Efficiency of Ni Nanoparticles Supported on Hierarchical Porous Nitrogen-Doped Carbon for Hydrogenolysis of Kraft Lignin in Flow and Batch Systems
Authorized Users Only
2017
Authors
Lama, Sandy M. G.Pampel, Jonas
Fellinger, Tim-Patrick
Beškoski, Vladimir P.
Slavković-Beškoski, Latinka J.
Antonietti, Markus
Molinari, Valerio
Article (Published version)
Metadata
Show full item recordAbstract
Ni nanoparticles supported on nitrogen-doped carbon (NDC) prepared via salt-melt synthesis with a hierarchical porosity were successfully applied as the catalyst for the degradation of Kraft lignin. It is shown that Ni-NDC is more efficient when compared to Ni nanoparticles deposited on an N-free carbon support, prepared with similar porosity features (Ni-C) and to Ni nanoparticles deposited on a commercial carbon (Ni-Cref). The efficiency of these materials was compared for reactions performed both in batch and flow reactors, highlighting the effect of the reactor setup on the stability of the recovered catalysts.
Keywords:
Kraft lignin / Heterogeneous catalysis / Nitrogen-doped carbon / Nickel / Hydrogenation / Porosity / Flow and batch system / Hierarchical porositySource:
ACS Sustainable Chemistry and Engineering, 2017, 5, 3, 2415-2420Funding / projects:
- Max Planck Institute
DOI: 10.1021/acssuschemeng.6b02761
ISSN: 2168-0485
WoS: 000395846900045
Scopus: 2-s2.0-85014533837
Collections
Institution/Community
VinčaTY - JOUR AU - Lama, Sandy M. G. AU - Pampel, Jonas AU - Fellinger, Tim-Patrick AU - Beškoski, Vladimir P. AU - Slavković-Beškoski, Latinka J. AU - Antonietti, Markus AU - Molinari, Valerio PY - 2017 UR - https://vinar.vin.bg.ac.rs/handle/123456789/1447 AB - Ni nanoparticles supported on nitrogen-doped carbon (NDC) prepared via salt-melt synthesis with a hierarchical porosity were successfully applied as the catalyst for the degradation of Kraft lignin. It is shown that Ni-NDC is more efficient when compared to Ni nanoparticles deposited on an N-free carbon support, prepared with similar porosity features (Ni-C) and to Ni nanoparticles deposited on a commercial carbon (Ni-Cref). The efficiency of these materials was compared for reactions performed both in batch and flow reactors, highlighting the effect of the reactor setup on the stability of the recovered catalysts. T2 - ACS Sustainable Chemistry and Engineering T1 - Efficiency of Ni Nanoparticles Supported on Hierarchical Porous Nitrogen-Doped Carbon for Hydrogenolysis of Kraft Lignin in Flow and Batch Systems VL - 5 IS - 3 SP - 2415 EP - 2420 DO - 10.1021/acssuschemeng.6b02761 ER -
@article{ author = "Lama, Sandy M. G. and Pampel, Jonas and Fellinger, Tim-Patrick and Beškoski, Vladimir P. and Slavković-Beškoski, Latinka J. and Antonietti, Markus and Molinari, Valerio", year = "2017", abstract = "Ni nanoparticles supported on nitrogen-doped carbon (NDC) prepared via salt-melt synthesis with a hierarchical porosity were successfully applied as the catalyst for the degradation of Kraft lignin. It is shown that Ni-NDC is more efficient when compared to Ni nanoparticles deposited on an N-free carbon support, prepared with similar porosity features (Ni-C) and to Ni nanoparticles deposited on a commercial carbon (Ni-Cref). The efficiency of these materials was compared for reactions performed both in batch and flow reactors, highlighting the effect of the reactor setup on the stability of the recovered catalysts.", journal = "ACS Sustainable Chemistry and Engineering", title = "Efficiency of Ni Nanoparticles Supported on Hierarchical Porous Nitrogen-Doped Carbon for Hydrogenolysis of Kraft Lignin in Flow and Batch Systems", volume = "5", number = "3", pages = "2415-2420", doi = "10.1021/acssuschemeng.6b02761" }
Lama, S. M. G., Pampel, J., Fellinger, T., Beškoski, V. P., Slavković-Beškoski, L. J., Antonietti, M.,& Molinari, V.. (2017). Efficiency of Ni Nanoparticles Supported on Hierarchical Porous Nitrogen-Doped Carbon for Hydrogenolysis of Kraft Lignin in Flow and Batch Systems. in ACS Sustainable Chemistry and Engineering, 5(3), 2415-2420. https://doi.org/10.1021/acssuschemeng.6b02761
Lama SMG, Pampel J, Fellinger T, Beškoski VP, Slavković-Beškoski LJ, Antonietti M, Molinari V. Efficiency of Ni Nanoparticles Supported on Hierarchical Porous Nitrogen-Doped Carbon for Hydrogenolysis of Kraft Lignin in Flow and Batch Systems. in ACS Sustainable Chemistry and Engineering. 2017;5(3):2415-2420. doi:10.1021/acssuschemeng.6b02761 .
Lama, Sandy M. G., Pampel, Jonas, Fellinger, Tim-Patrick, Beškoski, Vladimir P., Slavković-Beškoski, Latinka J., Antonietti, Markus, Molinari, Valerio, "Efficiency of Ni Nanoparticles Supported on Hierarchical Porous Nitrogen-Doped Carbon for Hydrogenolysis of Kraft Lignin in Flow and Batch Systems" in ACS Sustainable Chemistry and Engineering, 5, no. 3 (2017):2415-2420, https://doi.org/10.1021/acssuschemeng.6b02761 . .