Nanoparticles" in Acta Physica Polonica. Series A: General Physics, Physics of Condensed Matter, Optics and Quantum Electronics, Atomic and Molecular Physics, Applied Physics, 131, no. 4 (2017):869-871,
https://doi.org/10.12693/APhysPolA.131.869 . .
3
3
4

Structural and magnetic properties of hydrothermally synthesized beta-MnO2 and alpha-KxMnO2 nanorods

Barudžija, Tanja; Kusigerski, Vladan; Cvjetićanin, Nikola; Šorgić, Saša; Perović, Marija M.; Mitrić, Miodrag

(Elsevier, 2016)

TY  - JOUR
AU  - Barudžija, Tanja
AU  - Kusigerski, Vladan
AU  - Cvjetićanin, Nikola
AU  - Šorgić, Saša
AU  - Perović, Marija M.
AU  - Mitrić, Miodrag
PY  - 2016
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/920
AB  - Hydrothermal synthesis was applied for obtaining different manganese dioxide polymorphs whose morphology, structure and magnetic properties were thoroughly investigated. Variations in the synthesis pathways lead to the formation of tetragonal rutile-type beta-MnO2 and two tetragonal hollandite-type alpha-KxMnO2 samples with different concentration of potassium cations (x = 0.15 and 0.18). SEM images showed nanorod shape of all specimens, while microstructure characterization done by XRD measurements revealed that crystallites have an elongated rod-like shape and, hence, it confirmed the anisotropic morphology. Magnetic ordering of beta-MnO2 is antiferromagnetic below 93 K, while both alpha-KxMnO2 samples possess more complicated low-temperature behaviour of the reentrant spin-glass type: the onset of the spin-glass like state occurs at temperatures below the weak ferromagnetic ordering. (C) 2016 Elsevier B.V. All rights reserved.
PB  - Elsevier
T2  - Journal of Alloys and Compounds
T1  - Structural and magnetic properties of hydrothermally synthesized beta-MnO2 and alpha-KxMnO2 nanorods
VL  - 665
SP  - 261
EP  - 270
DO  - 10.1016/j.jallcom.2016.01.024
ER  - 
@article{
author = "Barudžija, Tanja and Kusigerski, Vladan and Cvjetićanin, Nikola and Šorgić, Saša and Perović, Marija M. and Mitrić, Miodrag",
year = "2016",
abstract = "Hydrothermal synthesis was applied for obtaining different manganese dioxide polymorphs whose morphology, structure and magnetic properties were thoroughly investigated. Variations in the synthesis pathways lead to the formation of tetragonal rutile-type beta-MnO2 and two tetragonal hollandite-type alpha-KxMnO2 samples with different concentration of potassium cations (x = 0.15 and 0.18). SEM images showed nanorod shape of all specimens, while microstructure characterization done by XRD measurements revealed that crystallites have an elongated rod-like shape and, hence, it confirmed the anisotropic morphology. Magnetic ordering of beta-MnO2 is antiferromagnetic below 93 K, while both alpha-KxMnO2 samples possess more complicated low-temperature behaviour of the reentrant spin-glass type: the onset of the spin-glass like state occurs at temperatures below the weak ferromagnetic ordering. (C) 2016 Elsevier B.V. All rights reserved.",
publisher = "Elsevier",
journal = "Journal of Alloys and Compounds",
title = "Structural and magnetic properties of hydrothermally synthesized beta-MnO2 and alpha-KxMnO2 nanorods",
volume = "665",
pages = "261-270",
doi = "10.1016/j.jallcom.2016.01.024"
}
Barudžija, T., Kusigerski, V., Cvjetićanin, N., Šorgić, S., Perović, M. M.,& Mitrić, M.. (2016). Structural and magnetic properties of hydrothermally synthesized beta-MnO2 and alpha-KxMnO2 nanorods. in Journal of Alloys and Compounds
Elsevier., 665, 261-270.
https://doi.org/10.1016/j.jallcom.2016.01.024
Barudžija T, Kusigerski V, Cvjetićanin N, Šorgić S, Perović MM, Mitrić M. Structural and magnetic properties of hydrothermally synthesized beta-MnO2 and alpha-KxMnO2 nanorods. in Journal of Alloys and Compounds. 2016;665:261-270.
doi:10.1016/j.jallcom.2016.01.024 .
Barudžija, Tanja, Kusigerski, Vladan, Cvjetićanin, Nikola, Šorgić, Saša, Perović, Marija M., Mitrić, Miodrag, "Structural and magnetic properties of hydrothermally synthesized beta-MnO2 and alpha-KxMnO2 nanorods" in Journal of Alloys and Compounds, 665 (2016):261-270,
https://doi.org/10.1016/j.jallcom.2016.01.024 . .
17
18
19

The glassy behaviour of poorly crystalline Fe2O3 nanorods obtained by thermal decomposition of ferrous oxalate

Perović, Marija M.; Kusigerski, Vladan; Mraković, Ana Đ.; Spasojević, Vojislav; Blanuša, Jovan; Nikolić, Violeta N.; Schneeweiss, Oldřich B.; David, B.; Pizurova, Nadežda

(2015)

TY  - JOUR
AU  - Perović, Marija M.
AU  - Kusigerski, Vladan
AU  - Mraković, Ana Đ.
AU  - Spasojević, Vojislav
AU  - Blanuša, Jovan
AU  - Nikolić, Violeta N.
AU  - Schneeweiss, Oldřich B.
AU  - David, B.
AU  - Pizurova, Nadežda
PY  - 2015
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/429
AB  - Nanorod ferrous oxalate dihydrate (FeC2O4 x 2H(2)O) which had been synthesized by the microemulsion method, was used as a precursor in the thermal decomposition process performed in air atmosphere. The formation of nanocrystalline hematite as the final product was preceded by the appearence of an intermediate product. Comprehensive study comprising several complementary techniques (x-ray diffraction, transmission electron microscopy, selected area electron diffraction, thermogravimetric/differential thermal analyses and SQUID magnetometry) confirmed that the intermediate product corresponds to the poorly crystalline Fe2O3. Due to the specific nanorod shape and poorly crystalline structure, the investigated Fe2O3 showed high coercive field value of similar to 0.5 T at 5 K. Special attention in this study was devoted to the peculiar magnetic properties of poorly crystalline Fe2O3, which were thoroughly investigated by employing sophisticated experimental procedures such as relaxation of thermoremanent magnetization for different cooling fields, zero field and field cooled memory effects as well as aging experiments for different waiting times. At low temperatures and weak applied magnetic fields, the investigated system behaves similarly to spin glasses, manifesting slow, collective relaxation dynamics of magnetic moments through memory, rejuvenation and aging effects.
T2  - Nanotechnology
T1  - The glassy behaviour of poorly crystalline Fe2O3 nanorods obtained by thermal decomposition of ferrous oxalate
VL  - 26
IS  - 11
DO  - 10.1088/0957-4484/26/11/115705
ER  - 
@article{
author = "Perović, Marija M. and Kusigerski, Vladan and Mraković, Ana Đ. and Spasojević, Vojislav and Blanuša, Jovan and Nikolić, Violeta N. and Schneeweiss, Oldřich B. and David, B. and Pizurova, Nadežda",
year = "2015",
abstract = "Nanorod ferrous oxalate dihydrate (FeC2O4 x 2H(2)O) which had been synthesized by the microemulsion method, was used as a precursor in the thermal decomposition process performed in air atmosphere. The formation of nanocrystalline hematite as the final product was preceded by the appearence of an intermediate product. Comprehensive study comprising several complementary techniques (x-ray diffraction, transmission electron microscopy, selected area electron diffraction, thermogravimetric/differential thermal analyses and SQUID magnetometry) confirmed that the intermediate product corresponds to the poorly crystalline Fe2O3. Due to the specific nanorod shape and poorly crystalline structure, the investigated Fe2O3 showed high coercive field value of similar to 0.5 T at 5 K. Special attention in this study was devoted to the peculiar magnetic properties of poorly crystalline Fe2O3, which were thoroughly investigated by employing sophisticated experimental procedures such as relaxation of thermoremanent magnetization for different cooling fields, zero field and field cooled memory effects as well as aging experiments for different waiting times. At low temperatures and weak applied magnetic fields, the investigated system behaves similarly to spin glasses, manifesting slow, collective relaxation dynamics of magnetic moments through memory, rejuvenation and aging effects.",
journal = "Nanotechnology",
title = "The glassy behaviour of poorly crystalline Fe2O3 nanorods obtained by thermal decomposition of ferrous oxalate",
volume = "26",
number = "11",
doi = "10.1088/0957-4484/26/11/115705"
}
Perović, M. M., Kusigerski, V., Mraković, A. Đ., Spasojević, V., Blanuša, J., Nikolić, V. N., Schneeweiss, O. B., David, B.,& Pizurova, N.. (2015). The glassy behaviour of poorly crystalline Fe2O3 nanorods obtained by thermal decomposition of ferrous oxalate. in Nanotechnology, 26(11).
https://doi.org/10.1088/0957-4484/26/11/115705
Perović MM, Kusigerski V, Mraković AĐ, Spasojević V, Blanuša J, Nikolić VN, Schneeweiss OB, David B, Pizurova N. The glassy behaviour of poorly crystalline Fe2O3 nanorods obtained by thermal decomposition of ferrous oxalate. in Nanotechnology. 2015;26(11).
doi:10.1088/0957-4484/26/11/115705 .
Perović, Marija M., Kusigerski, Vladan, Mraković, Ana Đ., Spasojević, Vojislav, Blanuša, Jovan, Nikolić, Violeta N., Schneeweiss, Oldřich B., David, B., Pizurova, Nadežda, "The glassy behaviour of poorly crystalline Fe2O3 nanorods obtained by thermal decomposition of ferrous oxalate" in Nanotechnology, 26, no. 11 (2015),
https://doi.org/10.1088/0957-4484/26/11/115705 . .
6
4
4

