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dc.creatorJovanović, Svetlana P.
dc.creatorSyrgiannis, Zois
dc.creatorMarković, Zoran M.
dc.creatorBonasera, Aurelio
dc.creatorKepić, Dejan P.
dc.creatorBudimir, Milica
dc.creatorMilivojević, Dušan
dc.creatorSpasojević, Vuk D.
dc.creatorDramićanin, Miroslav
dc.creatorPavlović, Vladimir B.
dc.creatorTodorović-Marković, Biljana
dc.date.accessioned2018-03-01T16:33:24Z
dc.date.available2018-03-01T16:33:24Z
dc.date.issued2015
dc.identifier.issn1944-8244 (print)
dc.identifier.urihttp://vinar.vin.bg.ac.rs/handle/123456789/839
dc.description.abstractHerein, the ability of gamma irradiation to enhance the photoluminescence properties of graphene quantum dots (GQDs) was investigated. Different doses of gamma-irradiation were used on GQDs to examine the way in which their structure and optical properties can be affected. The photoluminescence quantum yield was increased six times for the GQDs irradiated with high doses compared to the nonirradiated material. Both photoluminescence lifetime and values of optical band gap were increased with the dose of applied gamma irradiation. In addition, the exploitation of the gamma-irradiated GQDs as photosensitizers was examined by monitoring the production of singlet oxygen under UV illumination. The main outcome was that the GQDs irradiated at lower doses act as better photoproducers than the ones irradiated at higher doses. These results corroborate that the structural changes caused by gamma irradiation have a direct impact on GQD ability to produce singlet oxygen and their photostability under prolonged UV illumination. This makes low-dose irradiated GQDs promising candidates for photodynamic therapy.en
dc.relationinfo:eu-repo/grantAgreement/MESTD/Basic Research (BR or ON)/172003/RS//
dc.rightsrestrictedAccessen
dc.sourceACS Applied Materials and Interfacesen
dc.subjectgraphene quantum dotsen
dc.subjectgamma irradiationen
dc.subjectphotoluminescenceen
dc.subjectquantum yielden
dc.subjectphotodynamic therapyen
dc.titleModification of Structural and Luminescence Properties of Graphene Quantum Dots by Gamma Irradiation and Their Application in a Photodynamic Therapyen
dc.typearticleen
dcterms.abstractМиливојевић Душан; Драмићанин Мирослав; Тодоровић-Марковић Биљана; Марковић Зоран; Будимир Милица; Спасојевиц, Вук Д.; Сyргианнис, Зоис; Јовановиц, Светлана П.; Бонасера, Aурелио; Кепић Дејан; Павловиц, Владимир Б.;
dc.citation.volume7
dc.citation.issue46
dc.citation.spage25865
dc.citation.epage25874
dc.identifier.wos000366005600040
dc.identifier.doi10.1021/acsami.5b08226
dc.citation.rankM21a
dc.identifier.pmid26540316
dc.identifier.scopus2-s2.0-84948682203


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