Lyon, Keenan

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  • Lyon, Keenan (1)
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Analytical modeling of electron energy loss spectroscopy of graphene: Ab initio study versus extended hydrodynamic model

Đorđević, Tijana; Radović, Ivan; Despoja, Vito; Lyon, Keenan; Borka, Duško; Mišković, Zoran L.

(2018)

TY  - JOUR
AU  - Đorđević, Tijana
AU  - Radović, Ivan
AU  - Despoja, Vito
AU  - Lyon, Keenan
AU  - Borka, Duško
AU  - Mišković, Zoran L.
PY  - 2018
UR  - https://vinar.vin.bg.ac.rs/handle/123456789/1831
AB  - We present an analytical modeling of the electron energy loss (EEL) spectroscopy data for free-standing graphene obtained by scanning transmission electron microscope. The probability density for energy loss of fast electrons traversing graphene under normal incidence is evaluated using an optical approximation based on the conductivity of graphene given in the local, i.e., frequency-dependent form derived by both a two-dimensional, two-fluid extended hydrodynamic (eHD) model and an ab initio method. We compare the results for the real and imaginary parts of the optical conductivity in graphene obtained by these two methods. The calculated probability density is directly compared with the EEL spectra from three independent experiments and we find very good agreement, especially in the case of the eHD model. Furthermore, we point out that the subtraction of the zero-loss peak from the experimental EEL spectra has a strong influence on the analytical model for the EEL spectroscopy data. (C) 2017 Elsevier B.V. All rights reserved.
T2  - Ultramicroscopy
T1  - Analytical modeling of electron energy loss spectroscopy of graphene: Ab initio study versus extended hydrodynamic model
VL  - 184
SP  - 134
EP  - 142
DO  - 10.1016/j.ultramic.2017.08.014
ER  - 
@article{
author = "Đorđević, Tijana and Radović, Ivan and Despoja, Vito and Lyon, Keenan and Borka, Duško and Mišković, Zoran L.",
year = "2018",
abstract = "We present an analytical modeling of the electron energy loss (EEL) spectroscopy data for free-standing graphene obtained by scanning transmission electron microscope. The probability density for energy loss of fast electrons traversing graphene under normal incidence is evaluated using an optical approximation based on the conductivity of graphene given in the local, i.e., frequency-dependent form derived by both a two-dimensional, two-fluid extended hydrodynamic (eHD) model and an ab initio method. We compare the results for the real and imaginary parts of the optical conductivity in graphene obtained by these two methods. The calculated probability density is directly compared with the EEL spectra from three independent experiments and we find very good agreement, especially in the case of the eHD model. Furthermore, we point out that the subtraction of the zero-loss peak from the experimental EEL spectra has a strong influence on the analytical model for the EEL spectroscopy data. (C) 2017 Elsevier B.V. All rights reserved.",
journal = "Ultramicroscopy",
title = "Analytical modeling of electron energy loss spectroscopy of graphene: Ab initio study versus extended hydrodynamic model",
volume = "184",
pages = "134-142",
doi = "10.1016/j.ultramic.2017.08.014"
}
Đorđević, T., Radović, I., Despoja, V., Lyon, K., Borka, D.,& Mišković, Z. L.. (2018). Analytical modeling of electron energy loss spectroscopy of graphene: Ab initio study versus extended hydrodynamic model. in Ultramicroscopy, 184, 134-142.
https://doi.org/10.1016/j.ultramic.2017.08.014
Đorđević T, Radović I, Despoja V, Lyon K, Borka D, Mišković ZL. Analytical modeling of electron energy loss spectroscopy of graphene: Ab initio study versus extended hydrodynamic model. in Ultramicroscopy. 2018;184:134-142.
doi:10.1016/j.ultramic.2017.08.014 .
Đorđević, Tijana, Radović, Ivan, Despoja, Vito, Lyon, Keenan, Borka, Duško, Mišković, Zoran L., "Analytical modeling of electron energy loss spectroscopy of graphene: Ab initio study versus extended hydrodynamic model" in Ultramicroscopy, 184 (2018):134-142,
https://doi.org/10.1016/j.ultramic.2017.08.014 . .
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