Magnetic Properties and Mossbauer spectroscopy of NdFe(1-x)MnxO(3)

Lazurova, J.; Mihalik, M.; Mihalik, Jr., M.; Vavra, M.; Zentkova, M.; Briancin, J.; Perović, Marija M.; Kusigerski, Vladan; Schneeweiss, Oldřich B.; Roupcova, P.; Kamenev, K. V.; Misek, M.; Jaglicic, Z.

(2015)

TY  - CONF
AU  - Lazurova, J.
AU  - Mihalik, M.
AU  - Mihalik, Jr., M.
AU  - Vavra, M.
AU  - Zentkova, M.
AU  - Briancin, J.
AU  - Perović, Marija M.
AU  - Kusigerski, Vladan
AU  - Schneeweiss, Oldřich B.
AU  - Roupcova, P.
AU  - Kamenev, K. V.
AU  - Misek, M.
AU  - Jaglicic, Z.
PY  - 2015
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/7067
AB  - The effect of particle reduction to nanoscale size and substitution of Mn3+ ions for Fe3+ ions on the crystal structure, lattice dynamics, Mossbauer spectra and magnetic properties in NdFe(1-x)MnxO(3) compounds have been studied. X-ray powder diffraction and Raman spectroscopy revealed that the Jahn-Teller distortion of lattice dominates for samples with x GT 0.4. The average particle size of NdFeO3 nanoparticles (NAP) increases with annealing at 600 degrees C from about 15 nm to 25 nm. The presence of superparamagnetic particles was indicated by Mossbauer measurements in NdFeO3 NAP system. Sextets in NdFe(1-x)MnxO(3) Mssbauer spectra can be modelled with several local environments of Fe3+ induced by substitution. The reduction of dimensionality and the substitution induce a decrease of the Neel temperature T-Nl from 691 K to 544 K for NAP or to 356 K for x = 0.4, however the temperature of spin reorientation T-SR increases with substitution. The saturated magnetization obtained at 1.9 K increases and ferromagnetic component is removed below T-SR with the substitution.
C3  - Journal of Physics: Conference Series
T1  - Magnetic Properties and Mossbauer spectroscopy of NdFe(1-x)MnxO(3)
VL  - 592
DO  - 10.1088/1742-6596/592/1/012117
ER  - 
@conference{
author = "Lazurova, J. and Mihalik, M. and Mihalik, Jr., M. and Vavra, M. and Zentkova, M. and Briancin, J. and Perović, Marija M. and Kusigerski, Vladan and Schneeweiss, Oldřich B. and Roupcova, P. and Kamenev, K. V. and Misek, M. and Jaglicic, Z.",
year = "2015",
abstract = "The effect of particle reduction to nanoscale size and substitution of Mn3+ ions for Fe3+ ions on the crystal structure, lattice dynamics, Mossbauer spectra and magnetic properties in NdFe(1-x)MnxO(3) compounds have been studied. X-ray powder diffraction and Raman spectroscopy revealed that the Jahn-Teller distortion of lattice dominates for samples with x GT 0.4. The average particle size of NdFeO3 nanoparticles (NAP) increases with annealing at 600 degrees C from about 15 nm to 25 nm. The presence of superparamagnetic particles was indicated by Mossbauer measurements in NdFeO3 NAP system. Sextets in NdFe(1-x)MnxO(3) Mssbauer spectra can be modelled with several local environments of Fe3+ induced by substitution. The reduction of dimensionality and the substitution induce a decrease of the Neel temperature T-Nl from 691 K to 544 K for NAP or to 356 K for x = 0.4, however the temperature of spin reorientation T-SR increases with substitution. The saturated magnetization obtained at 1.9 K increases and ferromagnetic component is removed below T-SR with the substitution.",
journal = "Journal of Physics: Conference Series",
title = "Magnetic Properties and Mossbauer spectroscopy of NdFe(1-x)MnxO(3)",
volume = "592",
doi = "10.1088/1742-6596/592/1/012117"
}
Lazurova, J., Mihalik, M., Mihalik, Jr., M., Vavra, M., Zentkova, M., Briancin, J., Perović, M. M., Kusigerski, V., Schneeweiss, O. B., Roupcova, P., Kamenev, K. V., Misek, M.,& Jaglicic, Z.. (2015). Magnetic Properties and Mossbauer spectroscopy of NdFe(1-x)MnxO(3). in Journal of Physics: Conference Series, 592.
https://doi.org/10.1088/1742-6596/592/1/012117
Lazurova J, Mihalik M, Mihalik JM, Vavra M, Zentkova M, Briancin J, Perović MM, Kusigerski V, Schneeweiss OB, Roupcova P, Kamenev KV, Misek M, Jaglicic Z. Magnetic Properties and Mossbauer spectroscopy of NdFe(1-x)MnxO(3). in Journal of Physics: Conference Series. 2015;592.
doi:10.1088/1742-6596/592/1/012117 .
Lazurova, J., Mihalik, M., Mihalik, Jr., M., Vavra, M., Zentkova, M., Briancin, J., Perović, Marija M., Kusigerski, Vladan, Schneeweiss, Oldřich B., Roupcova, P., Kamenev, K. V., Misek, M., Jaglicic, Z., "Magnetic Properties and Mossbauer spectroscopy of NdFe(1-x)MnxO(3)" in Journal of Physics: Conference Series, 592 (2015),
https://doi.org/10.1088/1742-6596/592/1/012117 . .
10
11
11

Experimental evidence for simultaneous relaxation processes in super spin glass gamma-Fe2O3 nanoparticle system

Nikolić, Violeta N.; Perović, Marija M.; Kusigerski, Vladan; Bošković, Marko; Mraković, Ana Đ.; Blanuša, Jovan; Spasojević, Vojislav

(2015)

TY  - JOUR
AU  - Nikolić, Violeta N.
AU  - Perović, Marija M.
AU  - Kusigerski, Vladan
AU  - Bošković, Marko
AU  - Mraković, Ana Đ.
AU  - Blanuša, Jovan
AU  - Spasojević, Vojislav
PY  - 2015
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/561
AB  - Spherical gamma-Fe2O3 nanoparticles with the narrow size distribution of (5 +/- 1) nm were synthesized by the method of thermal decomposition from iron acetyl acetonate precursor. The existence of super spin-glass state at low temperatures and in low applied magnetic fields was confirmed by DC magnetization measurements on a SQUID magnetometer. The comprehensive investigation of magnetic relaxation dynamics in low-temperature region was conducted through the measurements of single-stop and multiple stop ZFC memory effects, ZFC magnetization relaxation, and AC susceptibility measurements. The experimental findings revealed the peculiar change of magnetic relaxation dynamics at T approximate to 10 K, which arose as a consequence of simultaneous existence of different relaxation processes in Fe2O3 nanoparticle system. Complementarity of the applied measurements was utilized in order to single out distinct relaxation processes as well as to elucidate complex relaxation mechanisms in the investigated interacting nanoparticle system.
T2  - Journal of Nanoparticle Research
T1  - Experimental evidence for simultaneous relaxation processes in super spin glass gamma-Fe2O3 nanoparticle system
VL  - 17
IS  - 3
DO  - 10.1007/s11051-015-2952-2
ER  - 
@article{
author = "Nikolić, Violeta N. and Perović, Marija M. and Kusigerski, Vladan and Bošković, Marko and Mraković, Ana Đ. and Blanuša, Jovan and Spasojević, Vojislav",
year = "2015",
abstract = "Spherical gamma-Fe2O3 nanoparticles with the narrow size distribution of (5 +/- 1) nm were synthesized by the method of thermal decomposition from iron acetyl acetonate precursor. The existence of super spin-glass state at low temperatures and in low applied magnetic fields was confirmed by DC magnetization measurements on a SQUID magnetometer. The comprehensive investigation of magnetic relaxation dynamics in low-temperature region was conducted through the measurements of single-stop and multiple stop ZFC memory effects, ZFC magnetization relaxation, and AC susceptibility measurements. The experimental findings revealed the peculiar change of magnetic relaxation dynamics at T approximate to 10 K, which arose as a consequence of simultaneous existence of different relaxation processes in Fe2O3 nanoparticle system. Complementarity of the applied measurements was utilized in order to single out distinct relaxation processes as well as to elucidate complex relaxation mechanisms in the investigated interacting nanoparticle system.",
journal = "Journal of Nanoparticle Research",
title = "Experimental evidence for simultaneous relaxation processes in super spin glass gamma-Fe2O3 nanoparticle system",
volume = "17",
number = "3",
doi = "10.1007/s11051-015-2952-2"
}
Nikolić, V. N., Perović, M. M., Kusigerski, V., Bošković, M., Mraković, A. Đ., Blanuša, J.,& Spasojević, V.. (2015). Experimental evidence for simultaneous relaxation processes in super spin glass gamma-Fe2O3 nanoparticle system. in Journal of Nanoparticle Research, 17(3).
https://doi.org/10.1007/s11051-015-2952-2
Nikolić VN, Perović MM, Kusigerski V, Bošković M, Mraković AĐ, Blanuša J, Spasojević V. Experimental evidence for simultaneous relaxation processes in super spin glass gamma-Fe2O3 nanoparticle system. in Journal of Nanoparticle Research. 2015;17(3).
doi:10.1007/s11051-015-2952-2 .
Nikolić, Violeta N., Perović, Marija M., Kusigerski, Vladan, Bošković, Marko, Mraković, Ana Đ., Blanuša, Jovan, Spasojević, Vojislav, "Experimental evidence for simultaneous relaxation processes in super spin glass gamma-Fe2O3 nanoparticle system" in Journal of Nanoparticle Research, 17, no. 3 (2015),
https://doi.org/10.1007/s11051-015-2952-2 . .
3
3
3

Synthesis and microstructural properties of mixed iron-gallium oxides

Krehula, Stjepko; Ristić, Mira; Kubuki, Shiro; Iida, Yusuke; Perović, Marija M.; Fabian, Martin; Musić, Svetozar

(2015)

TY  - JOUR
AU  - Krehula, Stjepko
AU  - Ristić, Mira
AU  - Kubuki, Shiro
AU  - Iida, Yusuke
AU  - Perović, Marija M.
AU  - Fabian, Martin
AU  - Musić, Svetozar
PY  - 2015
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/265
AB  - Various mixed Fe-Ga oxides were prepared by the calcination of mixed Fe-Ga oxyhydroxide precursors (alpha-Fe1 xGaxOOH solid solutions, 0 LT = x LT = 1) at 500 or 1000 degrees C. Isostructural corundum-type oxides alpha-Fe2O3 and alpha-Ga2O3, as well as their solid solutions alpha-Fe-2 xGaxO3 in the entire concentration range (x = 0, 0.4, 1, 1.6 and 2) were prepared by calcination at 500 degrees C. An increase in the Ga content in alpha-Fe2 xGaxO3 resulted in a reduction of the unit cell size, a weakened hyperfine magnetic field, a disappearance of the Morin transition, an increase of magnetization at low temperatures, a shift in the position of IR bands to higher wavenumbers, and a lower intensity of absorption bands in the UV-Vis-NIR spectra. The calcination of Fe-Ga oxyhydroxides at 1000 degrees C resulted in the formation of a rhombohedral alpha-Fe-2 xGaxO3 phase for x = 0 and 0.4. An orthorhombic GaFeO3 phase with Fe3+ cations located in 3 different octahedral sites was obtained by the calcination at 1000 degrees C of mixed Fe-Ga oxyhydroxide with the Fe:Ga ratio of 1:1. A monoclinic phase b-Fe-2 xGaxO3 (x = 1.6 and 2) was obtained by the calcination at 1000 degrees C of Fe-Ga oxyhydroxides with 80 and 100 mol% Ga. The monoclinic beta-Ga1.6Fe0.4O3 showed two strong luminescence peaks in the blue region of the PL spectrum. (C) 2015 Elsevier B.V. All rights reserved.
T2  - Journal of Alloys and Compounds
T1  - Synthesis and microstructural properties of mixed iron-gallium oxides
VL  - 634
SP  - 130
EP  - 141
DO  - 10.1016/j.jallcom.2015.02.065
ER  - 
@article{
author = "Krehula, Stjepko and Ristić, Mira and Kubuki, Shiro and Iida, Yusuke and Perović, Marija M. and Fabian, Martin and Musić, Svetozar",
year = "2015",
abstract = "Various mixed Fe-Ga oxides were prepared by the calcination of mixed Fe-Ga oxyhydroxide precursors (alpha-Fe1 xGaxOOH solid solutions, 0 LT = x LT = 1) at 500 or 1000 degrees C. Isostructural corundum-type oxides alpha-Fe2O3 and alpha-Ga2O3, as well as their solid solutions alpha-Fe-2 xGaxO3 in the entire concentration range (x = 0, 0.4, 1, 1.6 and 2) were prepared by calcination at 500 degrees C. An increase in the Ga content in alpha-Fe2 xGaxO3 resulted in a reduction of the unit cell size, a weakened hyperfine magnetic field, a disappearance of the Morin transition, an increase of magnetization at low temperatures, a shift in the position of IR bands to higher wavenumbers, and a lower intensity of absorption bands in the UV-Vis-NIR spectra. The calcination of Fe-Ga oxyhydroxides at 1000 degrees C resulted in the formation of a rhombohedral alpha-Fe-2 xGaxO3 phase for x = 0 and 0.4. An orthorhombic GaFeO3 phase with Fe3+ cations located in 3 different octahedral sites was obtained by the calcination at 1000 degrees C of mixed Fe-Ga oxyhydroxide with the Fe:Ga ratio of 1:1. A monoclinic phase b-Fe-2 xGaxO3 (x = 1.6 and 2) was obtained by the calcination at 1000 degrees C of Fe-Ga oxyhydroxides with 80 and 100 mol% Ga. The monoclinic beta-Ga1.6Fe0.4O3 showed two strong luminescence peaks in the blue region of the PL spectrum. (C) 2015 Elsevier B.V. All rights reserved.",
journal = "Journal of Alloys and Compounds",
title = "Synthesis and microstructural properties of mixed iron-gallium oxides",
volume = "634",
pages = "130-141",
doi = "10.1016/j.jallcom.2015.02.065"
}
Krehula, S., Ristić, M., Kubuki, S., Iida, Y., Perović, M. M., Fabian, M.,& Musić, S.. (2015). Synthesis and microstructural properties of mixed iron-gallium oxides. in Journal of Alloys and Compounds, 634, 130-141.
https://doi.org/10.1016/j.jallcom.2015.02.065
Krehula S, Ristić M, Kubuki S, Iida Y, Perović MM, Fabian M, Musić S. Synthesis and microstructural properties of mixed iron-gallium oxides. in Journal of Alloys and Compounds. 2015;634:130-141.
doi:10.1016/j.jallcom.2015.02.065 .
Krehula, Stjepko, Ristić, Mira, Kubuki, Shiro, Iida, Yusuke, Perović, Marija M., Fabian, Martin, Musić, Svetozar, "Synthesis and microstructural properties of mixed iron-gallium oxides" in Journal of Alloys and Compounds, 634 (2015):130-141,
https://doi.org/10.1016/j.jallcom.2015.02.065 . .
12
12
13

Mossbauer Spectra and Crystallite Size Related Magnetic/Electric Properties of Yb Substituted Zn-Ferrite Nanoparticles

Bošković, Marko; Perović, Marija M.; Vučinić-Vasić, Milica; Spasojević, Vojislav; Stojanovic, G.; Antić, Bratislav

(2014)

TY  - JOUR
AU  - Bošković, Marko
AU  - Perović, Marija M.
AU  - Vučinić-Vasić, Milica
AU  - Spasojević, Vojislav
AU  - Stojanovic, G.
AU  - Antić, Bratislav
PY  - 2014
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/6005
AB  - Influence of thermal-annealing-controlled crystallite size on the magnetic/electric properties of Yb substituted Zn-ferrite nanoparticles (ZnFe1.95Yb0.05O4) is studied, and results of the analysis are presented here. Room temperature Mossbauer spectrum of as-prepared sample shows coexistence of the sextet/doublet structure due to the particle size distribution. The central doublet originating from superparamagnetic relaxations of smaller particles is found to constitute the major fraction of the Fe-57 signal in samples obtained by thermal annealing of as-prepared sample at various temperatures in 300 degrees C-800 degrees C range. The determined quadrupole splitting (QS) parameters are significantly higher compared to corresponding bulk counterpart value and display decreasing trend with the crystallite size increase. The similar to 29 nm-sample, obtained by annealing at 800 degrees C, shows bulk-like properties, both in terms of the observed QS value and observed distribution of iron ions within the spinel lattice. Electric resistivity has non-monotonic dependence on crystallite-size, which could be attributed to enhanced disorder in as-prepared material. Partial substitution of iron by ytterbium in Zn-ferrite is found to increase the dielectric constant.
T2  - Nanoscience and Nanotechnology Letters
T1  - Mossbauer Spectra and Crystallite Size Related Magnetic/Electric Properties of Yb Substituted Zn-Ferrite Nanoparticles
VL  - 6
IS  - 4
SP  - 314
EP  - 318
DO  - 10.1166/nnl.2014.1758
ER  - 
@article{
author = "Bošković, Marko and Perović, Marija M. and Vučinić-Vasić, Milica and Spasojević, Vojislav and Stojanovic, G. and Antić, Bratislav",
year = "2014",
abstract = "Influence of thermal-annealing-controlled crystallite size on the magnetic/electric properties of Yb substituted Zn-ferrite nanoparticles (ZnFe1.95Yb0.05O4) is studied, and results of the analysis are presented here. Room temperature Mossbauer spectrum of as-prepared sample shows coexistence of the sextet/doublet structure due to the particle size distribution. The central doublet originating from superparamagnetic relaxations of smaller particles is found to constitute the major fraction of the Fe-57 signal in samples obtained by thermal annealing of as-prepared sample at various temperatures in 300 degrees C-800 degrees C range. The determined quadrupole splitting (QS) parameters are significantly higher compared to corresponding bulk counterpart value and display decreasing trend with the crystallite size increase. The similar to 29 nm-sample, obtained by annealing at 800 degrees C, shows bulk-like properties, both in terms of the observed QS value and observed distribution of iron ions within the spinel lattice. Electric resistivity has non-monotonic dependence on crystallite-size, which could be attributed to enhanced disorder in as-prepared material. Partial substitution of iron by ytterbium in Zn-ferrite is found to increase the dielectric constant.",
journal = "Nanoscience and Nanotechnology Letters",
title = "Mossbauer Spectra and Crystallite Size Related Magnetic/Electric Properties of Yb Substituted Zn-Ferrite Nanoparticles",
volume = "6",
number = "4",
pages = "314-318",
doi = "10.1166/nnl.2014.1758"
}
Bošković, M., Perović, M. M., Vučinić-Vasić, M., Spasojević, V., Stojanovic, G.,& Antić, B.. (2014). Mossbauer Spectra and Crystallite Size Related Magnetic/Electric Properties of Yb Substituted Zn-Ferrite Nanoparticles. in Nanoscience and Nanotechnology Letters, 6(4), 314-318.
https://doi.org/10.1166/nnl.2014.1758
Bošković M, Perović MM, Vučinić-Vasić M, Spasojević V, Stojanovic G, Antić B. Mossbauer Spectra and Crystallite Size Related Magnetic/Electric Properties of Yb Substituted Zn-Ferrite Nanoparticles. in Nanoscience and Nanotechnology Letters. 2014;6(4):314-318.
doi:10.1166/nnl.2014.1758 .
Bošković, Marko, Perović, Marija M., Vučinić-Vasić, Milica, Spasojević, Vojislav, Stojanovic, G., Antić, Bratislav, "Mossbauer Spectra and Crystallite Size Related Magnetic/Electric Properties of Yb Substituted Zn-Ferrite Nanoparticles" in Nanoscience and Nanotechnology Letters, 6, no. 4 (2014):314-318,
https://doi.org/10.1166/nnl.2014.1758 . .
1
1

Crystal structure and magnetic properties of Y-2(Cu1-xMgx)(2)O-5 obtained by SHS method

Gebrel, Z.; Blanuša, Jovan; Kusigerski, Vladan; Spasojević, Vojislav; Mraković, Ana Đ.; Perović, Marija M.; Alqat, A.

(2014)

TY  - JOUR
AU  - Gebrel, Z.
AU  - Blanuša, Jovan
AU  - Kusigerski, Vladan
AU  - Spasojević, Vojislav
AU  - Mraković, Ana Đ.
AU  - Perović, Marija M.
AU  - Alqat, A.
PY  - 2014
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/5714
AB  - The single-phase polycrystalline samples of Y-2(Cu1-xMgx)(2)O-5, x = 0.0, 0.05, 0.15 were successfully synthesized by a modified self-propagating high temperature synthesis. Effects of Mg+2 substitution for Cu+2 in metamagnetic Y2Cu2O5 on its crystal structure and magnetic properties have been analyzed by X-ray diffraction and magnetic measurements performed within 2-300 K range. Mg doping was found to introduce small distortions in the main intradimmer superexchange paths so that ferromagnetic correlations decrease with Mg concentration. More significant impact of Cu substitution was found on the low temperature magnetism due to the breaking of infinite Cu-O chains. The formation of finite size chains introduces low temperature paramagnetic contribution and reduction in Neel temperature. Overall results give a strong indication that the antiferromagnetic ordering as well as metamagnetism persists up to the 15% of the Mg concentration. (C) 2013 Elsevier B.V. All rights reserved.
T2  - Journal of Alloys and Compounds
T1  - Crystal structure and magnetic properties of Y-2(Cu1-xMgx)(2)O-5 obtained by SHS method
VL  - 582
SP  - 186
EP  - 189
DO  - 10.1016/j.jallcom.2013.08.033
ER  - 
@article{
author = "Gebrel, Z. and Blanuša, Jovan and Kusigerski, Vladan and Spasojević, Vojislav and Mraković, Ana Đ. and Perović, Marija M. and Alqat, A.",
year = "2014",
abstract = "The single-phase polycrystalline samples of Y-2(Cu1-xMgx)(2)O-5, x = 0.0, 0.05, 0.15 were successfully synthesized by a modified self-propagating high temperature synthesis. Effects of Mg+2 substitution for Cu+2 in metamagnetic Y2Cu2O5 on its crystal structure and magnetic properties have been analyzed by X-ray diffraction and magnetic measurements performed within 2-300 K range. Mg doping was found to introduce small distortions in the main intradimmer superexchange paths so that ferromagnetic correlations decrease with Mg concentration. More significant impact of Cu substitution was found on the low temperature magnetism due to the breaking of infinite Cu-O chains. The formation of finite size chains introduces low temperature paramagnetic contribution and reduction in Neel temperature. Overall results give a strong indication that the antiferromagnetic ordering as well as metamagnetism persists up to the 15% of the Mg concentration. (C) 2013 Elsevier B.V. All rights reserved.",
journal = "Journal of Alloys and Compounds",
title = "Crystal structure and magnetic properties of Y-2(Cu1-xMgx)(2)O-5 obtained by SHS method",
volume = "582",
pages = "186-189",
doi = "10.1016/j.jallcom.2013.08.033"
}
Gebrel, Z., Blanuša, J., Kusigerski, V., Spasojević, V., Mraković, A. Đ., Perović, M. M.,& Alqat, A.. (2014). Crystal structure and magnetic properties of Y-2(Cu1-xMgx)(2)O-5 obtained by SHS method. in Journal of Alloys and Compounds, 582, 186-189.
https://doi.org/10.1016/j.jallcom.2013.08.033
Gebrel Z, Blanuša J, Kusigerski V, Spasojević V, Mraković AĐ, Perović MM, Alqat A. Crystal structure and magnetic properties of Y-2(Cu1-xMgx)(2)O-5 obtained by SHS method. in Journal of Alloys and Compounds. 2014;582:186-189.
doi:10.1016/j.jallcom.2013.08.033 .
Gebrel, Z., Blanuša, Jovan, Kusigerski, Vladan, Spasojević, Vojislav, Mraković, Ana Đ., Perović, Marija M., Alqat, A., "Crystal structure and magnetic properties of Y-2(Cu1-xMgx)(2)O-5 obtained by SHS method" in Journal of Alloys and Compounds, 582 (2014):186-189,
https://doi.org/10.1016/j.jallcom.2013.08.033 . .

Synthesis and characterization of bentonites rich in beidellite with incorporated Al or Al-Fe oxide pillars

Bankovic, P.; Milutinovic-Nikolic, A.; Mojovic, Z.; Jovic-Jovicic, N.; Perović, Marija M.; Spasojević, Vojislav; Jovanović, Dragana J.

(2013)

TY  - JOUR
AU  - Bankovic, P.
AU  - Milutinovic-Nikolic, A.
AU  - Mojovic, Z.
AU  - Jovic-Jovicic, N.
AU  - Perović, Marija M.
AU  - Spasojević, Vojislav
AU  - Jovanović, Dragana J.
PY  - 2013
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/5162
AB  - Pillared clays (PILCs) based on bentonite clay from Bogovina (Serbia) were obtained using Al3+ and Fe3+ pillaring cations in different ratios. Thorough characterization of the starting material and PILCs was performed for better understanding of the catalytic activity that they had exibited in the catalytic wet peroxide oxidation (CWPO) of organic pollutants in water. The characterization consisted of the following techniques: XRD, XRD of oriented samples (swelling test), Greene-Kelley test (smectite type determination), TGA/DTA followed by XRD analysis of samples heated at characteristic temperatures, elemental analysis using ICP-OES and microwave digestion. FTIR, DR UV-Vis, Mossbauer spectroscopy, nitrogen physisorption at -196 degrees C and SEM imaging. Smectite in admixture with quartz was identified, together with impurities like feldspar, illite, chlorite and X-ray amorphous matter. Smectite mineral was dominantly of the beidellite type. Pillaring led to changes in the d(001) smectite basal spacing and stabilization of the smectite structure. Increasing Fe3+ content of the pillaring solutions resulted in the increased incorporation of iron into the PILCs as isolated octahedrally coordinated Fe3+ cations, smaller and bigger oligonuclear octahedrally coordinated Fe3+ species and octahedrally coordinated Fe3+ particles. The structure of incorporated pillars was similar to that of naturally occurring minerals akageneite and lepidocrocite. Micro- and mesoporosity were improved due to pillaring and the layered smectite structure was retained. (c) 2012 Elsevier Inc. All rights reserved.
T2  - Microporous and Mesoporous Materials
T1  - Synthesis and characterization of bentonites rich in beidellite with incorporated Al or Al-Fe oxide pillars
VL  - 165
SP  - 247
EP  - 256
DO  - 10.1016/j.micromeso.2012.08.029
ER  - 
@article{
author = "Bankovic, P. and Milutinovic-Nikolic, A. and Mojovic, Z. and Jovic-Jovicic, N. and Perović, Marija M. and Spasojević, Vojislav and Jovanović, Dragana J.",
year = "2013",
abstract = "Pillared clays (PILCs) based on bentonite clay from Bogovina (Serbia) were obtained using Al3+ and Fe3+ pillaring cations in different ratios. Thorough characterization of the starting material and PILCs was performed for better understanding of the catalytic activity that they had exibited in the catalytic wet peroxide oxidation (CWPO) of organic pollutants in water. The characterization consisted of the following techniques: XRD, XRD of oriented samples (swelling test), Greene-Kelley test (smectite type determination), TGA/DTA followed by XRD analysis of samples heated at characteristic temperatures, elemental analysis using ICP-OES and microwave digestion. FTIR, DR UV-Vis, Mossbauer spectroscopy, nitrogen physisorption at -196 degrees C and SEM imaging. Smectite in admixture with quartz was identified, together with impurities like feldspar, illite, chlorite and X-ray amorphous matter. Smectite mineral was dominantly of the beidellite type. Pillaring led to changes in the d(001) smectite basal spacing and stabilization of the smectite structure. Increasing Fe3+ content of the pillaring solutions resulted in the increased incorporation of iron into the PILCs as isolated octahedrally coordinated Fe3+ cations, smaller and bigger oligonuclear octahedrally coordinated Fe3+ species and octahedrally coordinated Fe3+ particles. The structure of incorporated pillars was similar to that of naturally occurring minerals akageneite and lepidocrocite. Micro- and mesoporosity were improved due to pillaring and the layered smectite structure was retained. (c) 2012 Elsevier Inc. All rights reserved.",
journal = "Microporous and Mesoporous Materials",
title = "Synthesis and characterization of bentonites rich in beidellite with incorporated Al or Al-Fe oxide pillars",
volume = "165",
pages = "247-256",
doi = "10.1016/j.micromeso.2012.08.029"
}
Bankovic, P., Milutinovic-Nikolic, A., Mojovic, Z., Jovic-Jovicic, N., Perović, M. M., Spasojević, V.,& Jovanović, D. J.. (2013). Synthesis and characterization of bentonites rich in beidellite with incorporated Al or Al-Fe oxide pillars. in Microporous and Mesoporous Materials, 165, 247-256.
https://doi.org/10.1016/j.micromeso.2012.08.029
Bankovic P, Milutinovic-Nikolic A, Mojovic Z, Jovic-Jovicic N, Perović MM, Spasojević V, Jovanović DJ. Synthesis and characterization of bentonites rich in beidellite with incorporated Al or Al-Fe oxide pillars. in Microporous and Mesoporous Materials. 2013;165:247-256.
doi:10.1016/j.micromeso.2012.08.029 .
Bankovic, P., Milutinovic-Nikolic, A., Mojovic, Z., Jovic-Jovicic, N., Perović, Marija M., Spasojević, Vojislav, Jovanović, Dragana J., "Synthesis and characterization of bentonites rich in beidellite with incorporated Al or Al-Fe oxide pillars" in Microporous and Mesoporous Materials, 165 (2013):247-256,
https://doi.org/10.1016/j.micromeso.2012.08.029 . .
42
39
41

Magnetne relaksacije i memorijski efekti u interagujućim nanočestičnim manganitima i oksidima gvožđa

Perović, Marija M.

(Универзитет у Београду, Физички факултет, 2013)

TY  - THES
AU  - Perović, Marija M.
PY  - 2013
UR  - http://eteze.bg.ac.rs/application/showtheses?thesesId=1278
UR  - https://fedorabg.bg.ac.rs/fedora/get/o:8141/bdef:Content/download
UR  - http://vbs.rs/scripts/cobiss?command=DISPLAY&base=70036&RID=
UR  - http://nardus.mpn.gov.rs/123456789/3200
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/7265
AB  - Iako je razumevanje neravnotežnih relaksacionih fenomena u spinskim staklima sličnim(SSG) sistemima od velikog interesa kako sa teorijskog, tako i sa stanovišta mogućihprimena, osnovni fizički mehanizmi još uvek nisu u potpunosti shvaćeni. Iz tog razloga se ufokusu eksperimentalnog istraživanja predstavljenog u ovoj doktorskoj disertaciji nalazemagnetni relaksacioni fenomeni, koji su proučavani u dve grupe nanočestičnih materijala,manganitima i oksidima gvožđa. Posebna pažnja posvećena je ispitivanju uticajameđučestičnih interakcija na pojavu niskotemperaturskog kolektivnog stanja, kao i namagnetne osobine sistema jednodomenskih čestica. Sistematsko proučavanje kompleksneneravnotežne dinamike kroz ispitivanje magnetnih relaksacija, starenja i memorijskih efekataizvedeno je na osnovu sveobuhvatnih merenja magnetizacije u magnetnom poljujednosmerne (DC) i naizmenične (AC) struje...
AB  - Although the understanding of nonequillibrium relaxation phenomena in super spin glass(SSG) nanoparticle systems is of the great importance from both fundamental andtechnological point of view, the underlying physical processes are still not explained. For thatreason, the experimental research presented in this thesis is focused on magnetic relaxation intwo strongly interacting nanoparticle systems, manganites and iron oxides. The main goal ofthe study was to investigate the effect of interparticle interaction on the magnetic propertiesof single domain magnetic particles as well as to determine its importance on the formationof low temperature collective state. The complex nonequillibrium dynamics was revealedthrough the systematic investigations of magnetic relaxations, aging and memory effects bymeans of DC and AC magnetization measurements...
PB  - Универзитет у Београду, Физички факултет
T2  - Универзитет у Београду
T1  - Magnetne relaksacije i memorijski efekti u interagujućim nanočestičnim manganitima i oksidima gvožđa
T1  - Magnetic relaxation and memory effects in interacting nanoparticle manganites and iron oxides
UR  - https://hdl.handle.net/21.15107/rcub_nardus_3200
ER  - 
@phdthesis{
author = "Perović, Marija M.",
year = "2013",
abstract = "Iako je razumevanje neravnotežnih relaksacionih fenomena u spinskim staklima sličnim(SSG) sistemima od velikog interesa kako sa teorijskog, tako i sa stanovišta mogućihprimena, osnovni fizički mehanizmi još uvek nisu u potpunosti shvaćeni. Iz tog razloga se ufokusu eksperimentalnog istraživanja predstavljenog u ovoj doktorskoj disertaciji nalazemagnetni relaksacioni fenomeni, koji su proučavani u dve grupe nanočestičnih materijala,manganitima i oksidima gvožđa. Posebna pažnja posvećena je ispitivanju uticajameđučestičnih interakcija na pojavu niskotemperaturskog kolektivnog stanja, kao i namagnetne osobine sistema jednodomenskih čestica. Sistematsko proučavanje kompleksneneravnotežne dinamike kroz ispitivanje magnetnih relaksacija, starenja i memorijskih efekataizvedeno je na osnovu sveobuhvatnih merenja magnetizacije u magnetnom poljujednosmerne (DC) i naizmenične (AC) struje..., Although the understanding of nonequillibrium relaxation phenomena in super spin glass(SSG) nanoparticle systems is of the great importance from both fundamental andtechnological point of view, the underlying physical processes are still not explained. For thatreason, the experimental research presented in this thesis is focused on magnetic relaxation intwo strongly interacting nanoparticle systems, manganites and iron oxides. The main goal ofthe study was to investigate the effect of interparticle interaction on the magnetic propertiesof single domain magnetic particles as well as to determine its importance on the formationof low temperature collective state. The complex nonequillibrium dynamics was revealedthrough the systematic investigations of magnetic relaxations, aging and memory effects bymeans of DC and AC magnetization measurements...",
publisher = "Универзитет у Београду, Физички факултет",
journal = "Универзитет у Београду",
title = "Magnetne relaksacije i memorijski efekti u interagujućim nanočestičnim manganitima i oksidima gvožđa, Magnetic relaxation and memory effects in interacting nanoparticle manganites and iron oxides",
url = "https://hdl.handle.net/21.15107/rcub_nardus_3200"
}
Perović, M. M.. (2013). Magnetne relaksacije i memorijski efekti u interagujućim nanočestičnim manganitima i oksidima gvožđa. in Универзитет у Београду
Универзитет у Београду, Физички факултет..
https://hdl.handle.net/21.15107/rcub_nardus_3200
Perović MM. Magnetne relaksacije i memorijski efekti u interagujućim nanočestičnim manganitima i oksidima gvožđa. in Универзитет у Београду. 2013;.
https://hdl.handle.net/21.15107/rcub_nardus_3200 .
Perović, Marija M., "Magnetne relaksacije i memorijski efekti u interagujućim nanočestičnim manganitima i oksidima gvožđa" in Универзитет у Београду (2013),
https://hdl.handle.net/21.15107/rcub_nardus_3200 .

An integrated study of thermal treatment effects on the microstructure and magnetic properties of Zn-ferrite nanoparticles

Antić, Bratislav; Perović, Marija M.; Kremenović, Aleksandar S.; Blanuša, Jovan; Spasojević, Vojislav; Vulic, Predrag; Bessais, Lotfi; Božin, Emil S.

(2013)

TY  - JOUR
AU  - Antić, Bratislav
AU  - Perović, Marija M.
AU  - Kremenović, Aleksandar S.
AU  - Blanuša, Jovan
AU  - Spasojević, Vojislav
AU  - Vulic, Predrag
AU  - Bessais, Lotfi
AU  - Božin, Emil S.
PY  - 2013
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/5305
AB  - The evolution of the magnetic state, crystal structure and microstructure parameters of nanocrystalline zinc-ferrite, tuned by thermal annealing of similar to 4 nm nanoparticles, was systematically studied by complementary characterization methods. Structural analysis of neutron and synchrotron x-ray radiation data revealed a mixed cation distribution in the nanoparticle samples, with the degree of inversion systematically decreasing from 0.25 in an as-prepared nanocrystalline sample to a non-inverted spinel structure with a normal cation distribution in the bulk counterpart. The results of DC magnetization and Mossbauer spectroscopy experiments indicated a superparamagnetic relaxation in similar to 4 nm nanoparticles, albeit with different freezing temperatures T-f of 27.5 K and 46 K, respectively. The quadrupole splitting parameter decreases with the annealing temperature due to cation redistribution between the tetrahedral and octahedral sites of the spinel structure and the associated defects. DC magnetization measurements indicated the existence of significant interparticle interactions among nanoparticles (superspins). Additional confirmation for the presence of interparticle interactions was found from the fit of the Tf(H) dependence to the AT line, from which a value of the anisotropy constant of K-eff = 5.6 x 10(5) erg cm(-3) was deduced. Further evidence for strong interparticle interactions was found from AC susceptibility measurements, where the frequency dependence of the freezing temperature T-f(f) was satisfactory described by both Vogel-Fulcher and dynamic scaling theory, both applicable for interacting systems. The parameters obtained from these fits suggest collective freezing of magnetic moments at T-f.
T2  - Journal of Physics: Condensed Matter
T1  - An integrated study of thermal treatment effects on the microstructure and magnetic properties of Zn-ferrite nanoparticles
VL  - 25
IS  - 8
DO  - 10.1088/0953-8984/25/8/086001
ER  - 
@article{
author = "Antić, Bratislav and Perović, Marija M. and Kremenović, Aleksandar S. and Blanuša, Jovan and Spasojević, Vojislav and Vulic, Predrag and Bessais, Lotfi and Božin, Emil S.",
year = "2013",
abstract = "The evolution of the magnetic state, crystal structure and microstructure parameters of nanocrystalline zinc-ferrite, tuned by thermal annealing of similar to 4 nm nanoparticles, was systematically studied by complementary characterization methods. Structural analysis of neutron and synchrotron x-ray radiation data revealed a mixed cation distribution in the nanoparticle samples, with the degree of inversion systematically decreasing from 0.25 in an as-prepared nanocrystalline sample to a non-inverted spinel structure with a normal cation distribution in the bulk counterpart. The results of DC magnetization and Mossbauer spectroscopy experiments indicated a superparamagnetic relaxation in similar to 4 nm nanoparticles, albeit with different freezing temperatures T-f of 27.5 K and 46 K, respectively. The quadrupole splitting parameter decreases with the annealing temperature due to cation redistribution between the tetrahedral and octahedral sites of the spinel structure and the associated defects. DC magnetization measurements indicated the existence of significant interparticle interactions among nanoparticles (superspins). Additional confirmation for the presence of interparticle interactions was found from the fit of the Tf(H) dependence to the AT line, from which a value of the anisotropy constant of K-eff = 5.6 x 10(5) erg cm(-3) was deduced. Further evidence for strong interparticle interactions was found from AC susceptibility measurements, where the frequency dependence of the freezing temperature T-f(f) was satisfactory described by both Vogel-Fulcher and dynamic scaling theory, both applicable for interacting systems. The parameters obtained from these fits suggest collective freezing of magnetic moments at T-f.",
journal = "Journal of Physics: Condensed Matter",
title = "An integrated study of thermal treatment effects on the microstructure and magnetic properties of Zn-ferrite nanoparticles",
volume = "25",
number = "8",
doi = "10.1088/0953-8984/25/8/086001"
}
Antić, B., Perović, M. M., Kremenović, A. S., Blanuša, J., Spasojević, V., Vulic, P., Bessais, L.,& Božin, E. S.. (2013). An integrated study of thermal treatment effects on the microstructure and magnetic properties of Zn-ferrite nanoparticles. in Journal of Physics: Condensed Matter, 25(8).
https://doi.org/10.1088/0953-8984/25/8/086001
Antić B, Perović MM, Kremenović AS, Blanuša J, Spasojević V, Vulic P, Bessais L, Božin ES. An integrated study of thermal treatment effects on the microstructure and magnetic properties of Zn-ferrite nanoparticles. in Journal of Physics: Condensed Matter. 2013;25(8).
doi:10.1088/0953-8984/25/8/086001 .
Antić, Bratislav, Perović, Marija M., Kremenović, Aleksandar S., Blanuša, Jovan, Spasojević, Vojislav, Vulic, Predrag, Bessais, Lotfi, Božin, Emil S., "An integrated study of thermal treatment effects on the microstructure and magnetic properties of Zn-ferrite nanoparticles" in Journal of Physics: Condensed Matter, 25, no. 8 (2013),
https://doi.org/10.1088/0953-8984/25/8/086001 . .
20
21
22

Combustion synthesis as a novel approach in preparation of polycrystalline Y2Cu2O5

Gebrel, Z.; Blanuša, Jovan; Spasojević, Vojislav; Kusigerski, Vladan; Mraković, Ana Đ.; Alqat, A.; Perović, Marija M.

(2013)

TY  - JOUR
AU  - Gebrel, Z.
AU  - Blanuša, Jovan
AU  - Spasojević, Vojislav
AU  - Kusigerski, Vladan
AU  - Mraković, Ana Đ.
AU  - Alqat, A.
AU  - Perović, Marija M.
PY  - 2013
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/5515
AB  - Polycrystalline samples of Y2Cu2O5 were for the first time sintered from precursors obtained by two combustion routes - the glycine-nitrate method (sample S1) and a modified self-propagating high-temperature synthesis (sample S2). The detailed X-ray diffraction analysis has confirmed that both samples are well crystallized and single phase, with the high crystallization degree and cation ordering within a Cu sublattice. Magnetic characterization has shown magnetic behavior typical of pure Y2Cu2O5. The distinctive advantages of these new synthesis routes in comparison to the ceramic sintering are in simplification of the overall procedure as well as in a significant reduction of synthesis duration from several days down to 31 h (S1) or 12 h (S2). (C) 2013 Elsevier B.V. All rights reserved.
T2  - Journal of Alloys and Compounds
T1  - Combustion synthesis as a novel approach in preparation of polycrystalline Y2Cu2O5
VL  - 568
SP  - 55
EP  - 59
DO  - 10.1016/j.jallcom.2013.03.133
ER  - 
@article{
author = "Gebrel, Z. and Blanuša, Jovan and Spasojević, Vojislav and Kusigerski, Vladan and Mraković, Ana Đ. and Alqat, A. and Perović, Marija M.",
year = "2013",
abstract = "Polycrystalline samples of Y2Cu2O5 were for the first time sintered from precursors obtained by two combustion routes - the glycine-nitrate method (sample S1) and a modified self-propagating high-temperature synthesis (sample S2). The detailed X-ray diffraction analysis has confirmed that both samples are well crystallized and single phase, with the high crystallization degree and cation ordering within a Cu sublattice. Magnetic characterization has shown magnetic behavior typical of pure Y2Cu2O5. The distinctive advantages of these new synthesis routes in comparison to the ceramic sintering are in simplification of the overall procedure as well as in a significant reduction of synthesis duration from several days down to 31 h (S1) or 12 h (S2). (C) 2013 Elsevier B.V. All rights reserved.",
journal = "Journal of Alloys and Compounds",
title = "Combustion synthesis as a novel approach in preparation of polycrystalline Y2Cu2O5",
volume = "568",
pages = "55-59",
doi = "10.1016/j.jallcom.2013.03.133"
}
Gebrel, Z., Blanuša, J., Spasojević, V., Kusigerski, V., Mraković, A. Đ., Alqat, A.,& Perović, M. M.. (2013). Combustion synthesis as a novel approach in preparation of polycrystalline Y2Cu2O5. in Journal of Alloys and Compounds, 568, 55-59.
https://doi.org/10.1016/j.jallcom.2013.03.133
Gebrel Z, Blanuša J, Spasojević V, Kusigerski V, Mraković AĐ, Alqat A, Perović MM. Combustion synthesis as a novel approach in preparation of polycrystalline Y2Cu2O5. in Journal of Alloys and Compounds. 2013;568:55-59.
doi:10.1016/j.jallcom.2013.03.133 .
Gebrel, Z., Blanuša, Jovan, Spasojević, Vojislav, Kusigerski, Vladan, Mraković, Ana Đ., Alqat, A., Perović, Marija M., "Combustion synthesis as a novel approach in preparation of polycrystalline Y2Cu2O5" in Journal of Alloys and Compounds, 568 (2013):55-59,
https://doi.org/10.1016/j.jallcom.2013.03.133 . .
1
2
2

Modified self-propagating high-temperature synthesis of nanosized La0.7Ca0.3MnO3

Mraković, Ana Đ.; Blanuša, Jovan; Primc, Darinka; Perović, Marija M.; Jaglicic, Zvonko; Kusigerski, Vladan; Spasojević, Vojislav

(2013)

TY  - JOUR
AU  - Mraković, Ana Đ.
AU  - Blanuša, Jovan
AU  - Primc, Darinka
AU  - Perović, Marija M.
AU  - Jaglicic, Zvonko
AU  - Kusigerski, Vladan
AU  - Spasojević, Vojislav
PY  - 2013
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/5463
AB  - A modified solid-state combustion route was developed for the preparation of nanocrystalline manganite La0.7Ca0.3MnO3 in a single-step process, using metal nitrates and glucose/KNO3 redox mixture. The obtained sample was found to crystallize within O type of orthorhombic perovskite structure (space group Pnma), without the presence of other structural phases or impurities. Nanoparticles are found to have particle size in the range 12-35 nm, and to be highly crystalline without the presence of amorphous surface layer. Magnetic measurements show that nanoparticles display bulk-like magnetic properties, with ferromagnetic phase transition at 125 K and the absence of superparamagnetic or spin-glass behavior. (C) 2012 Elsevier Ltd and Techna Group S.r.l. All rights reserved.
T2  - Ceramics International
T1  - Modified self-propagating high-temperature synthesis of nanosized La0.7Ca0.3MnO3
VL  - 39
IS  - 4
SP  - 3771
EP  - 3777
DO  - 10.1016/j.ceramint.2012.10.216
ER  - 
@article{
author = "Mraković, Ana Đ. and Blanuša, Jovan and Primc, Darinka and Perović, Marija M. and Jaglicic, Zvonko and Kusigerski, Vladan and Spasojević, Vojislav",
year = "2013",
abstract = "A modified solid-state combustion route was developed for the preparation of nanocrystalline manganite La0.7Ca0.3MnO3 in a single-step process, using metal nitrates and glucose/KNO3 redox mixture. The obtained sample was found to crystallize within O type of orthorhombic perovskite structure (space group Pnma), without the presence of other structural phases or impurities. Nanoparticles are found to have particle size in the range 12-35 nm, and to be highly crystalline without the presence of amorphous surface layer. Magnetic measurements show that nanoparticles display bulk-like magnetic properties, with ferromagnetic phase transition at 125 K and the absence of superparamagnetic or spin-glass behavior. (C) 2012 Elsevier Ltd and Techna Group S.r.l. All rights reserved.",
journal = "Ceramics International",
title = "Modified self-propagating high-temperature synthesis of nanosized La0.7Ca0.3MnO3",
volume = "39",
number = "4",
pages = "3771-3777",
doi = "10.1016/j.ceramint.2012.10.216"
}
Mraković, A. Đ., Blanuša, J., Primc, D., Perović, M. M., Jaglicic, Z., Kusigerski, V.,& Spasojević, V.. (2013). Modified self-propagating high-temperature synthesis of nanosized La0.7Ca0.3MnO3. in Ceramics International, 39(4), 3771-3777.
https://doi.org/10.1016/j.ceramint.2012.10.216
Mraković AĐ, Blanuša J, Primc D, Perović MM, Jaglicic Z, Kusigerski V, Spasojević V. Modified self-propagating high-temperature synthesis of nanosized La0.7Ca0.3MnO3. in Ceramics International. 2013;39(4):3771-3777.
doi:10.1016/j.ceramint.2012.10.216 .
Mraković, Ana Đ., Blanuša, Jovan, Primc, Darinka, Perović, Marija M., Jaglicic, Zvonko, Kusigerski, Vladan, Spasojević, Vojislav, "Modified self-propagating high-temperature synthesis of nanosized La0.7Ca0.3MnO3" in Ceramics International, 39, no. 4 (2013):3771-3777,
https://doi.org/10.1016/j.ceramint.2012.10.216 . .
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17

An ac susceptibility study of spin dynamics in a super spin glass nanoparticle La0.7Ca0.3MnO3 system: simultaneous relaxation processes

Perović, Marija M.; Kusigerski, Vladan; Spasojević, Vojislav; Mraković, Ana Đ.; Blanuša, Jovan; Zentkova, M.; Mihalik, M.

(2013)

TY  - JOUR
AU  - Perović, Marija M.
AU  - Kusigerski, Vladan
AU  - Spasojević, Vojislav
AU  - Mraković, Ana Đ.
AU  - Blanuša, Jovan
AU  - Zentkova, M.
AU  - Mihalik, M.
PY  - 2013
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/5395
AB  - In this paper, we present the results of a systematic study of nonequilibrium dynamics in a strongly interacting super spin glass (SSG) nanoparticle La0.7Ca0.3MnO3 system by alternating current (ac) susceptibility measurements. Cole-Cole analysis of the obtained data revealed the simultaneous existence of two separated relaxation processes, which can be assigned to the relaxation of different magnetic entities. Along with the expected relaxation of the collective SSG phase, the existence of individual, nonagglomerated particles, which do not take part in the collective phase and relax independently, was proposed. A full dynamical scaling analysis was performed in order to elucidate the nature of the transition to a low-temperature SSG state in the interacting La0.7Ca0.3MnO3 nanoparticle sample.
T2  - Journal of Physics. D: Applied Physics
T1  - An ac susceptibility study of spin dynamics in a super spin glass nanoparticle La0.7Ca0.3MnO3 system: simultaneous relaxation processes
VL  - 46
IS  - 16
DO  - 10.1088/0022-3727/46/16/165001
ER  - 
@article{
author = "Perović, Marija M. and Kusigerski, Vladan and Spasojević, Vojislav and Mraković, Ana Đ. and Blanuša, Jovan and Zentkova, M. and Mihalik, M.",
year = "2013",
abstract = "In this paper, we present the results of a systematic study of nonequilibrium dynamics in a strongly interacting super spin glass (SSG) nanoparticle La0.7Ca0.3MnO3 system by alternating current (ac) susceptibility measurements. Cole-Cole analysis of the obtained data revealed the simultaneous existence of two separated relaxation processes, which can be assigned to the relaxation of different magnetic entities. Along with the expected relaxation of the collective SSG phase, the existence of individual, nonagglomerated particles, which do not take part in the collective phase and relax independently, was proposed. A full dynamical scaling analysis was performed in order to elucidate the nature of the transition to a low-temperature SSG state in the interacting La0.7Ca0.3MnO3 nanoparticle sample.",
journal = "Journal of Physics. D: Applied Physics",
title = "An ac susceptibility study of spin dynamics in a super spin glass nanoparticle La0.7Ca0.3MnO3 system: simultaneous relaxation processes",
volume = "46",
number = "16",
doi = "10.1088/0022-3727/46/16/165001"
}
Perović, M. M., Kusigerski, V., Spasojević, V., Mraković, A. Đ., Blanuša, J., Zentkova, M.,& Mihalik, M.. (2013). An ac susceptibility study of spin dynamics in a super spin glass nanoparticle La0.7Ca0.3MnO3 system: simultaneous relaxation processes. in Journal of Physics. D: Applied Physics, 46(16).
https://doi.org/10.1088/0022-3727/46/16/165001
Perović MM, Kusigerski V, Spasojević V, Mraković AĐ, Blanuša J, Zentkova M, Mihalik M. An ac susceptibility study of spin dynamics in a super spin glass nanoparticle La0.7Ca0.3MnO3 system: simultaneous relaxation processes. in Journal of Physics. D: Applied Physics. 2013;46(16).
doi:10.1088/0022-3727/46/16/165001 .
Perović, Marija M., Kusigerski, Vladan, Spasojević, Vojislav, Mraković, Ana Đ., Blanuša, Jovan, Zentkova, M., Mihalik, M., "An ac susceptibility study of spin dynamics in a super spin glass nanoparticle La0.7Ca0.3MnO3 system: simultaneous relaxation processes" in Journal of Physics. D: Applied Physics, 46, no. 16 (2013),
https://doi.org/10.1088/0022-3727/46/16/165001 . .
13
12
15

Relaxation phenomena in super spin glass nanoparticle manganite La0.7Ca0.3MnO3

Perović, Marija M.; Mraković, Ana Đ.; Kusigerski, Vladan; Blanuša, Jovan; Spasojević, Vojislav

(2012)

TY  - JOUR
AU  - Perović, Marija M.
AU  - Mraković, Ana Đ.
AU  - Kusigerski, Vladan
AU  - Blanuša, Jovan
AU  - Spasojević, Vojislav
PY  - 2012
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/5059
AB  - Investigation of complex, nonequilibrium dynamics of super spin glass nanoparticle La0.7Ca0.3MnO3 sample was conducted through the comprehensive set of magnetization relaxation measurements. It comprised measurements of thermoremanent and zero-field cooled magnetization time decay under various temperature and field conditions, as well as study of the ageing effect for different waiting times. A variety of theoretical models dealing with nonequilibrium dynamics in spin glasses was successfully implemented in the description of experimentally observed relaxation phenomena. Collective behaviour observed at low temperatures and intermediate magnetic fields was found to be the consequence of the random orientation of easy axes and significant dipolar interactions between nanoparticle moments. (c) 2012 Elsevier B.V. All rights reserved.
T2  - Materials Chemistry and Physics
T1  - Relaxation phenomena in super spin glass nanoparticle manganite La0.7Ca0.3MnO3
VL  - 136
IS  - 1
SP  - 196
EP  - 204
DO  - 10.1016/j.matchemphys.2012.06.052
ER  - 
@article{
author = "Perović, Marija M. and Mraković, Ana Đ. and Kusigerski, Vladan and Blanuša, Jovan and Spasojević, Vojislav",
year = "2012",
abstract = "Investigation of complex, nonequilibrium dynamics of super spin glass nanoparticle La0.7Ca0.3MnO3 sample was conducted through the comprehensive set of magnetization relaxation measurements. It comprised measurements of thermoremanent and zero-field cooled magnetization time decay under various temperature and field conditions, as well as study of the ageing effect for different waiting times. A variety of theoretical models dealing with nonequilibrium dynamics in spin glasses was successfully implemented in the description of experimentally observed relaxation phenomena. Collective behaviour observed at low temperatures and intermediate magnetic fields was found to be the consequence of the random orientation of easy axes and significant dipolar interactions between nanoparticle moments. (c) 2012 Elsevier B.V. All rights reserved.",
journal = "Materials Chemistry and Physics",
title = "Relaxation phenomena in super spin glass nanoparticle manganite La0.7Ca0.3MnO3",
volume = "136",
number = "1",
pages = "196-204",
doi = "10.1016/j.matchemphys.2012.06.052"
}
Perović, M. M., Mraković, A. Đ., Kusigerski, V., Blanuša, J.,& Spasojević, V.. (2012). Relaxation phenomena in super spin glass nanoparticle manganite La0.7Ca0.3MnO3. in Materials Chemistry and Physics, 136(1), 196-204.
https://doi.org/10.1016/j.matchemphys.2012.06.052
Perović MM, Mraković AĐ, Kusigerski V, Blanuša J, Spasojević V. Relaxation phenomena in super spin glass nanoparticle manganite La0.7Ca0.3MnO3. in Materials Chemistry and Physics. 2012;136(1):196-204.
doi:10.1016/j.matchemphys.2012.06.052 .
Perović, Marija M., Mraković, Ana Đ., Kusigerski, Vladan, Blanuša, Jovan, Spasojević, Vojislav, "Relaxation phenomena in super spin glass nanoparticle manganite La0.7Ca0.3MnO3" in Materials Chemistry and Physics, 136, no. 1 (2012):196-204,
https://doi.org/10.1016/j.matchemphys.2012.06.052 . .
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